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| 1 | Jointly Building 'Belt and Road' for Mutual Benefits显示文摘Editor’s Note:From May 26-28,Mr.Ji Bingxuan,Vice-Chairman of the Standing Committee of the National People’s Congress and Vice-President of the Chinese Association for International Understanding(CAFIU),visited Albania,leading a CAFIU delegation.The following is the script of the speech that Vice-President Ji delivered at a symposium | Ji Binxuan Cui Li | 2016 | International Understanding2016，，2： | 0 |
| 2 | Optimization of process parameters for preparation of powdered activated coke to achieve maximum SO_(2)adsorption using response surface methodology显示文摘Powdered activated coke(PAC)is a good adsorbent of SO_(2),but its adsorption capacity is affected by many factors in the preparation process.To prepare the PAC with a high SO_(2)adsorption capacity using JJ-coal under flue gas atmosphere,six parameters(oxygen-coal equivalent ratio,reaction temperature,reaction time,O_(2)concentration,CO_(2)concentration,and H_(2)O concentration)were screened and optimized using the response surface methodology(RSM).The results of factor screening experiment show that reaction temperature,O_(2)concentration,and H_(2)O(g)concentration are the significant factors.Then,a quadratic polynomial regression model between the significant factors and SO_(2)adsorption capacity was established using the central composite design(CCD).The model optimization results indicate that when reaction temperature is 904.74℃,O_(2)concentration is 4.67%,H_(2)O concentration is 27.98%,the PAC(PAC-OP)prepared had a higher SO_(2)adsorption capacity of 68.15 mg/g while its SO_(2)adsorption capacity from a validation experiment is 68.82 mg/g,and the error with the optimal value is 0.98%.Compared to two typical commercial activated cokes(ACs),PAC-OP has relatively more developed pore structures,and its SBET and Vtot are 349 m^(2)/g and 0.1475 cm3/g,significantly higher than the 186 m^(2)/g and 0.1041 cm3/g of AC1,and the 132 m^(2)/g and 0.0768 cm3/g of AC2.Besides,it also has abundant oxygen-containing functional groups,its surface O content being 12.09%,higher than the 10.42%of AC1 and 10.49%of AC2.Inevitably,the SO_(2)adsorption capacity of PAC-OP is also significantly higher than that of both AC1 and AC2,which is 68.82 mg/g versus 32.53 mg/g and 24.79 mg/g,respectively. | Binxuan ZHOU Tao WANG Tianming XU Cheng LI Yuan ZHAO Jiapeng FU Zhen ZHANG Zhanlong SONG Chunyuan MA | 2021 | Frontiers in Energy2021，15，1： | 0 |
| 3 | Bacterial Cellulose-Based Janus Films with Radiative Cooling and Solar Heating Properties for All-Season Thermal Management显示文摘Advanced radiative cooling materials with both heating and cooling mode is of pivotal importance for all-season energy-saving in buildings.In this work,we report the design and fabrication of bacterial cellulose-based Janus films(J-BC)with radiative cooling and solar heating properties,which were developed by two-step vacuum-assisted filtration of modified MXene-doped bacterial cellulose and modified silicon nitride(Si_(3)N_(4))-doped bacterial cellulose,followed by hot-pressing and drying treatments.The as-prepared J-BC films show a unique Janus structure where modified MXene nanosheets and cellulose nanofibers are on the bottom surface,and modified silicon nitride(Si_(3)N_(4))nanoparticles and cellulose nanofibers are on the top surface.The radiative cooling effect of J-BC films is enabled by the Si_(3)N_(4)-doped bacterial cellulose due to the high mid-infrared emissivity of Si_(3)N_(4) nanoparticles,which shows a high solar reflection of~98.1%and high emissivity of~93.6%in the atmospheric transparency window(8-13μm).Thanks to the enhanced photothermal conversion of the modified MXene nanosheets,a reduced solar reflection(6.6%)and relatively low thermal emissivity in the atmospheric window(71.4%)are achieved,making sure the solar heating effect of J-BC films.In the outdoor tests,J-BC films achieve a sub-ambient temperature drop of~3.8°C and an above-ambient temperature rise of~14.2°C.Numerical prediction demonstrated that the J-BC films with dual modes have great potential of all-season energy saving for buildings and a corresponding energy-saving map in China is also created.The work disclosed herein can provide an avenue for the shaping of advanced radiative cooling materials for emerging applications of personal thermal management,sustainable energy-efficient buildings,and beyond. | Shukuan Shi Cristian Valenzuela Yanzhao Yang Yuan Liu Binxuan Li Ling Wang Wei Feng | 2023 | Chinese Journal of Chemistry2023，41，20： | 0 |
| 4 | Study of the reaction mechanism for preparing powdered activated coke with SO_(2)adsorption capability via one-step rapid activation method under flue gas atmosphere显示文摘In this study,the impact of different reaction times on the preparation of powdered activated carbon(PAC)using a one-step rapid activation method under flue gas atmosphere is investigated,and the underlying reaction mechanism is summarized.Results indicate that the reaction process of this method can be divided into three stages:stage I is the rapid release of volatiles and the rapid consumption of O_(2),primarily occurring within a reaction time range of 0-0.5 s;stage II is mainly the continuous release and diffusion of volatiles,which is the carbonization and activation coupling reaction stage,and the carbonization process is the main in this stage.This stage mainly occurs at the reaction time range of 0.5 -2.0 s when SL-coal is used as material,and that is 0.5-3.0 s when JJ-coal is used as material;stage III is mainly the activation stage,during which activated components diffuse to both the surface and interior of particles.This stage mainly involves the reaction stage of CO_(2)and H2O(g)activation,and it mainly occurs at the reaction time range of 2.0-4.0 s when SL-coal is used as material,and that is 3.0-4.0 s when JJ-coal is used as material.Besides,the main function of the first two stages is to provide more diffusion channels and contact surfaces/activation sites for the diffusion and activation of the activated components in the third stage.Mastering the reaction mechanism would serve as a crucial reference and foundation for designing the structure,size of the reactor,and optimal positioning of the activator nozzle in PAC preparation. | Binxuan Zhou Jingcai Chang Jun Li Jinglan Hong Tao Wang Liqiang Zhang Ping Zhou Chunyuan Ma | 2024 | Chinese Journal of Chemical Engineering2024，65，1： | 0 |
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