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| 1 | Anti-diabetic effects and mechanisms of action of a Chinese herbal medicine preparation JQ-R in vitro and in diabetic KKAy mice显示文摘Refined-JQ(JQ-R) is a mixture of refined extracts from Coptis chinensis(Ranunculaceae),Astragalus membranaceus(Leguminosae) and Lonicera japonica(Caprifoliaceae), the three major herbs of Jin Qi-Jiang Tang tablet, a traditional Chinese medicine(TCM) formula. The mechanisms by which JQ-R regulates glucose metabolism and improves insulin sensitivity were studied in type 2 diabetic KK^(Ay)mice and insulin-resistant L6 myotubes. To investigate the mechanisms by which JQ-R improves insulin sensitivity, a model of insulin-resistant cells induced with palmitic acid(PA) was established in L6 myotubes. Glucose uptake and expression of factors involved in insulin signaling, stress, and inflammatory pathways were detected by immunoblotting. JQ-R showed beneficial effects on glucose homeostasis and insulin resistance in a euglycemic clamp experiment and decreased fasting insulin levels in diabetic KK^(Ay)mice. JQ-R also improved the plasma lipid profiles. JQ-R directly increased the activity of superoxide dismutase(SOD) and decreased malondialdehyde(MDA) as well as inducible nitric oxide synthase(iNOS) levels in insulin-resistant L6 cells, and elevated the insulin-stimulated glucose uptake with upregulated phosphorylation of AKT. The phosphorylation levels of nuclear factor kappa B(NF-κB p65), inhibitor of NF-κB(IκBα), c-Jun N-terminal kinase(JNK1/2) and extracellular-signal-regulated kinases(ERK1/2) were also changed after JQ-R treatment compared with the control group. Together these findings suggest that JQ-R improved glucose and lipid metabolism in diabetic KK^(Ay)mice. JQ-R directly enhanced insulin-stimulated glucose uptake in insulin-resistant myotubes with improved insulin signalling and inflammatory response and oxidative stress. JQ-R could be a candidate to achieve improved glucose metabolism and insulin sensitivity in type 2 diabetes mellitus. | Quan Liu Shuainan Liu Lihui Gao Sujuan Sun Yi Huan Caina Li Yue Wang Nan Guo Zhufang Shen | 2017 | Acta Pharmaceutica Sinica B2017，7，4： | 11 |
| 2 | Facile synthesis of Li3V2(PO4)3/C cathode material for lithium-ion battery via freeze-drying显示文摘In this work, we report a facile route for the synthesis of Li3V2(PO4)3/C cathode material via freezedrying and then calcination. The effect of calcination temperature on the electrochemical properties of the Li3V2(PO4)3/C is also investigated. When used as a lithium-ion battery cathode, the optimized Li3V2(PO4)3/C (LVP-800) through calcination at 800 ℃ exhibits a high initial charge and discharge capacity. The excellent electrochemical performance of LVP-800 is attributed to the good crystallinity and uniform morphology of the electrode material. In addition, the residual carbon can also improve the conductivity and buffer the volume expansion during the Li-ion extraction/reinsertion. Meanwhile, charge compensation also plays an important role in excellent electrochemical performance. | Shuainan Guo Ying Bai Zhenfeng Geng Feng Wu Chuan Wu | 2019 | Journal of Energy Chemistry2019，28，5： | 8 |
| 3 | Role of ultrasonic oscillation in chemical processes in microreactors:A mesoscale issue显示文摘The integration of microreactor and ultrasound represents an emerging area for process intensification and has attracted considerable attention in recent years.One of the most important meso-scientific issues in ultrasound techniques is acoustic cavitation,which plays a vital role in the macroscopic performance of an ultrasonic microreactor.In this review,we first briefly summarize the latest research on acoustic cavitation phenomena in microreactors.The effects of channel configuration,solvent properties,and ultrasound parameters are systematically reviewed.In addition,the role of acoustic cavitation in various chemical processes(e.g.,mixing,absorption,emulsification,and particle synthesis)is presented from a mesoscale perspective,which in turn provides guidance for ultrasound applications.A thorough under-standing of the ultrasound intensification mechanism will contribute to the future development of this promising technology. | Shuainan Zhao Chaoqun Yao Zhengya Dong Guangwen Chen Quan Yuan | 2020 | Particuology2020，18，1： | 3 |
| 4 | Application of contrast-enhanced ultrasound in minimally invasive ablation of benign thyroid nodules显示文摘Objective:This study aimed to investigate the application value of contrast-enhanced ultrasound(CEUS)before and after minimally invasive ablation procedures for benign thyroid nodule(s)(BTN).Methods:This prospective study included patients with BTNs scheduled to undergo ultrasound-guided minimally invasive ablation treatment.CEUS was performed before and after ablation(at 1 day,and 1,6,and 12 months after ablation).Changes in microvascular perfusion and the volume of BTNs were noted and assessed.Results:Sixty-two patients(62 BTNs),who underwent ablation procedures between June 2016 and August 2020,were included.All lesions were confirmed by biopsy,and histopathological results were obtained before ablation treatment.On preoperative CEUS,the lesions exhibited hyperenhancement(53.23%)or iso-enhancement(46.77%)during the arterial phase,and all lesions exhibited iso-enhancement in the venous and late phases.One day after ablation,none of the BTNs exhibited obvious enhancement on CEUS.One(1.61%)lesion was retreated due to a nodule-like enhancement area detected by CEUS at the 6-month follow-up.The mean nodular volume reduction rate(VRR)at 1,6,and 12 months follow-up demonstrated no significant difference between the two ablation groups(microwave ablation versus radiofrequency ablation).Twelve months after ablation,the mean(±SD)VRR of all BTNs was 60.3±10.3%.Conclusion:CEUS helped guide treatment decisions for BTNs before ablation treatment.Moreover,it could also be used to accurately and noninvasively evaluate treatment efficacy. | Jiaying Cao Peili Fan Feihang Wang Shuainan Shi Lingxiao Liu Zhiping Yan Yi Dong Wenping Wang | 2022 | Journal of Interventional Medicine2022，5，1： | 3 |
| 5 | Reversible Al^(3+) storage mechanism in anatase TiO_(2) cathode material for ionic liquid electrolyte-based aluminum-ion batteries显示文摘Rechargeable aluminum ion battery(AIB) with high theoretical specific capacity, abundant elements and low cost engages considerable attention as a promising next generation energy storage and conversion system. Nevertheless, to date, one of the major barriers to pursuit better AIB is the limited applicable cathode materials with the ability to store aluminum highly reversibly. Herein, a highly reversible AIB is proposed using mesoporous TiO2 microparticles(M-TiO2) as the cathode material. The improved performance of Ti O2/Al battery is ascribed to the high ionic conductivity and material stability, which is caused by the stable architecture with a mesoporous microstructure and no random aggregation of secondary particles. In addition, we conducted detailed characterization to gain deeper understanding of the Al^(3+) storage mechanism in anatase Ti O2 for AIB. Our findings demonstrate clearly that Al^(3+)can be reversibly stored in anatase TiO2 by intercalation reactions based on ionic liquid electrolyte. Especially, DFT calculations were used to investigate the accurate insertion sites of aluminum ions in M-Ti O2 and the volume changes of M-TiO2 cells during discharging. As for the controversial side reactions in AIBs, in this work, by normalized calculation, we confirm that M-Ti O2 alone participate in the redox reaction. Moreover, cyclic voltammetry(CV) test was performed to investigate the pseudocapacitive behavior. | Na Zhu Feng Wu Zhaohua Wang Liming Ling Haoyi Yang Yaning Gao Shuainan Guo liumin Suo Hong Li Huajie Xu Ying Bai Chuan Wu | 2020 | Journal of Energy Chemistry2020，29，12： | 3 |
| 6 | Efficient single-component white light emitting diodes enabled by lanthanide ions doped lead halide perovskites via controlling Forster energy transfer and specific defect clearance显示文摘Currently,a major challenge for metal-halide perovskite light emitting diodes(LEDs)is to achieve stable and efficient white light emission due to halide ion segregation.Herein,we report a promising method to fabricate white perovskite LEDs using lanthanide(Ln^(3+))ions doped CsPbCl_(3) perovskite nanocrystals(PeNCs).First,K^(+)ions are doped into the lattice to tune the perovskite bandgap by partially substituting Cs^(+)ions,which are well matched to the transition energy of some Ln^(3+)ions from the ground state to the excited state,thereby greatly improving the Förster energy transfer efficiency from excitons to Ln3+ions.Then,creatine phosphate(CP),a phospholipid widely found in organisms,serves as a tightly binding surface-capping multi-functional ligand which regulates the film formation and enhances the optical and electrical properties of PeNC film.Consequently,the Eu^(3+)doped PeNCs based-white LEDs show a peak luminance of 1678 cd m^(-2) and a maximum external quantum efficiency(EQE)of 5.4%,demonstrating excellent performance among existing white PeNC LEDs from a single chip.Furthermore,the method of bandgap modulation and the defect passivation were generalized to other Ln^(3+)ions doped perovskite LEDs and successfully obtained improved electroluminescence(EL).This work demonstrates the comprehensive and universal strategies in the realization of highly efficient and stable white LEDs via single-component Ln^(3+)ions doped PeNCs,which provides an optimal solution for the development of low-cost and simple white perovskite LEDs. | Rui Sun Donglei Zhou Yujiao Ding Yue Wang Yuqi Wang Xinmeng Zhuang Shuainan Liu Nan Ding Tianyuan Wang Wen Xu Hongwei Song | 2022 | Light(Science & Applications)2022，11，12： | 3 |
| 7 | Effect of rich R-TiO2 on the rate and cycle properties of Li4Ti5O12 as anode for lithium ion batteries显示文摘Li4Ti5012 (LTO) with rich R-TiO2 (17.06, 23.69, and 34.42 wt%), namely, R-TiO2@Li4Ti5O12 composites, were synthesized using the hydrothermal method and tetrabutyl titanate (TBT) as the precursor. Rietveld refinement of X-ray diffraction (XRD) results show that the proportion of Li occupying 16d sites is extraordinary low and the lattice constants of LTO and R-TiO2 change with the ritanium dioxide content. EIS measurements showed that with in creasing R-TiO2 content, both its charge transfer impedance (Rct) and lithium ion diffusion coefficient (DLi) decreased. The changes of Rct and DLi caused by the increase of titanium dioxide content have synergic-antagonistic effects on the rate and cycle properties of Li4Ti5012. The rate performance is positively related to DLi, while the cycle property is negatively correlated with Rct, indicati ng that the rate performs nee is mainly related to DLi, while Rct more significantly affects the cycle performance. LTO-RT-17.06% exhibited excellent rate properties, especially under a high current density (5.0 C, 132.5 mAh/g) and LTO-RT-34.42% showed superior long-term cycle performance (0.012% capacity loss per cycle) compared to that of LTO-RT-17.06% and LTO-RT-23.69%. | Delai Qian Yijie Gu Shuainan Guo Hongquan Liu Yunbo Chen Juan Wang Guoxuan Ma Chuan Wu | 2019 | Journal of Energy Chemistry2019，28，5： | 3 |
| 8 | The application of 2-NBDG as a fluorescent tracer for assessing hepatic glucose production in mice during hyperinsulinemic euglycemic clamp显示文摘Methods of performing insulin clamps vary between laboratories.Here we present a protocol of insulin clamping in conscious mice,with the significant advantage of avoiding multiple surgical catheterizations and non-physiologic metabolism during the induction of anesthesia.Using this technique we also established a new method for measuring hepa tic glucose production(HGP)using a fuorescent D-glucose analog,2-[N-(7-nitrobenz-2-oxa-1,3-diazol-4-yl)amino]-2-deoxyglu-cose(2-NBDG).To prove the reliability and feasibility of this method,whole-body insulin sensitivity was compared between conscious normal ICR mice and diabetic KK^(Ay) mice using the insulin clamp.Basal and clamp HGP was compared between normal C57 mice and diabetic db/db mice by using the modified clamp with 2-NBDG as a tracer.The glucose infusion rate(GIR),an index of insulin sensitivity,was significantly lower in KKAy mice than normal ICR mice.(6.2±1.3 mg/kg/min vs.31.3±2.9 mg/kg/min,P<0.001).The db/db mice also showed higher basal hepatic glucose production(25.8±2.2 mg/kg/min vs.16.7±2.5 mg/kg/min,P<0.05),higher clamp HGP after insulin suppression(7.3±1.0 mg/kg/min vs.0 mg/kg/min,P<0.001),and lower GIR(71.6±2.8 mg/kg/min vs.15.2±1.6 mg/kg/min,P<0.001)than that obtained with normal C57 mice.In conclusion,this is the first report of the application of 2-NBDG,rather than isotopic tracers,for the determination of HGP in vivo. | Shuainan Liu Quan Liu Sujuan Sun Qian Jiang Jun Peng Zhufang Shen | 2012 | Acta Pharmaceutica Sinica B2012，2，4： | 2 |
| 9 | A cell-based fluorescent glucose transporter assay for SGLT2 inhibitor discovery显示文摘The sodium/glucose cotransporter 2(SGLT2)is responsible for the majority of glucose reabsorption in the kidney,and currently,SGLT2 inhibitors are considered as promising hypoglycemic agents for the treatment of type 2 diabetes mellitus.By constructing CHO cell lines that stably express the human SGLT2 transmembrane protein,along with a fluorescent glucose transporter assay that uses 2-[N-(7-nitrobenz-2-oxa-l,3-diazol-4-yl)amino]2-deoxyglucose(2-NBDG)as a glucose analog,we have developed a nonradioactive,cell-based assay for the discovery and characterization of SGLT2 inhibitors. | Yi Huan Linyi Li Quan Liu Shuainan Liu Zhufang Shen | 2013 | Acta Pharmaceutica Sinica B2013，3，2： | 1 |
| 10 | The immunomodulatory effect of bone marrow stromal cells (BMSCs) on interleukin (IL)-23/IL-17-mediated ischemic stroke in mice显示文摘 | Shuainan Ma Di Zhong Hongping Chen Yi Zheng Yanyan Sun Jian Luo Hulun Li Guozhong Li Yanhong Yin | 2013 | Journal of Neuroimmunology . 2013 (1-2)2013，，1： | 1 |
| 11 | Effects of Plant Community Type on Soil Methane Flux in Semiarid Loess Hilly Region,Central Gansu Province,China显示文摘Methane(CH_(4))is an important greenhouse gas second only to CO_(2)in terms of its greenhouse effect.Vegetation plays an important role in controlling soil CH_(4)fluxes,but the spatial variability of soil CH_(4)fluxes during vegetation restoration in Loess Hilly Region(LHR)is not fully understood.The effects of different plant community types[Medicago sativa grassland(MS);Xanthoceras sorbifolium forestland(XS);Caragana korshinskii bushland(CK);Hippophae rhamnoides shrubland(HR);and Stipa bungeana grassland(SB)]on soil CH_(4)flux in LHR were studied via the static chamber technique.The results showed that the five plant community types were sinks of soil CH_(4)in LHR,the plant community type significantly affected the soil CH_(4)flux,and the average CH_(4)uptake from high to low was in SB,HR,CK,MS,and XS.During the whole study period,the soil CH_(4)flux showed similar interannual variation.The maximum absorption of soil CH_(4)appeared in the growing season,while the minimum appeared in winter.Soil CH_(4)uptake was positively correlated with soil temperature and soil moisture.Soil temperature and moisture are important controlling factors for the temporal variability of soil CH_(4)flux.In LHR,the Stipa bungeana grassland is the more suitable plant community type for reducing soil CH_(4)emissions.In the process of vegetation restoration in LHR,the soil CH_(4)absorption potential of different plant community types should be considered,ecological benefits should be taken into account,and vegetation more suitable for mitigating the greenhouse effect should be selected. | Chuanjie YANG Guang LI Lijuan YAN Weiwei MA Jiangqi WU Yan TAN Shuainan LIU Shikang ZHANG | 2022 | Advances in Atmospheric Sciences2022，39，8： | 1 |
| 12 | Separation and recovery of rare earth from waste nickel-metal hydride batteries by phosphate based extraction-precipitation显示文摘A novel type of extraction-precipitation strategy based on phosphate was developed to recover rare earth(RE,i.e.,La,Ce,Nd,and Pr)from waste nickel-metal hydride(NiMH)batteries.This method does not require saponification and organic solvents.The novel phosphates,i.e.,dibenzyl phosphate(DBP),diphenyl phosphate(DPP),triphenyl phosphate(TPP)were studied as extraction-precipitants.DBP has high precipitation efficiencies for RE^(3+),which can reach 97.84%,100%,100%and 99.77%,respectively.In addition,the precipitation efficiencies of Mn^(2+),Co^(2+)and Ni^(2+)are less than 1.75%.DBP-RE has the largest particle size(D10=52.6μm,D50=135.35μm,D90=296.08μm),which is much larger than the precipitations formed by NH_(4)HCO_(3),H_(2)C2O_(4),CaO and MgO.The larger precipitation particle sizes contribute to improving the solid-liquid separation efficiency.With 3 mol/L hydrochloric acid,the stripping efficiency of DBP-RE reaches 98.60%,and the purity of recovered RE is 99.85%.The regenerated DBP can be directly used for the recycling extraction.Therefore,the novel extraction-precipitation strategy is a green and sustainable separation method. | Hailan Zhi Shuainan Ni Xiang Su Wenqi Xie Hepeng Zhang Xiaoqi Sun | 2022 | Journal of Rare Earths2022，40，6： | 0 |
| 13 | CoSnO_(3)/C nanocubes with oxygen vacancy as high-capacity cathode materials for rechargeable aluminum batteries显示文摘Rechargeable aluminum batteries(RABs)are attractive cadidates for next-generation energy storage and conversion,due to the low cost and high safety of Al resources,and high capacity of metal Al based on the three-electrons reaction mechanism.However,the development of RABs is greatly limited,because of the lack of advanced cathode materials,and their complicated and unclear reaction mechanisms.Exploring the novel nanostructured transition metal and carbon composites is an effective route for obtaining ideal cathode materials.In this work,we synthesize porous CoSnO_(3)/C nanocubes with oxygen vacancies for utilizing as cathodes in RABs for the first time.The intrinsic structure stability of the mixed metal cations and carbon coating can improve the cycling performance of cathodes by regulating the internal strains of the electrodes during volume expansion.The nanocubes with porous structures contribute to fast mass transportation which improves the rate capability.In addition to this,abundant oxygen vacancies promote the adsorption affinity of cathodes,which improves storage capacity.As a result,the CoSnO_(3)/C cathodes display an excellent reversible capacity of 292.1 mAh g^(-1) at 0.1 A g^(-1),a good rate performance with 109 mAh g^(-1) that is maintained even at 1 A g^(-1) and the provided stable cycling behavior for 500 cycles.Besides,a mechanism of intercalation of Al^(3+)within CoSnO_(3)/C cathode is proposed for the electrochemical process.Overall,this work provides a step toward the development of advanced cathode materials for RABs by engineering novel nanostructured mixed transition-metal oxides with carbon composite and proposes novel insights into chemistry for RABs. | Shuainan Guo Mingquan Liu Haoyi Yang Xin Feng Ying Bai Chuan Wu | 2023 | Green Energy & Environment2023，8，3： | 0 |
| 14 | Separation of aluminum from rare earth by solvent extraction with 4-octyloxybenzoic acid显示文摘Leaching method is usually used to extract rare earth(RE)elements from ion adsorbed RE ores.In the leaching process,some impurities such as aluminum(Al)enter the leaching solution.The separation of Al from RE by carboxylic acid extractant 4-octyloxybenzoic acid(POOA)was studied in this article.By changing the pH value,temperature,solvent,saponification degree and other parameters,the extraction and separation performance of POOA in chloride system was systematically studied.Through specific extraction experiments and slope analysis,it can be seen that the stoichiometric ratio of POOA to Al is 3:1during the extraction process.The separation factor of Al^(3+)and Pr^(3+)can reach about 160.00.Compared with easily emulsified naphthenic acid,POOA achieves better phase separation.The above results show that saponified POOA(S-POOA)has a good separation effect on Al and RE.Under the condition of low concentration stripping acid of 0.60 mol/L HCl,the developed extraction system can be almost completely stripped,and the stripping rate reaches 97.52%.The regenerated POOA can be directly used for the recycling extraction. | Gaoshan Yu Zhiyuan Zeng Yun Gao Shuainan Ni Hepeng Zhang Xiaoqi Sun | 2023 | Journal of Rare Earths2023，41，2： | 0 |
| 15 | 骨髓造血细胞来源的半乳糖苷凝集素导致细胞和系统胰岛素抵抗显示文摘肥胖时巨噬细胞与其他免疫细胞在胰岛素靶组织大量聚集,构成一种慢性炎症状态和胰岛素抵抗。半乳糖苷凝集素Galectin-3(Ga13)主要来源于巨噬细胞。无论在肥胖小鼠或者肥胖病人,Ga13水平明显增加。 | 李平平 Shuainan Liu Min Lu Gautum Bandyopadhyay Dayoung Oh Takeshi Imamura Andrew M.F.Johnson Dorothy Sears Zhufang Shen Bing Cui Lijuan Kong Shaocong Hou Xiao Liang Salvatore Iovino Steven M.Watkins Wei Ying Olivia Osborn Joshua Wollam Martin Brenner Jerrold M.Olefsky | 2017 | 科学新闻2017，19，4： | 0 |
| 16 | Conservation:Elephant in the Room显示文摘A national park for Asian elephants is being developed in Yunnan Province.Will it help solve the tension between elephant survival and livelihoods?In mid-August 2021,a group of Asian elephants returned to their habitat in the south of Yunnan Province,after a 1,500-kilometer journey to the north of the province which started in March 2020.Now Yunnan is accelerating the designation of a national Asian elephant park,according to a report by the Yunnan Daily on August 1l.The report came a day before World Elephant Day,which was created in 2012 by Canadian filmmaker Patricia Sims,director of the award-winning film about human-elephant relations,When the Elephants Were Young and the Elephant Reintroduction Foundation of Thailand,an initiative of Queen Sirikit of Thailand to improve awareness of elephant protection worldwide. | Hu Yuanhang Han Shuainan | 2022 | China Weekly2022，，10： | 0 |
| 17 | Exosome Biomarkers in Cardiovascular Diseases and their Prospective Forensic Application in the Identification of Sudden Cardiac Death显示文摘Sudden cardiac death(SCD)is a common cause of death due to the high prevalence and mortality of cardiovascular disease(CVD).Currently,the forensic identification of SCD relies on traditional histomorphological examination,lacking stable biomarkers with high specificity and sensitivity.Previous studies have shown that exosomes(Exos)are ideal vectors and the application of Exos provides novel insight as the diagnostic biomarkers and treatment of CVD,and is hot research filed in biomedicine.This review briefly describes the biology of Exos,including the biogenesis of Exos and the mechanisms of action.The research progresses on Exos multi‑omics,i.e.,genomics,proteomics and metabolomics,and their roles in the diagnosis of different types of CVD,especially coronary heart disease and cardiomyopathy,are summarized.In addition,the current difficulties of applications of Exos in forensic identification of SCD and the prospective forensic applications in the future are highlighted.The aim of this review is to summarize the current advances of Exos in CVD in a disease‑oriented manner,and to provide a reference for future forensic pathological identification of SCD,as well as the early diagnosis of SCD in clinic. | Ye Wang Jie Wang Li Hu Shuainan Huang Yue Cao Youjia Yu Feng Chen | 2022 | Journal of Forensic Science and Medicine2022，8，4： | 0 |
| 18 | Ultrasonic emulsification: basic characteristics, cavitation, mechanism, devices and application显示文摘Emulsion systems are widely applied in agriculture,food,cosmetic,pharmaceutical and biomedical industries.Ultrasound has attracted much attention in emulsion preparation,especially for nanoemulsion,due to its advantages of being eco-friendly,cost-effective and energy-efficient.This review provides an overview for readers to the area of ultrasonic emulsification technology.It briefly introduces and summarizes knowledge of ultrasonic emulsification,including emulsion characteristics,acoustic cavitation,emulsification mechanism,ultrasonic devices and applications.The combination of microfluidics and ultrasound is highlighted with huge advantages in controlling cavitation phenomena and emulsification intensification.A novel scale of dμC^(0.6)/μD^(0.33)−EV is proposed to be able to compare the energy efficiency of emulsion preparation in different devices. | Chaoqun Yao Shuainan Zhao Lixue Liu Zhikai Liu Guangwen Chen | 2022 | Frontiers of Chemical Science and Engineering2022，16，11： | 0 |
| 19 | Recyclable hydrolyzed polymers of intrinsic microporosity-1/Fe_(3)O_(4) magnetic composites as adsorbents for selective cationic dye adsorption显示文摘Polymers of intrinsic microporosity shows great potential for dye adsorption and magnetic Fe_(3)O_(4) are easy to be separated.In this work,hydrolyzed polymers of intrinsic microporosity-1/Fe_(3)O_(4) composite adsorbents were prepared by phase inversion and hydrolysis process for cationic dye adsorption.The chemical structure and morphology of the composite adsorbents were systematically characterized by several characterization methods.Using methylene blue as the target dye,the influences of solution pH,contact time,initial dye concentration,and system temperature on the methylene blue adsorption process were investigated.The incorporation of Fe_(3)O_(4) particle into hydrolyzed polymers of intrinsic microporosity-1 endow the adsorbent with high magnetic saturation(20.7 emu·g^(–1))which allows the rapid separation of the adsorbent.Furthermore,the adsorption process was simulated by adsorption kinetics,isotherms and thermodynamics to gain insight onto the intrinsic adsorption mechanism.In addition,the composite adsorbents are able to selectively adsorb cationic dyes from mixed dyes solution.Hydrolyzed polymers of intrinsic microporosity/Fe_(3)O_(4) shows only a slight decrease for methylene blue adsorption after 10 adsorption/regeneration cycles,demonstrating the outstanding regeneration performance.The high adsorption capacity,outstanding regeneration ability,together with simple preparation method,endow the composite adsorbents great potential for selective removal of cationic dyes in wastewater system. | Feng Zhang Shuainan Xu Xiumei Geng Meixia Shan Yatao Zhang | 2024 | Frontiers of Chemical Science and Engineering2024，18，2： | 0 |
| 20 | Domain-Decomposition Localized Method of Fundamental Solutions for Large-Scale Heat Conduction in Anisotropic Layered Materials显示文摘The localized method of fundamental solutions(LMFS)is a relatively new meshless boundary collocation method.In the LMFS,the global MFS approxima-tion which is expensive to evaluate is replaced by local MFS formulation defined in a set of overlapping subdomains.The LMFS algorithm therefore converts differential equations into sparse rather than dense matrices which are much cheaper to calcu-late.This paper makes thefirst attempt to apply the LMFS,in conjunction with a domain-decomposition technique,for the numerical solution of steady-state heat con-duction problems in two-dimensional(2D)anisotropic layered materials.Here,the layered material is decomposed into several subdomains along the layer-layer inter-faces,and in each of the subdomains,the solution is approximated by using the LMFS expansion.On the subdomain interface,compatibility of temperatures and heatfluxes are imposed.Preliminary numerical experiments illustrate that the proposed domain-decomposition LMFS algorithm is accurate,stable and computationally efficient for the numerical solution of large-scale multi-layered materials. | Shuainan Liu Zhuojia Fu Yan Gu | 2022 | Advances in Applied Mathematics and Mechanics2022，14，3： | 0 |
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