| 1 | Polymeric Carbon Nitride-based Single Atom Photocatalysts for CO_(2) Reduction to C1 Products显示文摘Photocatalytic CO_(2)reduction to C1 fuels is considered to be an important way for alleviating increasingly serious energy crisis and environmental pollution.Due to the environment-friendly,simple preparation,easy formation of highly-stable metal-nitrogen(M-Nx)coordination bonds,and suitable band structure,polymeric carbon nitride-based single-atom catalysts(C_(3)N_(4)-based SACs)are expected to become a potential for CO_(2)reduction under visible-light irradiation.In this review,we summarize the recent advancement on C_(3)N_(4)-based SACs for photocatalytic CO_(2)reduction to C1 products,including the reaction mechanism for photocatalytic CO_(2)reduction to C1 products,the structure and synthesis methods of C_(3)N_(4)-based SACs and their applications toward photocatalytic CO_(2)reduction reaction(CO_(2)RR)for C1 production.The current challenges and future opportunities of C_(3)N_(4)-based SACs for photoreduction of CO_(2)are also discussed. | MIAO Tianchang DI Xin HAO Feini ZHENG Gengfeng HAN Qing | 2022 | Chemical Research in Chinese Universities2022，38，5： | 0 |
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