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2篇 您的检索式:作者名="Wayesh Qarony"
    题名 作者 年代 出处 被引量
1Spray Pyrolyzed TiO2 Embedded Multi-Layer Front Contact Design for High-Efficiency Perovskite Solar Cells显示文摘The photovoltaic performance of perovskite solar cells(PSCs)can be improved by utilizing efficient front contact.However,it has always been a significant challenge for fabricating high-quality,scalable,controllable,and cost-effective front contact.This study proposes a realistic multi-layer front contact design to realize efficient single-junction PSCs and perovskite/perovskite tandem solar cells(TSCs).As a critical part of the front contact,we prepared a highly compact titanium oxide(TiO2)film by industrially viable Spray Pyrolysis Deposition(SPD),which acts as a potential electron transport layer(ETL)for the fabrication of PSCs.Optimization and reproducibility of the TiO2 ETL were discreetly investigated while fabricating a set of planar PSCs.As the front contact has a significant influence on the optoelectronic properties of PSCs,hence,we investigated the optics and electrical effects of PSCs by three-dimensional(3D)finite-difference time-domain(FDTD)and finite element method(FEM)rigorous simulations.The investigation allows us to compare experimental results with the outcome from simulations.Furthermore,an optimized single-junction PSC is designed to enhance the energy conversion efficiency(ECE)by>30% compared to the planar reference PSC.Finally,the study has been progressed to the realization of all-perovskite TSC that can reach the ECE,exceeding 30%.Detailed guidance for the completion of high-performance PSCs is provided.Md.Shahiduzzaman Mohammad Ismail Hossain Sem Visal Tetsuya Kaneko Wayesh Qarony Shinjiro Umezu Koji Tomita Satoru Iwamori Dietmar Knipp Yuen Hong Tsang Md.Akhtaruzzaman Jean-Michel Nunzi Tetsuya Taima Masao Isomura 2021Nano-Micro Letters2021,13,2:0
2Controllable optical emission wavelength in all-inorganic halide perovskite alloy microplates grown by two-step chemical vapor deposition显示文摘All-inorganic halide perovskites(IHP),CsPbX_(3)(X=Cl,Br,I)exhibiting efficient optical emissions within the spectral range of 410 to 730 nm are potential candidates for many optoelectronic devices.Anion alloying of these IHPs is expected to achieve tunable emission wavelength covering the entire visible spectrum.Here,we developed a two-step chemical vapor deposition(CVD)process for growing quaternary IHP CsPbX_(3)(X=Cl/Br and Br/I)alloys.By exploiting the fast diffusion of halide anions in IHPs,the alloy composition can be precisely controlled by the growth time of the respective layers once the growth of the individual ternary IHP is optimized.Hence complexities in the multi-parameter optimization in the conventional CVD growth of quaternary alloys can be mitigated.Using this process,we synthesized single crystalline,homogeneous and thermally stable CsPbCl3_((1−X))Br_(3x)and CsPbBr3_((1−X))I_(3x)perovskites alloy microplates and demonstrated continuously tunable emission covering the spectrum from 428 to 715 nm by varying the halide compositions in the alloys.These alloy microplates also exhibit room temperature amplified spontaneous emissions(ASE)along with strong photonic discharges from the microplate’s edges and hence are potentially useful as a gain medium as well as optical cavities for emissions with wavelengths covering the visible spectrum.Mohammad K.Hossain Pengfei Guo Wayesh Qarony Yuen H.Tsang Chaoping Liu Sai W.Tsang Johnny C.Ho Kin M.Yu 2020Nano Research2020,13,11:0
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