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| 1 | An novel identification method of the environmental risk sources for surfacewater pollution accidents in chemical industrial parks显示文摘The chemical industry is a major source of various pollution accidents. Improving the management level of risk sources for pollution accidents has become an urgentdemand for most industrialized countries. In pollution accidents, the released chemicals harm the receptors to some extentdepending on their sensitivity or susceptibility. Therefore, identifying the potential risk sources from such a large number of chemical enterprises has become pressingly urgent. Based on the simulation of thewhole accident process, a novel and expandable identification method for risk sources causingwater pollution accidents is presented. The newlydeveloped approach, by analyzing and stimulating thewhole process of a pollution accident between sources and receptors, can be applied to identify risk sources, especially on the nationwide scale. Three major types of losses, such as social, economic and ecological losses,were normalized, analyzed and used for overall consequence modeling. A specific case study area, located in a chemical industry park (CIP) along the Yangtze River in Jiangsu Province, China,was selected to test the potential of the identification method. The results showed that therewere four risk sources for pollution accidents in this CIP. Aniline leakage in the HS Chemical Plantwould lead to the most serious impact on the surroundingwater environment. This potential accidentwould severelydamage the ecosystem up to3.8 kmdownstream of Yangtze River, and lead to pollution over adistance stretching to 73.7 kmdownstream. The proposed method is easily extended to the nationwide identification of potential risk sources. | Jianfeng Peng Yonghui Song Peng Yuan Shuhu Xiao Lu Han | 2013 | Journal of Environmental Sciences2013，25，7： | 9 |
| 2 | Enhanced photoelectrocatalytic degradation of ammonia by in situ photoelectrogenerated active chlorine on TiO_2 nanotube electrodes显示文摘TiO_2 nanotube(Ti NT) electrodes anodized in fluorinated organic solutions were successfully prepared on Ti sheets. Field-emission scanning electron microscopy(FE-SEM) and X-ray diffraction(XRD) were performed to characterize the TiNT electrodes. The linear voltammetry results under irradiation showed that the TiNT electrode annealed at 450°C presented the highest photoelectrochemical activity. By combining photocatalytic with electrochemical process, a significantly synergetic effect on ammonia degradation was observed with Na_2SO_4 as supporting electrolyte at pH 10.7. Furthermore, the photoelectrocatalytic efficiency on the ammonia degradation was greatly enhanced in presence of chloride ions without the limitation of pH. The degradation rate was improved by 14.8 times reaching 4.98 × 10^(-2) min^(-1) at pH 10.7 and a faster degradation rate of 6.34 × 10^(-2) min^(-1)was obtained at pH 3.01. The in situ photoelectrocatalytic generated active chlorine was proposed to be responsible for the improved efficiency. On the other hand, an enhanced degradation of ammonia using TiNT electrode fabricated in fluorinated organic solution was also confirmed compared to TiNT electrode anodized in fluorinated water solution and TiO_2 film electrode fabricated by sol–gel method. Finally, the effect of chloride concentration was also discussed. | Shuhu Xiao Dongjin Wan Kun Zhang Hongbin Qu Jianfeng Peng | 2016 | Journal of Environmental Sciences2016，28，12： | 2 |
| 3 | 显示文摘 | Zhu Hua Zhong Lian Xiao Shuhu | 2004 | Electrochimica Acta2004，49，： | 1 |
| 4 | Application ofPolyaniline to Galvanic Anodic Protection on Stainless Steel in H2SO4 Solutions显示文摘 | Zhong Lian Xiao Shuhu Hu Jie | 2006 | Corrosion Science2006，48，12： | 1 |
| 5 | Degradation of biologically treated landfill leachate by using electrochemical process combined with UV irradiation显示文摘 | Shuhu Xiao Jianfeng Peng Yonghui Song Dongsheng Zhang Ruixia Liu Ping Zeng | 2013 | Separation and Purification Technology2013，，： | 1 |
| 6 | Integrated UV-based photo microreactor-distillation technology toward process intensification of continuous ultra-high-purity electronic-grade silicon tetrachloride manufacture显示文摘Ultra-high-purity silicon tetrachloride(SiCl4)is demanded as an electronic-grade chemical to meet the stringent requirements of the rapidly developing semiconductor industry.The high requirement for ultra-high-purity SiCl4 has created the need for a high-efficient process for reducing energy consumption as well as satisfying product quality.In this paper,a mass of production technology of ultra-high-purity SiCl4 was successfully developed through chlorination reaction in the ultraviolet(UV)-based photo microreactor coupled with the distillation process.The influences of key operational parameters,including temperature,pressure,UV wavelength and light intensity on the product quality,especially for hydrogen-containing impurities,were quantified by the infrared transmittance of Fourier transform infrared spectroscopy(FT-IR)at 2185 cm^-1and 2160 cm^-1indicating that chara cteristic vib rational modes of Si-H bonds,as well as the operating conditions of distillation were also investigated as key factors for metal impurities removing.The advanced intensification of SiCl4 manufactured by the integration of photo microreactor and distillation achieves the products with superior specifications higher than the standard commercial products. | Ye Wan Wenhui Guo Jin Xiao Dazhou Yan Xiong Zhao Shuhu Guo Jianhua Liu Qifan Zhong Tao Yang Yu Zhao Xin Chang Xin Gao | 2020 | Chinese Journal of Chemical Engineering2020，28，9： | 1 |
| 7 | Treatment of berberine hydrochloride wastewater by using pulse electro-coagulation process with Fe electrode显示文摘 | Meijie Ren Yonghui Song Shuhu Xiao Ping Zeng Jianfeng Peng | 2011 | Chemical Engineering Journal2011，，1： | 1 |
| 8 | Application of polyaniline to galvanic anodie protection on stainless steel in H2SO4 solutions显示文摘 | Lian Zhong Shuhu Xiao Jie Hu | 2006 | Corrosion science2006，48，12： | 1 |
| 9 | Microwave electrodeless lamp assisted catalytic degradation of X-GRL with manganese dioxides: Adsorption and manganese(IV) reductive dissolution effects显示文摘 | Ruiping Liu Hongjie Wang Xu Zhao Shuhu Xiao Jiuhui Qu | 2008 | Catalysis Today2008，，1： | 1 |
| 10 | Accelerating Effect and Mechanism of Passivation of Polyaniline on Ferrous Metals显示文摘 | Zhu Hua Zhong Lian Xiao Shuhu | 2004 | Electrochimica Acta2004，49，： | 1 |
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