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| 1 | Synthesis of Al_2O_3-SiC Composite and Its Effect on the Properties of Low-carbon MgO-C Refractories显示文摘Al2O3-SiC composite was synthesized with pyrophyllite and natural graphite as raw materials by carbothermal reduction reaction under argon atmosphere. The effect of synthesis temperature on phase composition and microstructure was investigated. Low-carbon MgO-C refractories were prepared by using the synthesized Al2O3-SiC composite as additive. The effect of its addition on the slag penetration and corrosion resistance as well as oxidation resistance of the refractories was investigated, and the slag resistance and oxidation resistance mechanisms of the Al2O3-SiC composite were also discussed. The results show that the synthesis temperature has a great influence on preparation of Al2O3-SiC composite. The Al2O3-SiC composite can be synthesized at 1873-1973 K under argon atmosphere, with pyrophyllite and natural graphite as raw materials, and particle sizes of the composite synthesized at 1973 K are mainly distributed as 1-2 μm. The slag penetration and corrosion resistance of low-carbon MgO-C refractories can be remarkably improved by adding the synthesized Al2O3-SiC composite, and the oxidation resistance has an improvement to some extent. The increase of slag viscosity and the formation of MgAl2O4 can effectively inhibit the slag penetration and corrosion for the refractories. | Beiyue Ma Qiang Zhu Yong Sun Jingkun Yu Ying Li | 2010 | Journal of Materials Science & Technology2010，26，8： | 9 |
| 2 | Hygroscopicity of particles generated from photooxidation of α-pinene under diferent oxidation conditions in the presence of sulfate seed aerosols显示文摘Smog chamber experiments were conducted to investigate the hygroscopicity of particles generated from photooxidation of α-pinene/NOx with diferent sulfate seed aerosols or oxidation conditions. Hygroscopicity of particles was measured by a tandem diferential mobility analyzer(TDMA) in terms of hygroscopic growth factor(Gf), with a relative humidity of 85%. With sulfate seed aerosols present, Gf of the aerosols decreased very fast before notable secondary organic aerosols(SOA) formation was observed, indicating a heterogeneous process between inorganic seeds and organic products might take place as soon as oxidation begins, rather than only happening after gas-aerosol partition of organic products starts. The final SOA-coated sulfate particles had similar or lower Gf than seed-free SOA. The hygroscopicity of the final particles was not dependent on the thickness but on the hygroscopicity properties of the SOA, which were influenced by the initial sulfate seed particles. In the two designed aging processes, Gf of the particles increased more significantly with introduction of OH radical than with ozone. However, the hygroscopicity of SOA was very low even after a long time of aging, implying that either SOA aging in the chamber was very slow or the Gf of SOA did not change significantly in aging. Using an aerosol composition speciation monitor(ACSM) and matrix factorization(PMF) method, two factors for the components of SOA were identified, but the correlation between SOA hygroscopicity and the proportion of the more highly oxidized factor could be either positive or negative depending on the speciation of seed aerosols present. | Biwu Chu Kun Wang Hideto Takekawa Junhua Li Wei Zhou Jingkun Jiang Qinxing Ma Hong He Jiming Hao | 2014 | Journal of Environmental Sciences2014，26，1： | 6 |
| 3 | Maternal exposure to triclosan constitutes a yet unrecognized risk factor for autism spectrum disorders显示文摘Dear Editor,Autism spectrum disorders(ASD)are complex neurodevelopmental disorders characteristic of core behavioral traits like restricted,repetitive behaviors and deficiency in social interactions.1 The prevalence of ASD has rapidly increased worldwide,rising from 1/149 in 2000,1/68 in 2012,and to?1/40 in 2016 of children at the age of 3-17 in the United States.2 ASD prevalence was found to be associated with socioeconomic status(SES)as overpresented in high-income households,3 and to be significantly enriched in certain regions,e.g.,reaching up to 4.88%in Florida.2 In the last decades,advances in genetic studies have led to unprecedented understanding of the genetic factors that were associated with<50%of human ASD. | Zijian Hao Qionghui Wu Zhengwei Li Yali Li Qiu Li Xi Lai Huan Liu Menghuan Zhang Ting Yang Jie Chen Yaping Tang Jingkun Miao Huatai Xu Tingyu Li Ronggui Hu | 2019 | Cell Research2019，29，10： | 5 |
| 4 | Continuous and comprehensive atmospheric observations in Beijing:a station to understand the complex urban atmospheric environment显示文摘Due to profound impact on climate and human health,air quality has attracted attention from all levels of the civil society.The key step in the provision of required tools for the society to tackle the complex air quality problem is to characterize it in a comprehensive manner with a long-term perspective.Here,we describe a continuous and comprehensive observation station and its accompanying state-ofthe-art instrumentation that was established to investigate the complex urban atmospheric environment in a rapidly developing Chinese Megacity.The station,located in downtown Beijing,aims to study air quality by identifying the major atmospheric pollutants and key processes determining their formation and loss mechanisms.A few hundreds of parameters are continuously measured with the state-of-the-art instruments,including trace gas concentrations,aerosol particle size distributions,and mass concentrations,covering aerosol particle chemical composition from molecules to micrometer-sized aerosol particles.This produced long-term,comprehensive big data with around 1�10^(11)bytes per year.In this paper,we provide an overview on the facilities of the station,the instrumentation used,the workflow of continuous observations and examples of results from 2018 to 2019 and a basis for establishing a modern long-term,comprehensive atmospheric urban observation station in other megacities. | Yongchun Liu Chao Yan Zemin Feng Feixue Zheng Xiaolong Fan Yusheng Zhang Chang Li Ying Zhou Zhuohui Lin Yishou Guo Ying Zhang Li Ma Wenshuo Zhou Zhikun Liu Lubna Dada Kaspar Dallenbach Jenni Kontkanen Runlong Cai Tommy Chan Biwu Chu Wei Du Lei Yao Yonghong Wang Jing Cai Juha Kangasluoma Tom Kokkonen Joni Kujansuu Anton Rusanen Chenjuan Deng Yueyun Fu Rujing Yin Xiaoxiao Li Yiqun Lu Yiliang Liu Chaofan Lian Dongsen Yang Weigang Wang Maofa Ge Yuesi Wang Douglas R.Worsnop Heikki Junninen Hong He Veli-Matti Kerminen Jun Zheng Lin Wang Jingkun Jiang Tuukka Petaja Federico Bianchi Markku Kulmala | 2020 | Big Earth Data2020，4，3： | 3 |
| 5 | Preparation of SiC Porous Ceramics by Crystalline Silicon Cutting Waste显示文摘SiC porous ceramics were prepared at 1 400 ℃ for4 h with crystalline silicon cutting waste and activated carbon as main starting materials and NH_4HCO_3 as the pore-forming agent. Effects of NH_4HCO_3 additions( 0,20%,30%,40%,by mass) on the phase composition,microstructure,sintering properties,cold compressive strength and thermal shock resistance of as-prepared Si C porous ceramics were investigated. The results show that:( 1) addition of NH_4HCO_3 remarkably influences the apparent porosity and cold compressive strength of specimens. The apparent porosity achieves its maximum value( 63. 40%) when 40% NH_4HCO_3 is added,while the minimum cold compressive strength is 4. 77 MPa;( 2) the specimen with 40% NH_4HCO_3 has the best thermal shock resistance. The thermal cycling times between1 000 ℃ to room temperature reach 62;( 3) the addition of NH_4HCO_3 does not remarkably affect the phase composition of the specimens;( 4) the specimens include a large number of SiC particles and a small amount of SiC whiskers. | ZHANG Yaran MA Beiyue YU Jingyu SU Chang REN Xinming QIAN Fan LIU Guoqi LI Hongxia YU Jingkun | 2018 | China's Refractories2018，27，4： | 3 |
| 6 | Epidermal self-powered sweat sensors for glucose and lactate monitoring显示文摘Sweat could be a carrier of informative biomarkers for health status identification;therefore,wearable sweat sensors have attracted significant attention for research.An external power source is an important component of wearable sensors,however,the current power supplies,i.e.,batteries,limit further shrinking down the size of these devices and thus limit their application areas and scenarios.Herein,we report a stretchable self-powered biosensor with epidermal electronic format that enables the in situ detec-tion of lactate and glucose concentration in sweat.Enzymatic biofuel cells serve as self-powered sensing modules allowing the sweat sensor to exhibit a determination coefficient(R2)of 0.98 with a sensitivity of 2.48 mV/mM for lactate detection,and R2 of 0.96 with a sensitivity of 0.11 mV/μM for glucose detection.The microfluidic channels developed in an ultra-thin soft flexible polydimethylsiloxane layer not only enable the effective collection of sweat,but also provide excellent mechanical properties with stable performance output even under 30%stretching.The presented soft sweat sensors can be integrated at nearly any location of the body for the continuous monitoring of lactate and glucose changes during normal daily activities such as exercise.Our results provide a promising approach to develop next-generation sweat sensors for real-time and in situ sweat analysis. | Xingcan Huang Jiyu Li Yiming Liu Tszhung Wong Jingyou Su Kuanming Yao Jingkun Zhou Ya Huang Hu Li Dengfeng Li Mengge Wu Enming Song Shijiao Han Xinge Yu | 2022 | Bio-Design and Manufacturing2022，5，1： | 3 |
| 7 | Study on the phase-separated opaque glaze in ancient China from Qionglai kiln显示文摘 | Weidong Li Jiazhi Li Jun Wu Jingkun Guo | 2003 | Ceramics International2003，，8： | 2 |
| 8 | Curcumin inhibits the invasion of lung cancer cells by modulating thePKCα/Nox-2/ROS/ATF-2/MMP-9 signaling pathway显示文摘 | Zhigang Fan Xiaoyi Duan Hui Cai Li Wang Min Li Jingkun Qu Wanjun Li Yongheng Wang Jiansheng Wang | 2015 | Oncology Reports2015，，2： | 2 |
| 9 | Fabrication, microstructure and properties of highly transparent Nd:YAG laser ceramics显示文摘 | Jiang Li Yusong Wu Yubai Pan Wenbin Liu Liping Huang Jingkun Guo | 2008 | Optical Materials2008，，1： | 2 |
| 10 | Single-cell Transcriptomic Analysis Reveals the Cellular Heterogeneity of Mesenchymal Stem Cells显示文摘Ex vivo-expanded mesenchymal stem cells(MSCs)have been demonstrated to be a heterogeneous mixture of cells exhibiting varying proliferative,multipotential,and immunomodulatory capacities.However,the exact characteristics of MSCs remain largely unknown.By singlecell RNA sequencing of 61,296 MSCs derived from bone marrow and Wharton’s jelly,we revealed five distinct subpopulations.The developmental trajectory of these five MSC subpopulations was mapped,revealing a differentiation path from stem-like active proliferative cells(APCs)to multipotent progenitor cells,followed by branching into two paths:1)unipotent preadipocytes or 2)bipotent prechondro-osteoblasts that were subsequently differentiated into unipotent prechondrocytes.The stem-like APCs,expressing the perivascular mesodermal progenitor markers CSPG4/MCAM/NES,uniquely exhibited strong proliferation and stemness signatures.Remarkably,the prechondrocyte subpopulation specifically expressed immunomodulatory genes and was able to suppress activated CD3^(+T) cell proliferation in vitro,supporting the role of this population in immunoregulation.In summary,our analysis mapped the heterogeneous subpopulations of MSCs and identified two subpopulations with potential functions in self-renewal and immunoregulation.Our findings advance the definition of MSCs by identifying the specific functions of their heterogeneous cellular composition,allowing for more specific and effective MSC application through the purification of their functional subpopulations. | Chen Zhang Xueshuai Han Jingkun Liu Lei Chen Ying Lei Kunying Chen Jia Si Tian-yi Wang Hui Zhou Xiaoyun Zhao Xiaohui Zhang Yihua An Yueying Li Qian-Fei Wang | 2022 | Genomics, Proteomics & Bioinformatics2022，20，1： | 2 |
| 11 | Preparation of ZrN(ZrON)-SiAION Composite Ceramics via a Pressureless Sintering Process显示文摘ZrN- SiA lO N composite materials were synthesized at 1 550 ℃ for 6 h via a carbothermal reduction nitridation route using fly ash( ≤74 μm),zircon( ≤44 μm)and active carbon as starting materials. The processed ZrN- SiA lO N composite micropowders were mixed with polyvinyl alcohol as binder to prepare ZrN( ZrO N)-SiA lO N composite ceramics by carbon-embedded pressureless firing at 1 450,1 500 and 1 550 ℃ for 1 h,respectively. Influences of firing temperature on the phase compositions,microstructure and sintering properties of the ceramics were investigated. The results show that:( 1)β-SiA lO N based composite ceramics with different compositions can be prepared by controlling firing temperature,and the main crystalline phases of the specimen fired at1 550 ℃ for 1 h involve ZrN,ZrO N and β-SiA lO N( z =2,Si4Al2O2N6);( 2) ZrN( ZrO N),β-SiA lO N and a Fe- Si based compound can be observed in the microstructures of the specimens fired at different temperatures.ZrN( ZrO N) particles distribute homogeneously in theβ-SiA lO N matrix;( 3) raising firing temperature can increase the shrinkage ratio of the ceramics,and the volume shrinkage ratio increases from 19. 4% to 40. 3% when the firing temperature rises from 1 450 to 1 550 ℃. | MA Beiyue LI Ying LU Zhongxin YU Jingkun | 2014 | China's Refractories2014，23，4： | 2 |
| 12 | Effects of two transition metal sulfate salts on secondary organic aerosol formation in toluene/NOx photooxidation显示文摘Aerosol phase reactions play a very important role on secondary organic aerosol (SOA) formation, and metal-containing aerosols are important components in the atmosphere. In this study, we tested the effects of two transition metal sulfate salts, manganese sulfate (MnSO4) and zinc sulfate (ZnSO4), on the photochemical reactions of a toluene/NOx photooxidation system in a 2 m3 smog chamber. By comparing photochemical reaction products of experiments with and without transition metal sulfate seed aerosols, we evaluated the effects of transition metal sulfate seed aerosols on toluene consumption, NOx conversion and the formation of ozone and SOA. MnSO4 and ZnSO4 seed aerosols were found to have similar effects on photochemical reactions, both enhance the SOA production, while showing negligible effects on the gas phase compounds. These observations are consistent when varying metal sulfate aerosol concentrations. This is attributed to the catalytic effects of MnSO4 and ZnSO4 seed aerosols which may enhance the formation of condensable semivolatile compounds. Their subsequent partitioning into the aerosol phase leads to the observed SOA formation enhancement. | Biwu CHU Jiming HAO Junhua LI Hideto TAKEKAWA Kun WANG Jingkun JIANG | 2013 | Frontiers of Environmental Science & Engineering2013，7，1： | 2 |
| 13 | Phase Formation and Process Analysis of SiC-Al_2O_3-Al_6Si_2O_(13) Composite Powder via Carbothermal Reduction of Fly Ash at 1 550 ℃显示文摘Silicon carbide(SiC)-alumina(Al_2O_3)-mullite(Al_6Si_2O_(13)) composite powder was successfully synthesized at 1 550 ℃ for 5 h via carbothermal reduction reaction,and the effects of various mass ratios of active carbon to fly ash(0.38,0.44 and 0.58) on the phase composition and microstructure of products were investigated,and the formation process of the powder was also analyzed in detail.The products mainly consist ofβ-SiC,α-Al_2O_3,Al_6Si_2O_(13) and FeSi.Increasing carbon content favors the decomposition of Al_6Si_2O_(13) and formation of SiC.The average particle size of β-SiC andα-Al_2O_3 is about 1 μm and that of Al_6Si_2O_(13) is 5-10μm.The formation process of SiC-Al_2O_3-Al_6Si_2O_(13)powder includes the decomposition of mullite in fly ash and formation of SiC. | ZHANG Bowen MA Beiyue YIN Yue LI Shiming ZHANG Zhan LI Guangqiang YU Jingkun | 2016 | China's Refractories2016，25，4： | 1 |
| 14 | Mechanical properties and electrical conductivity of TiN-Al2O3 nanocomposites显示文摘 | Li Jingguo Gao Lian Guo Jingkun | 2003 | Journal of the European Ceramic Society2003，，23： | 1 |
| 15 | Garment embedded sweat-activated batteries in wearable electronics for continuous sweat monitoring显示文摘Thin,soft,and skin-integrated electronic system has great advantages for realizing continuous human healthcare monitoring.Here,we report an ultra-thin,flexible,and garment-based microelectronics powered by sweat-activated batteries(SABs)and applications of powering biosensors and microelectronic systems for real time sweat monitoring.The SAB cell is ultra-thin(1.25 mm)with excellent biocompatibility.The SAB has good electricity output with high capacity(14.33 mAh)and maximum power density(3.17 mW cm^(−2))after being activated by the sweat volume of 0.045 mL cm^(−2),which could continuously power 120 light emitting diodes over 3 h.The outputs could maintain stable after repeatable bending.Wireless microelectronics system could be continuously powered by the SABs for 3 h to monitor sweat and physiological information,including sweat Na+concentration,pH,and skin impedance.The reported integrated system provides a potential for solving the power issues of flexible wearable electronics and realizing personalized medicine. | Xingcan Huang Yiming Liu Jingkun Zhou Sina Khazaee Nejad Tsz Hung Wong Ya Huang Hu Li Chun Ki Yiu Wooyoung Park Jian Li Jingyou Su Ling Zhao Kuanming Yao Mengge Wu Zhan Gao Dengfeng Li Jiyu Li Rui Shi Xinge Yu | 2022 | npj Flexible Electronics2022，6，1： | 1 |
| 16 | Fabrication of transparent Yb, Cr: YAG ceramics by a solid - state reaction method显示文摘 | Yusong Wu Jiang Li Fagui Qiu Yubai Pan Qian Liu Jingkun Guo | 2006 | Ceramics International2006，32，7： | 1 |
| 17 | Covalent organic nanospheres as a fiber coating for solid-phase microextraction of genotoxic impurities followed by analysis using GC-MS显示文摘Covalent organic nanospheres(CONs)were explored as a fiber coating for solid-phase microextraction of genotoxic impurities(GTIs)from active ingredients(AIs).CONs were synthesized by an easy solutionphase procedure at 25℃.The obtained nanospheres exhibited a high specific surface area,good thermostability,high acid and alkali resistance,and favorable crystallinity and porosity.Two types of GTIs,alkyl halides(1-iodooctane,1-chlorobenzene,1-bromododecane,1,2-dichlorobenzene,1-bromooctane,1-chlorohexane,and 1,8-dibromooctane)and sulfonate esters(methyl p-toluenesulfonate and ethyl ptoluenesulfonate),were chosen as target molecules for assessing the performance of the coating.The prepared coating achieved high enhancement factors(5097-9799)for the selected GTIs.The strong affinity between CONs and GTIs was tentatively attributed to π-π and hydrophobicity interactions,large surface area of the CONs,and size-matching of the materials.Combined with gas chromatography-mass spectrometry(GC-MS),the established analytical method detected the GTIs in capecitabine and imatinib mesylate samples over a wide linear range(0.2-200 ng/g)with a low detection limit(0.04-2.0 ng/g),satisfactory recovery(80.03%-109.5%),and high repeatability(6.20%-14.8%)and reproducibility(6.20%-14.1%).Therefore,the CON-coated fibers are promising alternatives for the sensitive detection of GTIs in AI samples. | Yanfang Zhao Jingkun Li Hanyi Xie Huijuan Li Xiangfeng Chen | 2022 | Journal of Pharmaceutical Analysis2022，12，4： | 1 |
| 18 | Mechanical properties and electrical conductivity of TiN-Al2O3 nanocomposites 显示文摘 | Lian Gao Jingkun Guo | 2003 | Journal of the European Ceramics Society2003，23，： | 1 |
| 19 | Acidic degradation and enhanced antioxidant activities of exopolysaccharides from Cordyceps sinensis mycelial culture显示文摘 | YAN Jingkun LI Lin WANG Zhaomei | 2009 | Food Chem2009，117，4： | 1 |
| 20 | Fabrication and mechanical properties of A12 03-Ni composite from two dif- ferent powder mixtures显示文摘 | Li Guojun Huang Xiaoxian Guo Jingkun | 2003 | Mater Sci Eng2003，352，： | 1 |
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