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| 1 | A techno-economic and life cycle assessment for the production of green methanol from CO_(2): catalyst and process bottlenecks显示文摘The success of catalytic schemes for the large-scale valorization of CO_(2) does not only depend on the development of active,selective and stable catalytic materials but also on the overall process design.Here we present a multidisciplinary study(from catalyst to plant and techno-economic/lifecycle analysis)for the production of green methanol from renewable H2 and CO_(2).We combine an in-depth kinetic analysis of one of the most promising recently reported methanol-synthesis catalysts(InCo)with a thorough process simulation and techno-economic assessment.We then perform a life cycle assessment of the simulated process to gauge the real environmental impact of green methanol production from CO_(2).Our results indicate that up to 1.75 ton of CO_(2) can be abated per ton of produced methanol only if renewable energy is used to run the process,while the sensitivity analysis suggest that either rock-bottom H2 prices(1.5$kg1)or severe CO_(2) taxation(300$per ton)are needed for a profitable methanol plant.Besides,we herein highlight and analyze some critical bottlenecks of the process.Especial attention has been paid to the contribution of H2 to the overall plant costs,CH4 trace formation,and purity and costs of raw gases.In addition to providing important information for policy makers and industrialists,directions for catalyst(and therefore process)improvements are outlined. | Tomas Cordero-Lanzac Adrian Ramirez Alberto Navajas Lieven Gevers Sirio Brunialti Luis MGandía Andrés T.Aguayo S.Mani Sarathy Jorge Gascon | 2022 | Journal of Energy Chemistry2022，31，5： | 3 |
| 2 | TLR2, TLR2, CD14, CDllB, and CDllC expressions on monoeytes surface and cytokine production in patients with sepsis, severe sepsis, and septic shock显示文摘 | Brunialti MK Martins PS Barbosa de Carvalho H | 2006 | Shock2006，25，4： | 1 |
| 3 | Bacterial sensing, cell signaling, and modulation of the immune response during sepsis显示文摘 | Salomao R Brunialti MK Rapozo MM | 2012 | Shock2012，38，3： | 1 |
| 4 | TLR signalling pathway in patients with sepsis显示文摘 | Salomao R Martins PS Brunialti MKC | 2008 | Shock2008，30，1： | 1 |
| 5 | Increased percentages of T helper cells producing IL-17 and monocytes expressing markers of alternative activation in patients with sepsis显示文摘 | Brunialti MK Santos MC Rigato O | | 0，，05： | 1 |
| 6 | Leptospira interrogans activation of peripheral blood monocyte glycolipoprotein demonstrated in whole blood by the re- lease of IL-6显示文摘 | Dorigatti F Brunialti M Romero E | 2005 | Braz J Mde Biol Res2005，38，： | 1 |
| 7 | PCR-based diagnosis to evaluate the performance of malaria reference centers显示文摘 | Di Santi SM Kirchgatter K Brunialti KC | 2004 | Rev Inst Med Trop Sao Paulo2004，46，： | 1 |
| 8 | Differential expression of toll-like receptor signaling cascades in LPS-tolerant human peripheral blood mononuclear cells 显示文摘 | Mendes ME Baggio-Zappia GL Brunialti MK | 2011 | Immunobiology2011，216，3： | 1 |
| 9 | Bacterial sensing, cell signaling, and modulation of the immune response during sepsis 显示文摘 | Selomao R Brunialti MK Rapozo MM | 2012 | Shock2012，38，3： | 1 |
| 10 | Peripheral blood mononuclear cell activation induced by Leptospira interrogans glycolipoprotein 显示文摘 | Diament D Brunialti MK Romero EC Kallas EG Salomao R | 2002 | Infect Immun2002，70，4： | 1 |
| 11 | Increased percentages of T helper cells producing IL-17 and monocytes expressing markers of alternative activation in patients with sepsis显示文摘 | Brunialti MK Santos MC Rigato 0 | 2012 | PLoS One2012，7，37： | 1 |
| 12 | Leptospira interrogans activation of peripheral blood monocyte glycolipoprotein demonstrated in whole blood by the release of IL-6 显示文摘 | Dorigatti F Brunialti MK Romero EC Kallas EG Salomao R | 2005 | Braz J Med Biol Res2005，38，6： | 1 |
| 13 | Evaluation of the effect of ketamine on remifentanil-induced hyperalgesia: a double-blind, ran- domized study显示文摘 | Leal PC Salomao R Brunialti MK | 2015 | Journal of clinical anesthesia2015，27，4： | 1 |
| 14 | Effects of atmospheric pollution on lichen biodiversity (LB) in a Mediterranean region (Liguria,northwest Italy)显示文摘 | Giordani P Brunialti G Alleteo D | 2002 | Environmental Pollution2002，118，1： | 1 |
| 15 | Increased percentages of T helper cells producing IL-17 and monocytes expressing markers of alternative activation in patients with sepsis显示文摘 | Brunialti MK Santos MC Rigato O | 2012 | PLoS One2012，7，37： | 1 |
| 16 | TLR2, TLR4, CD14, CDllB, and CDllC expressions on monocytes surface and cytokine production in patients with sepsis, severesepsis, and septic shock显示文摘 | Brunialti MKC Martins PS de Carvalho HB | 2006 | Shock2006，25，4： | 1 |
| 17 | Peripheral Blood Mononuclear Cell Activation Induced by Leptospira interrogans Glycolipoprotein显示文摘 | Diament D Brunialti MK Romero EC | 2002 | Infection and immunity2002，70，4： | 1 |
| 18 | Bacterial Sensing, Cell Signaling, and Modulation of the Immune Response During Sepsis显示文摘 | Reinaldo Salomao Milena Karina Colo Brunialti Marjorie Marini Rapozo Giovana Lotici Baggio-Zappia Chris Galanos Marina Freudenberg | 2012 | Shock2012，，3： | 1 |
| 19 | TLR2,TLR4,CD14,CD11B,and CD11C expressions on monocytes surface and cytokine production in patients with sepsis,severe sepsis,and septic shock显示文摘 | Brunialti MK Martins PS Barbosa de Carvalho H | 2006 | Shock2006，25，4： | 1 |
| 20 | Evaluation of a rapid dipstick test,Malar-check,for the diagnosis of plasmodium falciparum malaria in Brazil显示文摘 | AVILA P E KIRCHGATTER K BRUNIALTI K C | 2002 | Rev Inst Med Trop Sao Paulo2002，44，5： | 1 |
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