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| 1 | The recent development of soft x-ray interference lithography in SSRF显示文摘This paper introduces the recent progress in methodologies and their related applications based on the soft x-ray interference lithography beamline in the Shanghai synchrotron radiation facility.Dual-beam,multibeam interference lithography and Talbot lithography have been adopted as basic methods in the beamline.To improve the experimental performance,a precise real-time vibration evaluation system has been established;and the lithography stability has been greatly improved.In order to meet the demands for higher resolution and practical application,novel experimental methods have been developed,such as high-order diffraction interference exposure,high-aspect-ratio and large-area stitching exposure,and parallel direct writing achromatic Talbot lithography.As of now,a 25 nm half-pitch pattern has been obtained;and a cm2 exposure area has been achieved in practical samples.The above methods have been applied to extreme ultraviolet photoresist evaluation,photonic crystal and surface plasmonic effect research,and so on. | Jun Zhao Shumin Yang Chaofan Xue Liansheng Wang Zhaofeng Liang Lei Zhang Yong Wang Yanqing Wu Renzhong Tai | 2020 | International Journal of Extreme Manufacturing2020，2，1： | 2 |
| 2 | Effects of iron precursors on the structure and catalytic performance of iron molybdate prepared by mechanochemical route for methanol to formaldehyde显示文摘Mechanochemical synthesis has been applied for many novel material preparations and gained more and more attention due to green and high-efficiency recently. In order to explore the influences of iron precursors on structure and performance of iron molybdate catalyst prepared by mechanochemical route, three typical and cheap iron precursors have been used in preparation of iron molybdate catalyst. Many characterization methods have been employed to obtain the physical and chemical properties of iron molybdate catalyst. Results indicate that iron precursors have the significant impact on the phase composition, crystal morphology and catalytic performance in the conversion of methanol to formaldehyde. It is hard to regulate the phase composition by changing Mo/Fe mole ratios for Fe2(SO4)3 as iron precursor. In addition, as for Fe2(SO4)3, the formaldehyde yield is lower than that from iron molybdate catalyst prepared with Fe(NO3)3·9H2O due to the reduction in Fe2(MoO4)3 phase as active phase. Based on mechanochemical and coprecipitation method, the solvent water could be a key factor for the formation of MoO3 and Fe2(MoO4) for FeCl3·6H2O and Fe2(SO4)3 as precursors. Iron molybdate catalyst prepared with Fe(NO3)3·9H2O by mechanochemical route, shows the best methanol conversion and formaldehyde yield in this reaction. | Lingtao Kong Shengtao Xu Xue Liu Chaofan Liu Dandan Zhang Ling Zhao | 2020 | Chinese Journal of Chemical Engineering2020，28，6： | 1 |
| 3 | Revealing the role of microalgae-bacteria niche for boosting wastewater treatment and energy reclamation in response to temperature显示文摘Conventional biological treatment usually cannot achieve the same high water quality as advanced treatment when conducted under varied temperatures.Here,satisfactory wastewater treatment efficiency was observed in a microalgae-bacteria consortia(MBC)over a wide temperature range because of the predominance of microalgae.Microalgae contributed more toward wastewater treatment at low temperature because of the unsatisfactory performance of the accompanying bacteria,which experienced cold stress(e.g.,bacterial abundance below 3000 sequences)and executed defensive strategies(e.g.,enrichment of cold-shock proteins).A low abundance of amoA-C and hao indicated that conventional nitrogen removal was replaced through the involvement of microalgae.Diverse heterotrophic bacteria for nitrogen removal were identified at medium and high temperatures,implying this microbial niche treatment contained diverse flexible consortia with temperature variation.Additionally,pathogenic bacteria were eliminated through microalgal photosynthesis.After fitting the neutral community model and calculating the ecological niche,microalgae achieved a maximum niche breadth of 5.21 and the lowest niche overlap of 0.38,while the accompanying bacterial community in the consortia were shaped through deterministic processes.Finally,the maximum energy yield of 87.4 kJ L^(-1)and lipid production of 1.9 g L^(-1)were achieved at medium temperature.Altogether,this study demonstrates that advanced treatment and energy reclamation can be achieved through microalgae-bacteria niche strategies. | Chaofan Zhang Xi Chen Meina Han Xue Li Haixing Chang Nanqi Ren Shih-Hsin Ho | 2023 | Environmental Science and Ecotechnology2023，，2： | 0 |
| 4 | Modified iron-molybdate catalysts with various metal oxides by a mechanochemical method:enhanced formaldehyde yield in methanol partial oxidation显示文摘A mechanochemical method was employed to prepare modified iron molybdate catalysts with various metal salts as precursors.The physicochemical properties of the iron molybdate catalysts were characterized,and their performances in catalyzing the reaction from methanol to formaldehyde(HCHO)were evaluated.Iron molybdate catalysts doped with Co(NO_(3))_(2)·6H_(2)Oand Al(NO_(3))_(3)·9H_(2)O resulted in high HCHO yields.Compared with a commercial catalyst,the HCHO yields in the reaction with the modified catalyst at an optimal Co/Mo molar ratio reached 97.37%.According to chemical state analysis,the formation of CoO and the efficient decrease in the MoO_(3)sublimation rate could be important factors enhancing the HCHO yield in reactions catalyzed with iron molybdate doped with different Co/Mo mole ratios. | Xue Liu Lingtao Kong Shengtao Xu Chaofan Liu Fengyun Ma | 2021 | Frontiers of Chemical Science and Engineering2021，15，5： | 0 |
| 5 | Multistage defense response of microalgae exposed to pharmaceuticals in wastewater显示文摘Recently, the use of microalgae for bioremediation of pharmaceuticals(Ph As) has attracted increasing interest. However, most studies focused more on microalgae removal performance, its defensive response to the Ph As during wastewater treatment remains unexplored. Herein, microalgal three defensive systems have been investigated in synthetic wastewater, with six Ph As as the typical drug. Results show that Ph As could bind to EPS, and this action in turn could help to alleviate the direct toxicity of Ph As to microalgae. Subsequently, the physiological analyses revealed the increase of superoxide dismutase(SOD), catalase(CAT), and peroxidase(POD) activities, potentially reducing the oxidative stress induced by Ph As. Furthermore, the enzyme activities of cytochrome P450(CYP450) and glutathione-S-transferase(GST) were significantly upregulated after exposure to SMX, CIP and BPA, followed by a significant decrease in biodegradation rates after the addition of CYP450 inhibitors, suggesting that the biotransformation and detoxification of Ph As occurred. Meanwhile, molecular docking further revealed that CYP450 could bind with Ph As via hydrogen bond and hydrophobic interaction, which proved their abilities to be metabolized and form transformation products in microalgae. These findings provide an advancing understanding of microalgae technologies to improve the treatment of wastewater contaminated with Ph As. | Yuhao Chu Chaofan Zhang Xi Chen Xue Li Nanqi Ren Shih-Hsin Ho | 2023 | Chinese Chemical Letters2023，34，4： | 0 |
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