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Novel high-entropy oxides for energy storage and conversion:From fundamentals to practical applications

查看全文 作　　者：Zi-Yu [1,2]Liu;Yu [1,2]Liu;Yujie [1,2,3]Xu;Hualiang [1,2,3]Zhang;Zongping [4]Shao;Zhenbin [5]Wang;Haisheng [1,2,3,6]Chen 高影响力作者 机构地区：[1]Institute of Engineering Thermophysics,Chinese Academy of Sciences,Beijing,100190,China;[2]Nanjing Institute of Future Energy System,Institute of Engineering Thermophysics,Chinese Academy of Sciences,Nanjing,China;[3]University of Chinese Academy of Sciences,Beijing,100049,China;[4]Curtin University,Australia;[5]Department of Materials Science and Engineering,City University of Hong Kong,Kowloon,999077,Hong Kong,China;[6]Dalian National Laboratory for Clean Energy,Chinese Academy of Sciences,Dalian,116023,China高影响力机构 出　　处：《Green Energy & Environment》索引2023年第8卷第5期,共17页高影响力期刊 基　　金：The authors are thankful for the financial support from the Beijing Natural Science Foundation(No.3222050);the National Natural Science Foundation of China(Nos.22075304 and 52202324). 摘　　要：High-entropy oxides(HEOs)are gaining prominence in the field of electrochemistry due to their distinctive structural characteristics,which give rise to their advanced stable and modifiable functional properties.This review presents fundamental preparations,incidental characterizations,and typical structures of HEOs.The prospective applications of HEOs in various electrochemical aspects of electrocatalysis and energy conversion-storage are also summarized,including recent developments and the general trend of HEO structure design in the catalysis containing oxygen evolution reaction(OER)and oxygen reduction reaction(ORR),supercapacitors(SC),lithium-ion batteries(LIBs),solid oxide fuel cells(SOFCs),and so forth.Moreover,this review notes some apparent challenges and multiple opportunities for the use of HEOs in the wide field of energy to further guide the development of practical applications.The influence of entropy is significant,and high-entropy oxides are expected to drive the improvement of energy science and technology in the near future. 关 键 词：High-entropy oxides ELECTROCHEMISTRY Energy storage and conversion
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