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86篇 您的检索式:作者名="ALSHEHRI"
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1Recent advances in nanostructured heterogeneous catalysts for N-cycle electrocatalysis显示文摘To restore the natural nitrogen cycle(N-cycle),artificial N-cycle electrocatalysis with flexibility,sustainability,and compatibility can convert intermittent renewable energy(e.g.,wind)to harmful or value-added chemicals with minimal carbon emissions.The background of such N-cycles,such as nitrogen fixation,ammonia oxidation,and nitrate reduction,is briefly introduced here.The discussion of emerging nanostructures in various conversion reactions is focused on the architecture/compositional design,electrochemical performances,reaction mechanisms,and instructive tests.Energy device advancements for achieving more functions as well as in situ/operando characterizations toward understanding key steps are also highlighted.Furthermore,some recently proposed reactions as well as less discussed C-N coupling reactions are also summarized.We classify inorganic nitrogen sources that convert to each other under an applied voltage into three types,namely,abundant nitrogen,toxic nitrate(nitrite),and nitrogen oxides,and useful compounds such as ammonia,hydrazine,and hydroxylamine,with the goal of providing more critical insights into strategies to facilitate the development of our circular nitrogen economy.Jie Liang Qian Liu Abdulmohsen Ali Alshehri Xuping Sun 2022Nano Research Energy2022,1,2:8
2In situ grown Fe_(3)O_(4)particle on stainless steel:A highly efficient electrocatalyst for nitrate reduction to ammonia显示文摘NH_(3)is an essential feedstock for fertilizer synthesis.Industry-scale NH_(3)synthesis mostly relies on the Haber-Bosch method,however,which suffers from massive CO_(2) emission and high energy consumption.Electrocatalytic NO_(3)-reduction is an attractive substitute to the Haber-Bosch method for synthesizing NH_(3)under mild conditions.As this reaction will produce a variety of products,it highly desires efficient and selective electrocatalyst for NH_(3)generation.Here,we report in situ grown Fe_(3)O_(4)particle on stainless steel(Fe_(3)O_(4)/SS)as a high-efficiency electrocatalyst for NO_(3)^(-)reduction to NH_(3).In 0.1 M NaOH with 0.1 M NaNO_(3),such Fe_(3)O_(4)/SS reaches a remarkable Faradaic efficiency of 91.5%and a high NH_(3)yield of 10,145μg·h^(-1)·cm^(-2)at-0.5 V vs.reversible hydrogen electrode(RHE).Furthermore,it owns robust structural and electrochemical stability.This work provides useful guidelines to expand the scope of metallic oxide electrocatalysts for NH_(3)synthesis.The catalytic mechanism is uncovered and discussed further by theoretical calculations.Xiaoya Fan Lisi Xie Jie Liang Yuchun Ren Longcheng Zhang Luchao Yue Tingshuai Li Yonglan Luo Na Li Bo Tang Yang Liu Shuyan Gao Abdulmohsen Ali Alshehri Qian Liu Qingquan Kong Xuping Sun 2022Nano Research2022,15,4:7
3Benzoate anions-intercalated NiFe-layered double hydroxide nanosheet array with enhanced stability for electrochemical seawater oxidation显示文摘Seawater electrolysis is an extremely attractive approach for harvesting clean hydrogen energy,but detrimental chlorine species(i.e.,chloride and hypochlorite)cause severe corrosion at the anode.Here,we report our recent finding that benzoate anions-intercalated NiFe-layered double hydroxide nanosheet on carbon cloth(BZ-NiFe-LDH/CC)behaves as a highly efficient and durable monolithic catalyst for alkaline seawater oxidation,affords enlarged interlayer spacing of LDH,inhibits chlorine(electro)chemistry,and alleviates local pH drop of the electrode.It only needs an overpotential of 320 mV to reach a current density of 500 mA·cm^(−2)in 1 M KOH.In contrast to the fast activity decay of NiFe-LDH/CC counterpart during long-term electrolysis,BZ-NiFe-LDH/CC achieves stable 100-h electrolysis at an industrial-level current density of 500 mA·cm^(−2)in alkaline seawater.Operando Raman spectroscopy studies further identify structural changes of disorderedδ(NiIII-O)during the seawater oxidation process.Longcheng Zhang Jie Liang Luchao Yue Kai Dong Jun Li Donglin Zhao Zerong Li Shengjun Sun Yongsong Luo Qian Liu Guanwei Cui Abdulmohsen Ali Alshehri Xiaodong Guo Xuping Sun 2022Nano Research Energy2022,1,3:6
4CoFe-LDH nanowire arrays on graphite felt: A high-performance oxygen evolution electrocatalyst in alkaline media显示文摘Developing non-noble-metal oxygen evolution reaction(OER) electrocatalysts with high performance is critical to electrocatalytic water splitting. In this work, we fabricated Co Fe-layered double hydroxide(LDH) nanowire arrays on graphite felt(Co Fe-LDH/GF) via a hydrothermal method. The Co Fe-LDH/GF, as a robust integrated 3 D OER anode, exhibits excellent catalytic activity with the need of low overpotential of 252 and 285 mV to drive current densities of 10 and 100 mA/cm^(2) in 1.0 mol/L KOH, respectively. In addition, it also maintains electrochemical durability for at least 24 h. This work would open up avenues for the development of GF like attractive catalyst supports for oxygen evolution applications.Biao Deng Jie Liang Luchao Yue Tingshuai Li Qian Liu Yang Liu Shuyan Gao Abdulmohsen Ali Alshehri Khalid Ahmed Alzahrani Yonglan Luo Xuping Sun 2022Chinese Chemical Letters2022,33,2:4
5FeOOH quantum dots decorated graphene sheet:An efficient electrocatalyst for ambient N2 reduction显示文摘Electrochemical N2 reduction offers a promising alternative to the Haber-Bosch process for sustainable NH3 synthesis at ambient conditions,but it needs efficient catalysts for the N2 reduction reaction(NRR).Here,we report that FeOOH quantum dots decorated graphene sheet acts as a superior catalyst toward enhanced electrocatalytic N2 reduction to NH3 under ambient conditions.In 0.1 M LiClO4,this hybrid attains a large NH3 yield rate and a high Faradaic efficiency of 27.3µg·h^−1·mg−1cat.and 14.6%at−0.4 V vs.reversible hydrogen electrode,respectively,rivalling the current efficiency of all Fe-based NRR electrocatalysts in aqueous media.It also shows strong durability during the electrolytic process.Xiaojuan Zhu Jinxiu Zhao Lei Ji Tongwei Wu Ting Wang Shuyan Gao Abdulmohsen Ali Alshehri Khalid Ahmed Alzahrani Yonglan Luo Yimo Xiang Baozhan Zheng Xuping Sun 2020Nano Research2020,13,1:4
6Prognosis factors of advanced gastric cancer according to sex and age显示文摘BACKGROUND Gastric cancer has a relatively high prevalence and is one of the most common causes of cancer-related death worldwide.However,the prognosis for gastric cancer remains poor,especially in the advanced stages,despite many improvements in diagnosis and treatment.AIM To evaluate the outcomes regarding advanced gastric cancer development according to sex and age.METHODS We retrospectively reviewed 2005 patients who underwent curative gastrectomy for advanced gastric cancer between 2002 and 2007 at a single Korean centre.Prognosis and risk factors for nodal involvement were evaluated according to sex and age.RESULTS In this retrospective cohort study,we examined the cases of 2005 patients[sex,1384 men(69%),621 women(31%)]with advanced gastric cancer.The patients’age range was 22-87 years(mean age:57.7±12.3 years),with approximately 53.3%of the patients being≤60 years old.Based on a Cox proportional hazards model,overall survival was independently predicted by older age,larger tumour size,lymphovascular invasion,lymph node metastasis,deeper tumour invasion,moderately-to-poorly differentiated tubular adenocarcinoma,and signet ring cell carcinoma.The same model revealed that relapse-free survival was independently predicted by advanced age,larger tumour size,lymphovascular invasion,deeper tumour invasion,poorly differentiated tubular adenocarcinoma,and signet ring cell carcinoma.CONCLUSION Among patients with advanced gastric cancer,older age independently predicted poor overall survival and relapse-free survival.However,there were no significant sex-based differences in relapse-free and overall survival.Abdulaziz Alshehri Hussain Alanezi Beom Su Kim 2020World Journal of Clinical Cases2020,8,9:4
7Ambient ammonia production via electrocatalytic nitrite reduction catalyzed by a CoP nanoarray显示文摘Industrial-scale ammonia(NH_(3))production mainly relies on the energy-intensive and environmentally unfriendly Haber-Bosch process.Such issue can be avoided by electrocatalytic N_(2) reduction which however suffers from limited current efficiency and NH3 yield.Herein,we demonstrate ambient NH_(3) production via electrochemical nitrite(NO_(2)^(-))reduction catalyzed by a CoP nanoarray on titanium mesh(CoP NA/TM).When tested in 0.1 M PBS(pH=7)containing 500 ppm N0_(2)^(-),such CoP NA/TM is capable of affording a large NH_(3) yield of 2,260.7±51.5μg·h^(-1)·cm^(-2) and a high Faradaic efficiency of 90.0±2.3%at-0.2 V vs.a reversible hydrogen electrode.Density functional theory calculations reveal that the potential-determining step for NO_(2)^(-)reduction over CoP(112)is*NO2→*NO_(2)H.Guilai Wen Jie Liang Qian Liu Tingshuai Li Xuguang An Fang Zhang Abdulmohsen Ali Alshehri Khalid Ahmed Alzahrani Yonglan Luo Qingquan Kong Xuping Sun 2022Nano Research2022,15,2:3
8脂质组学改善传统危险因素预测的2型糖尿病患者的心血管事件显示文摘临床脂质测定并未显示出糖尿病或心血管病相关的脂质代谢改变的复杂性。脂质组学则能够评估可作为疾病风险潜在标志物的数百种脂质种类。方法:纳入来自糖尿病治疗和血管保护行动。刘莉 叶鹏 Alshehry ZH Mundra PA Barlow CK Mellett NA Wong G McConville MJ Simes J Tonkin AM Sullivan DR Barnes EH Nestel PJ Kingwell BA Marre M Neal B Poulter NR Rodgers A Williams B Zoungas S Hillis GS Chalmers J Woodward M Meikle PJ 2016中华高血压杂志2016,24,10:3
9N-doped carbon nanotubes supported CoSe_(2) nanoparticles:A highly efficient and stable catalyst for H_(2)O_(2) electrosynthesis in acidic media显示文摘Electrocatalytic oxygen reduction reaction(ORR)provides an attractive alternative to anthraquinone process for H_(2)O_(2) synthesis.Rational design of earth-abundant electrocatalysts for H_(2)O_(2) synthesis via a two-electron ORR process in acids is attractive but still:very challenging.In this work,we report that nitrogen-doped carbon nanotubes as a multi-functional support for CoSe2 nanoparticles not only keep CoSe_(2) nanoparticles well dispersed but alter the crystal structure,which in turn improves the overall catalYtic behaviors and thereby renders high O_(2)-to-H_(2)O_(2) conversion efficiency.In 0.1 M HClO_(4),such CoSe_(2)@NCNTs hybrid delivers a high H_(2)O_(2) selectivity of 93.2% and a large H_(2)0_(2) yield rate of 172 ppm·h^(-1) with excellent durability up to 24 h.Moreover,CoSe_(2)@NCNTs performs effectively for organic dye degradation via electro-Fenton process.Longcheng Zhang Jie Liang Luchao Yue Zhaoquan Xu Kai Dong Qian Liu Yonglan Luo Tingshuai Li Xiaohong Cheng Guanwei Cui Bo Tang Abdulmohsen Ali Alshehri Khalid Ahmed Alzahrani Xiaodong Guo Xuping Sun 2022Nano Research2022,15,1:2
10N, O-doped carbon foam as metal-free electrocatalyst for efficient hydrogen production from seawater显示文摘Seawater electrolysis is the most promising technology for large scale hydrogen production due to the abundance and low cost of seawater in nature.However,compared with the traditional freshwater electrolysis,the issues of electrode poisoning and corrosion will occur during the seawater electrolysis process,and active and stable electrocatalysts for the hydrogen evolution reaction(HER)are thus highly desired.In this work,N,O-doped carbon foam in-situ derived from commercial melamine foam is proposed as a high-active metal-free HER electrocatalyst for seawater splitting.In acidic seawater,our catalyst shows high hydrogen generation performance with small overpotential of 161 mV at 10 mA·cm^(−2),a low Tafel slop of 97.5 mV·dec^(−1),and outstanding stability.Qian Liu Shengjun Sun Longcheng Zhang Yongsong Luo Qin Yang Kai Dong Xiaodong Fang Dongdong Zheng Abdulmohsen Ali Alshehri Xuping Sun 2022Nano Research2022,15,10:2
11Plasmonic light trapping for enhanced light absorption in film-coupled ultrathin metamaterial thermophotovoltaic cells显示文摘Ultrathin 房间为减少的重量,减少的费用和增加的灵活性由于他们的潜力获得了增加的注意。然而,在 ultrathin 房间的轻吸收与相应体积房间相比通常是很弱的。为了完成,在 ultrathin thermophotovoltaic (TPV ) 提高了光子吸收房间,这个工作建议了用层由一个顶夹了的纳米厚的镓 antimonide (GaSb ) 做的联合电影的 metamaterial 结构一个维(1D ) 金属性的栅栏和底部金属拍摄。光谱建议结构的正常吸收比用严密夫妇波浪算法(RCWA ) 被计算,吸收改进被阐明被归因于磁性的电磁声子(MP ) 的刺激,表面电浆子电磁声子(SPP ) ,和 Fabry-Perot (FP ) 回声。MP, SPP,和 FP 的机制被一个引导者电容器电路模型,分散关系,和阶段移动进一步分别地证实。栅栏时期,宽度,分隔符厚度,以及发生角度的效果被讨论。而且,电线走火电流密度,开电路的电压,产量电力,和变换效率与联合电影的 metamaterial 结构为 ultrathin GaSb TPV 房间被评估。这个工作将便于下一代的便宜 ultrathin 的发展红外线的 TPV 房间。Qing NI Hassan ALSHEHRI Yue YANG Hong YE Liping WANG 2018Frontiers in Energy2018,12,1:2
12Derivations of MV-algebras显示文摘Alshehri N O 2010Internation Journal of Mathematics and Mathematical Sciences2010,,31:1
13Certain types of interval-valued fuzzy graphs显示文摘Akram M Alshehri N O Dudek W A 2013Journal of Applied Mathematics2013,7,:1
14Derivation of MV-algebras显示文摘Alshehri N O 2010Int J Math Math Sci2010,31,:1
15Enhanced N_(2)-to-NH_(3)conversion efficiency on Cu3P nanoribbon electrocatalyst显示文摘Ambient electroreduction of nitrogen(N_(2))is considered as a green and feasible approach for ammonia(NH_(3))synthesis,which urgently demands for efficient electrocatalyst.Morphology has close relationship with catalytic activity of heterogeneous catalysts.Nanoribbon is attractive nanostructure,which possesses the flexibility of one-dimensional nanomaterials,the large surface area of two-dimensional nanomaterials,and lateral size confinement effects.In this work,Cu_(3)P nanoribbon is proposed as a highly efficient electrocatalyst for N_(2)-to-NH_(3)conversion under benign conditions.When measured in N_(2)-saturated 0.1 M HCl,such Cu_(3)P nanoribbon achieves high performance with an excellent Faradaic efficiency as high as 37.8%and a large yield of 18.9μg·h^(−1)·mgcat.−1 at−0.2 V.It also demonstrates outstanding stability in long-term electrolysis test at least for 45 h.Qian Liu Yiting Lin Shuang Gu Ziqiang Cheng Lisi Xie Shengjun Sun Longcheng Zhang Yongsong Luo Abdulmohsen Ali Alshehri Mohamed SHamdy Qingquan Kong Jiahong Wang Xuping Sun 2022Nano Research2022,15,8:1
16Ki- netics of the thermal decomposition of '/-irradiated cobaltous acetate显示文摘Alshehri S M Monshi M A S Abd Elsalam N M 2005International Immunopharmacology2005,5,3:1
17Folded novel accurate analytical and semi-analytical solutions of a generalized Calogero–Bogoyavlenskii–Schiff equation显示文摘This paper studies the analytical and semi-analytic solutions of the generalized Calogero–Bogoyavlenskii–Schiff(CBS)equation.This model describes the(2+1)–dimensional interaction between Riemann-wave propagation along the y-axis and the x-axis wave.The extended simplest equation(ESE)method is applied to the model,and a variety of novel solitarywave solutions is given.These solitary-wave solutions prove the dynamic behavior of soliton waves in plasma.The accuracy of the obtained solution is verified using a variational iteration(VI)semi-analytical scheme.The analysis and the match between the constructed analytical solution and the semi-analytical solution are sketched using various diagrams to show the accuracy of the solution we obtained.The adopted scheme’s performance shows the effectiveness of the method and its ability to be applied to various nonlinear evolution equations.Mostafa M A Khater S K Elagan M A El-Shorbagy S H Alfalqi J F Alzaidi Nawal A Alshehri 2021Communications in Theoretical Physics2021,73,9:1
18Risk factors for development of hypoxic - ischemic encephalopathy in Abha City - southwestern Saudi Arabia显示文摘AlShehri MA Eid WA 2005Afr J Med Med Sci2005,34,3:1
19Fibrin activates GPVI in human and mouse platelets显示文摘Alshehri OM Hughes CE Montague S 2015Blood2015,126,:1
20Lactate and acid base changes during laparoscopic cholecystectomy显示文摘Ibraheim OA Samarkandi AH Alshehry H 2006Middle East J Anesthesiol2006,18,4:1
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