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| 1 | Is graphite lithiophobic or lithiophilic?显示文摘Graphite and lithium metal are two classic anode materials and their composite has shown promising performance for rechargeable batteries.However,it is generally accepted that Li metal wets graphite poorly,causing its spreading and infiltration difficult.Here we show that graphite can either appear superlithiophilic or lithiophobic,depending on the local redox potential.By comparing the wetting performance of highly ordered pyrolytic graphite,porous carbon paper(PCP),lithiated PCP and graphite powder,we demonstrate that the surface contaminants that pin the contact-line motion and cause contact-angle hysteresis have their own electrochemical-stability windows.The surface contaminants can be either removed or reinforced in a time-dependent manner,depending on whether the reducing agents(C6→Li C6)or the oxidizing agents(air,moisture)dominate in the ambient environment,leading to bifurcating dynamics of either superfast or superslow wetting.Our findings enable new fabrication technology for Li–graphite composite with a controllable Li-metal/graphite ratio and present great promise for the mass production of Li-based anodes for use in high-energy-density batteries. | Jian Duan Yuheng Zheng Wei Luo Wangyan Wu Tengrui Wang Yong Xie Sa Li Ju Li Yunhui Huang | 2020 | National Science Review2020，7，7： | 8 |
| 2 | Carbon Monoxide Alleviates Wheat Seed Germination Inhibition and Counteracts Lipid Peroxidation Mediated by Salinity显示文摘最近在动物,内长的碳一氧化物(公司) 象氮的氧化物一样,作为另一个重要生理的送信人或 bioactive 分子被含有。然而,很少信息都不在整个植物对公司的生理的角色被知道。在现在的学习,我们报导 CO 施主血色素(0.1, 1.0 和 10.0 mol/L ) 的不同集中减轻了小麦(Triticum aestivum L。Yangmai 158 ) 种子萌芽抑制以一种剂量依赖者方式由 250 mmol/L NaCl 应力引起了。这些回答被不同气体的公司水的答案的增加也从 0.1% ~ 100.0% 浸透证明。在这些处理之中, 1.0 mol/L 血色素和公司水的答案的 1.0% 浸透的效果是最明显的。与非血色素处理相比,而且,在小麦种子的存储储备的降级也被加速。时间功课分析证明血色素的申请 dose-dependently 增加了 superoxide dismutase,过氧化氢酶, ascorbate peroxidase,和 guaiacol peroxidase 活动的活动,因此减少在发芽小麦种子的类脂化合物 peroxidation 使遭到了腌应力。同时,因为 CO scavenger 血红素(0.2 g/L ) 的增加堵住了 1.0 mol/L 血色素的各种各样的行动,血色素的回答为公司是特定的。一起拿,现在的学习的结果证明在低集中,公司能稀释咸度应力生产的种子萌芽抑制并且在发芽小麦种子抵抗类脂化合物 peroxidation。 | Sheng Xu Zhi-Sheng Sa Ze-Yu Cao Wei Xuan Ben-Kai Huang Teng-Fang Ling Qiong-Ying Hu Wen-Biao Shen | 2006 | Journal of Integrative Plant Biology2006，48，10： | 7 |
| 3 | The effect of Fe-Mn minerals and seawater interface and enrich-ment mechanism of ore-forming elements of polymetallic crusts and nodules from the South China Sea显示文摘Ferromanganese crusts and nodules are important submarine mineral resources that contain various metal elements with significant economic value. In this study, polymetallic crusts and nodules obtained from the South China Sea(SCS) were determined by using X-ray power diffraction(XRD), Raman spectroscopy(RS), Fourier transform infrared spectroscopy(FTIR), and X-ray photoelectron spectroscopy(XPS) to systematically investigate and analyze the mineralogical and spectral characteristics of the Fe-Mn minerals. XRD measurements revealed that the SCS polymetallic crusts and nodules were composed of vernadite, quartz, and plagioclase. The nodules also contained todorokite. The Fe-phase minerals of the SCS crusts and nodules were composed of amorphous Fe oxide/hydroxide, and the Mn-and Fe-phases minerals exhibited relatively poor degrees of crystallization. FTIR results showed that the Fe-Mn minerals in the crusts and nodules included a large number of surface hydroxyl groups. These surface hydroxyl groups contained protons that could provide reactive sites for complexation of ore-forming elements in seawater. XPS results indicated that the surfaces of the Fe-Mn minerals mainly contained Fe, Mn, and O. Fe was present in the trivalent oxidation state, while Mn, which may contain several bivalent oxidation state, was present in the tetravalent and trivalent oxidation states. The SCS polymetallic crusts and nodules were compared with Pacific seamount crusts, and results showed that the surface hydroxyl(-OH) groups of the SCS crusts and nodules numbered more than the lattice oxygen(O^(2-)). But the lattice oxygen of Pacific seamount crusts numbered more than the surface hydroxyl groups. This characteristic indicated that the degree of crystallization of Fe-Mn minerals from the Pacific Ocean was higher than that of minerals from the South China Sea. Comprehensive studies showed that ore-forming elements in the interface between seawater and the Fe-Mn minerals in the submarine ferromanganese crusts and nodules employed the following enrichment mechanisms:(1) the metal ion complexed with the surface hydroxyl of Fe-Mn minerals to form hydroxyl complexes, which were connected by coordination bonds or stable inner-sphere complexes that exchanged protons on the mineral surfaces;(2) the charged surfaces of the minerals and metal cations formed outer-sphere complexes, which made up the electrostatic double layer, through electrostatic adsorption; and(3) the metal cations isomorphously exchanged the Mn and Fe ions of the mineral lattice structure. | GUAN Yao SUN Xiaoming IANG Xiaodong SA Rina ZHOU Li HUANG Yi LIU Yating LI Xiaojie LU Rongfei WANG Chi | 2017 | Acta Oceanologica Sinica2017，36，6： | 4 |
| 4 | Carbon Monoxide: A Novel Antioxidant Against Oxidative Stress in Wheat Seedling Leaves显示文摘一氧化碳(公司) ,在动物的一个内长的发信号分子,也每氧化剂在老鼠导致的氧化包括肺类脂化合物的变细提供有势力 cytoprotective 效果。我们的最近的工作证明小麦的处理种的 0.01 亩 mol/L 血色素(一个公司施主) 在幼苗叶子减轻了导致盐的氧化损坏。在这份报告,我们进一步发现那个血色素预告的处理(<=0.1 亩 mol/L ) 能推迟小麦叶叶绿素损失由 H_2O_2 和对草快的进一步的处理调停了,二反应的氧种(ROS ) 来源, indose- 甚至时间依赖者礼貌。另外与控制样品相比,为 24 h 的 0.01 或 0.1 亩 mol/L 血色素展出了的幼苗 leavespretreatedwith H_2O_2 和 lipidperoxidation 的底层,以及叶绿素的更高的内容和抗氧化剂酶的活动。血色素施加的 Suchbeneficial 效果被抗氧化剂 butylatedhydroxytoluene (BHT ) 的预告的处理模仿,并且当 COscavenger 血红素(Hb ) ,或公司特定的合成禁止者 ZnPPIX 分别地被增加时,差别逆行。总起来说,直接在这篇论文介绍的结果第一次说明那个公司能强烈保护 ROS 的生产过剩引起的 plantsfromoxidative 损坏,并且加强公司是在各种各样的不能生活、关於生命的压力的一种有势力抗氧化剂的证据,同样类似的结果在动物组织被显示出。 | Zhi-Sheng Sa Li-Qin Huang Guo-Lin Wu Jin-Peng Ding Xiao-Yue Chen Tian Yu Ci Shi Wen-Biao Shen | 2007 | Journal of Integrative Plant Biology2007，49，5： | 4 |
| 5 | Dual-Functional Lithiophilic/Sulfiphilic Binary-Metal Selenide Quantum Dots Toward High-Performance Li-S Full Batteries显示文摘The commercial viability of lithium-sulfur batteries is still challenged by the notorious lithium polysulfides(Li PSs)shuttle effect on the sulfur cathode and uncontrollable Li dendrites growth on the Li anode.Herein,a bi-service host with Co-Fe binary-metal selenide quantum dots embedded in three-dimensional inverse opal structured nitrogen-doped carbon skeleton(3DIO FCSe-QDs@NC)is elaborately designed for both sulfur cathode and Li metal anode.The highly dispersed FCSe-QDs with superb adsorptive-catalytic properties can effectively immobilize the soluble Li PSs and improve diffusion-conversion kinetics to mitigate the polysulfide-shutting behaviors.Simultaneously,the 3D-ordered porous networks integrated with abundant lithophilic sites can accomplish uniform Li deposition and homogeneous Li-ion flux for suppressing the growth of dendrites.Taking advantage of these merits,the assembled Li-S full batteries with 3DIO FCSe-QDs@NC host exhibit excellent rate performance and stable cycling ability(a low decay rate of 0.014%over 2,000 cycles at 2C).Remarkably,a promising areal capacity of 8.41 mAh cm^(-2)can be achieved at the sulfur loading up to 8.50 mg cm^(-2)with an ultra-low electrolyte/sulfur ratio of 4.1μL mg^(-1).This work paves the bi-serve host design from systematic experimental and theoretical analysis,which provides a viable avenue to solve the challenges of both sulfur and Li electrodes for practical Li-S full batteries. | Youzhang Huang Liang Lin Yinggan Zhang Lie Liu Baisheng Sa Jie Lin Laisen Wang Dong-Liang Peng Qingshui Xie | 2023 | Nano-Micro Letters2023，15，5： | 2 |
| 6 | Effects of residual water on microtensile bond strength of one-bottle dentin adhesive systems with different solvent bases显示文摘Background The wet-bonding technique is recommended for the one-bottle dentin adhesive systems, but themoisture concept varies widely among the instructions of manufacturers as well as among investigators·The aimofthis study was to evaluate the effects of different dentin surface moisture on the microtensile bond strength(s) ofan ethanol/water-based adhesive system and an acetone-based system to dentin·Methods Forty intact human premolars extracted for orthodontic reasons were used·Superficial occlusal flatdentin surfaces of these premolars were exposed, finished with wet600-grit silicon carbide paper·Under four wetand dry conditions (overwet, blot dry, one-second dry and desiccated), resin composite was bonded to dentinby using Single Bond (SB) or Prime &Bond NT(PB) according to the manufacturers’instructions·The teethwere longitudinally sectioned in the“x”and“y”directions to obtain bonded beams with a cross-sectional area of0·81 mm2with a slow-speed diamond saw·The bonded specimens were tested in tension at a crosshead speed of1 mm/min until failure of the bonds·Failure modes were observed with a scanning electron microscope·Themean bond strengths were analyzed by one-way ANOVA and Turkey’s test·Results The bond strength of the overwet/SB, blotdry/SB, one-second dry/SB and desiccated/SB groups was10·87 MPa, 22·47 MPa, 24·91 MPa and 12·99 MPa, respectively·The bond strength of the overwet/PB, blotdry/PB, one-second dry/PB and desiccated/PB groups was 10·02 MPa, 20·67 MPa, 21·82 MPa and 10·09MPa, respectively·For both SB and PB, the blot dry group and one-second dry group revealed significantlyhigher bond strengths than the overwet and desiccated groups (P<0·05)·Conclusions In order to achieve the highest bond strength to dentin, keeping the dentin surface in anappropriately moist condition is critical for the one-bottle dentin adhesive systems with ethanol/water or acetonesolvent· | ZHANG Zhi-xing HUANG Cui ZHENG Tie-li WANG Sa CHENG Xiang-rong | 2005 | Chinese Medical Journal2005，，19： | 2 |
| 7 | Identification of a new member of the tumor necrosis factor family and its receptor,a human ortholog of mouse GITR显示文摘 | Gurney AL Marsters SA Huang RM | 1999 | Current Biology1999，9，4： | 1 |
| 8 | Comparison of cone beam computed tomography imaging with physical measures 显示文摘 | Stratemann SA Huang JC Maki K | 2008 | Dentomaxillofac Radiol2008，37，： | 1 |
| 9 | Antigenic and genetic divergence of rabies viru- ses from bat species indigenous to Canada显示文摘 | NADIN-DAVIS SA HUANG W ARMSTRONG J | 2001 | Virus Res2001，74，12： | 1 |
| 10 | Silencing Toll- like receptor-9 in pseudomonas aeruginosa keratitis 显示文摘 | Huang X Barrett RP McClellan SA Hazlett LD | 2005 | Invest Ophthalmol Vis Sci2005，46，42： | 1 |
| 11 | Long-term stable canine mandibular augmentation using autologous bone marrow stromal cells and hydroxyapatite/tricalcium phosphate显示文摘 | Kuznetsov SA Huang KE Marshall GW | 2008 | Biomaterials2008，29，31： | 1 |
| 12 | Type 2 iodothyronine deiodinase is the major source of plasma T3 in euthyroid humans显示文摘 | Maia AL Kim BW Huang SA | 2005 | J Clin Invest2005，115，9： | 1 |
| 13 | Differential expressions of cyclin-dependent kinase inhibitors ( p27 and p21 ) and their relation to p53 and Ki-67 in oral squamous tumorigenesis显示文摘 | Choi HR Tucker SA Huang Z | 2003 | Int J Oncol2003，22，2： | 1 |
| 14 | Reawakened interest in type Ⅲ iodothyronine deiodinase in critical illness and injury 显示文摘 | Huang SA Bianco AC | 2008 | Nat Clin Pract Endocrinol Metab2008，4，3： | 1 |
| 15 | Bioelectrochemical systems for efficient recalcitrant wastes treatment显示文摘 | Huang LP Cheng SA Chen GH | | 0，，04： | 1 |
| 16 | Molecular regulation of interleukin-13 and monocyte chemoattractant protein-1 expression in human mast cells by interleukin-ll3显示文摘 | Lee SA Fitzgerald SM Huang SK | 2004 | Respir Cell Mol Biol2004，31，3： | 1 |
| 17 | Comparison of cone beam computed tomography imaging with physical measures 显示文摘 | Stratemann SA Huang JC Maki K | 2008 | Dentomaxillofac Radiol2008，37，2： | 1 |
| 18 | Reawakened interest in type III iodothyro2nine deiodinase in critical illness and injury 显示文摘 | Huang SA Bianco AC | 2008 | Nat Clin PractEndocrinolMetab2008，4，3： | 1 |
| 19 | Comprehensive flow cytometry phenotype in acute leukemia at diagnosis and at relapse显示文摘 | Li X Du W Liu W Li X Li H Huang SA | 2010 | APMIS2010，118，5： | 1 |
| 20 | Paracrine-stimulated gene expression profile favors estradiol production in breast tumors显示文摘 | Amin SA Huang CC Reierstad S | 2006 | Mol Cell Endocrinol2006，253，12： | 1 |
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