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| 1 | Unlocking the door to highly efficient Ag-based nanoparticles catalysts for NaBH4-assisted nitrophenol reduction显示文摘Ag-based nano particles(NPs)catalysts have recently attracted in creasi ng atte ntion in NaBH4-assisted n itrophe nol reducti on,especially in 4?n itrophe nol(4?NP)reducti on.Moreover,Ag-based NPs catalysts are con sidered to be very promising for practical applicati ons because of their fascinating advantages,e.g.,easy preparation,relatively low cost and less toxicity,high activity and good stability.Basically,the size and shape of Ag NPs are well known as the key factors for achieving highly efficient catalytic reduction of 4-NP.In this review,three highly efficient Ag-based NPs catalysts(supported Ag NPs,anisotropic Ag NPs and bimetallic Ag NPs)are highlighted for the 4-NP reduction,in eluding the catalytic mecha nism and reactio n rate caused by their adjustments in size and shape.Although high catalytic activity has bee n demonstrated by several Ag-based NPs catalysts,further improvement in the catalytic performance is still desired.In terms of the most recent progress in Ag-based NPs catalysts for 4?NP reduction,this review provides a comprehensive assessment on the material selection,synthesis and catalytic characterizations of these catalysts.Moreover,this review aims to correlate the catalytic performance of Ag-based NPs catalysts with their size and shape,guiding the development of novel cost-effective and high-performance catalysts. | Guangfu Liao Yan Gong Liu Zhong Jiasheng Fang Li Zhang Zushun Xu Haiyang Gao Baizeng Fang | 2019 | Nano Research2019，12，10： | 9 |
| 2 | SARS-CoV-2 spike protein receptor-binding domain perturbates intracellular calcium homeostasis and impairs pulmonary vascular endothelial cells显示文摘Exposure to the spike protein or receptor-binding domain(S-RBD)of SARS-CoV-2 significantly influences endothelial cells and induces pulmonary vascular endotheliopathy.In this study,angiotensin-converting enzyme 2 humanized inbred(hACE2 Tg)mice and cultured pulmonary vascular endothelial cells were used to investigate how spike protein/S-RBD impacts pulmonary vascular endothelium.Results show that S-RBD leads to acute-to-prolonged induction of the intracellular free calcium concentration([Ca^(2+)]i)via acute activation of TRPV4,and prolonged upregulation of mechanosensitive channel Piezo1 and store-operated calcium channel(SOCC)key component Orai1 in cultured human pulmonary arterial endothelial cells(PAECs).In mechanism,S-RBD interacts with ACE2 to induce formation of clusters involving Orai1,Piezo1 and TRPC1,facilitate the channel activation of Piezo1 and SOCC,and lead to elevated apoptosis.These effects are blocked by Kobophenol A,which inhibits the binding between S-RBD and ACE2,or intracellular calcium chelator,BAPTA-AM.Blockade of Piezo1 and SOCC by GsMTx4 effectively protects the S-RBDinduced pulmonary microvascular endothelial damage in hACE2 Tg mice via normalizing the elevated[Ca^(2+)]i.Comparing to prototypic strain,Omicron variants(BA.5.2 and XBB)of S-RBD induces significantly less severe cell apoptosis.Transcriptomic analysis indicates that prototypic S-RBD confers more severe acute impacts than Delta or Lambda S-RBD.In summary,this study provides compelling evidence that S-RBD could induce persistent pulmonary vascular endothelial damage by binding to ACE2 and triggering[Ca^(2+)]i through upregulation of Piezo1 and Orai1.Targeted inhibition of ACE2-Piezo1/SOCC-[Ca^(2+)]i axis proves a powerful strategy to treat S-RBD-induced pulmonary vascular diseases. | Kai Yang Shiyun Liu Han Yan Wenju Lu Xiaoqian Shan Haixia Chen Changlei Bao Huazhuo Feng Jing Liao Shuxin Liang Lei Xu Haiyang Tang Jason X-J.Yuan Nanshan Zhong Jian Wang | 2023 | Signal Transduction and Targeted Therapy2023，8，8： | 2 |
| 3 | Comparative proteomic analysis of plasma from bipolar depression and depressive disorder: identification of proteins associated with immune regulatory显示文摘 | Jin Chen (1) (2) (3) ChengLong Huang (2) (3) (5) YiRen Song (1) (2) (3) HaiYang Shi (1) (2) (3) Dong Wu (2) (3) (5) YongTao Yang (2) (3) (4) ChengLong Rao (2) (3) (7) Li Liao (2) (3) (5) You Wu (2) (3) (6) JianYong Tang (2) (3) (5) Ke Cheng (1) (2) (3) Jian Zhou (2) (3) Peng Xie (1) (2) (3) | 2015 | Protein & Cell2015，6，12： | 1 |
| 4 | Geochemistry of subducted metabasites exhumed from the Mariana forearc:Implications for Pacific seamount subduction显示文摘Seamounts on the drifting oceanic crust are inevitably carried by plate motions and eventually accreted or subducted.However,the geochemical signatures of the subducted seamounts and the significance of seamount subduction are not well constrained.Hundreds of seamounts have subducted beneath the Philippine Sea Plate following the westward subduction of the Pacific Plate since the Eocene(~52 Ma).The subducted oceanic crust and seamount materials can be exhumed from the mantle depth to the seafloor in the Mariana forearc region by serpentinite mud volcanoes,providing exceptional opportunities to directly study the subducted oceanic crust and seamounts.The International Ocean Discovery Program(IODP)expedition 366 has recovered a few metamorphosed mafic clasts exhumed from the Mariana forearc serpentinite mud volcanoes,e.g.,the Fantangis?a and Asùt Tesoru seamounts.These mafic clasts have tholeiitic to alkaline affinities with distinct trace elements and Nd-Hf isotopes characteristics,suggesting different provenances and mantle sources.The tholeiites from the Fantangisna Seamount have trace element characteristics typical of mid-ocean ridge basalt.The Pacific-type Hf-Nd isotopic compositions,combined with the greenschist metamorphism of these tholeiites further suggest that they came from the subducted Pacific oceanic crust.The alkali basalts-dolerites from the Fantangisna and Asùt Tesoru seamounts show ocean island basalt(OIB)-like geochemical characteristics.The OIB-like geochemical signatures and the low-grade metamorphism of these alkali basalts-dolerites suggest they came from subducted seamounts that originally formed in an intraplate setting on the Pacific Plate.The Pacific Plate origin of these metabasites suggests they were formed in the Early Cretaceous or earlier.Two types of OIBs have been recognized from alkali metabasites,one of which is geochemically similar to the HIMU-EMI-type OIBs from the West Pacific Seamount Province,and another is similar to the EMII-type OIBs from the Samoa Island in southern Pacific,with negative Nb-Ta-Ti anomalies and enriched Nd-Hf isotopes.Generally,these alkali metabasites are sourced from the heterogeneous mantle sources that are similar to the present South Pacific Isotopic and Thermal Anomaly.This study provides direct evidence for seamount subduction in the Mariana convergent margins.We suggest seamount subduction is significant to element cycling,mantle heterogeneity,and mantle oxidation in subduction zones. | Jianghong Deng Lipeng Zhang He Liu Haiyang Liu Renqiang Liao Abdul Shakoor Mastoi Xiaoyong Yang Weidong Sun | 2021 | Geoscience Frontiers2021，12，3： | 1 |
| 5 | An intrinsically self-healing and anti-freezing molecular chains induced polyacrylamide-based hydrogel electrolytes for zinc manganese dioxide batteries显示文摘The anti-freezing strategy of hydrogels and their self-healing structure are often contradictory,it is vital to break through the molecular structure to design and construct hydrogels with intrinsic anti-freezing/self-healing for meeting the rapid development of flexible and wearable devices in diverse service conditions.Herein,we design a new hydrogel electrolyte(AF/SH-Hydrogel)with intrinsic anti-freezing/self-healing capabilities by introducing ethylene glycol molecules,dynamic chemical bonding(disulfide bond),and supramolecular interaction(multi-hydrogen bond)into the polyacrylamide molecular chain.Thanks to the exceptional freeze resistance(84%capacity retention at-20℃)and intrinsic self-healing capabilities(95%capacity retention after 5 cutting/self-healing cycles),the obtained AF/SH-Hydrogel makes the zinc||manganese dioxide cell an economically feasible battery for the state-of-the-art applications.The Zn||AF/SH-Hydrogel||MnO_(2)device offers a near-theoretical specific capacity of 285 m A h g^(-1)at 0.1 A g^(-1)(Coulombic efficiency≈100%),as well as good self-healing capability and mechanical flexibility in an ice bath.This work provides insight that can be utilized to develop multifunctional hydrogel electrolytes for application in next generation of self-healable and freeze-resistance smart aqueous energy storage devices. | Haiyang Liao Wenzhao Zhong Chen Li Jieling Han Xiao Sun Xinhui Xia Ting Li Abolhassan Noori Mir F.Mousavi Xin Liu Yongqi Zhang | 2024 | Journal of Energy Chemistry2024，89，2： | 0 |
| 6 | Bifunctional electrolyte regulation towards low-temperature and high-stability Zn-ion hybrid capacitor显示文摘Aqueous Zinc-based energy storage devices are considered as one of the potential candidates in future power technologies.Nevertheless,poor low temperature performance and uncontrollable Zn dendrite growth lead to the limited energy storage capability.Herein,an anti-hydrolysis,cold-resistant,economical,safe,and environmentally friendly electrolyte is developed by utilizing water,ethylene glycol(EG),and ZnCl_(2)with high ionic conductivity(7.9 mS cm^(-1)in glass fiber membrane at-20℃).The spectra data and DFT calculations show the competitive coordination of EG and Cl-to induce a unique solvation configuration of Zn^(2+),conducive to effectively inhibiting the hydrolysis of Zn^(2+),suppressing the dendrite growth,and broadening the working voltage range and temperature range of ZnCl_(2)electrolyte.The isotope tracing data confirm that Cl^(-)could effectively destroy the ZnO passivation film,promoting the formation of Zn nuclei and improving its reaction activity.Compared to the corresponding ZnSO4electrolyte,the Cu/Zn half-cell with the ZnCl_(2)electrolyte exhibits a stable cycle life of more than 1600 h at-20℃,even at the current density of 5 mA cm^(-2).The assembled Zn-ion hybrid capacitor possesses an average capacity of 42.68 m A h g^(-1)under-20℃at a current density of 5 A g^(-1),3.5 times than that of the modified ZnSO4electrolyte.Our work proposes a new approach for optimizing aqueous electrolytes to meet low temperature energy storage applications. | Shuo Yang Kui Xue Haiyang Liao Yuning Guo Liujiang Zhou Yongqi Zhang | 2023 | Journal of Energy Chemistry2023，，4： | 0 |
| 7 | Characteristics of distribution and migration of mercury in the sediment-water interface of Poyang Lake, China显示文摘 | Tianlong DENG Mengxia LIAO Haiyang YU Yi WU | 2006 | Chinese Journal Of Geochemistry2006，25，B08： | 0 |
| 8 | Transient synthesis of carbon-supported high-entropy alloy sulfide nanoparticles via flash Joule heating for efficient electrocatalytic hydrogen evolution显示文摘High entropy alloys(HEA)are frequently employed as catalysts in electrocatalytic hydrogen evolution.However,the traditional high entropy alloy synthesis methods are time-consuming,energy-intensive,and environmentally polluting,which limits their application in the hydrogen evolution reaction(HER).This study leveraged the capabilities of flash Joule heating(FJH)to synthesize carbon-supported high-entropy alloy sulfide nanoparticles(CC-S-HEA)on carbon cloth(CC)with good self-standing properties within 300 ms.The carbon thermal shock generated by the Joule heating could pyrolyze the sulfur source into gas,resulting in numerous pore structures and defects on CC,forming an S-doped carbon substrate(CC-S).Then the S atoms were used to stably anchor the metal atoms on CC-S to form high-density uniformly dispersed HEA particles.The electrochemical test results demonstrated that CC-S-HEA prepared at 60 V flash voltage had HER performance comparable to Pt/C.The density functional theory(DFT)calculation indicated that the S atoms on CC-S accelerated the electron transfer between the carbon substrate and HEA particles.Moreover,the unique electronic structure of CC-S-HEA was beneficial to H*adsorption and promoted catalytic kinetics.The simplicity and versatility of FJH synthesis are of great significance for optimizing the synthesis of HEA and improving the quality of HEA products,which provides a broad application prospect for the synthesis of nanocatalysts with efficient HER performance. | Yuntian Liao Rongtao Zhu Wenjun Zhang Haiyang Zhu Yang Sun Jiale Chen Zhenhua Dong Ronghuan Lv | 2024 | Nano Research2024，17，4： | 0 |
| 9 | Improvement on the topological localized interface enabled by chiral symmetry显示文摘Zero-energy topological states,which are protected by chiral symmetry against certain perturbations topologically,localize at interfaces between trivial and non-trivial phases in the Su–Schrieffer–Heeger(SSH)chain model.Here,we propose and demonstrate a method to manipulate chiral symmetry itself to improve the localized interfaces and enlarge the mode volume of topological states in the SSH model,thus optimizing the lasing performance of localized interfaces.As multiple defects corresponding to off-diagonal perturbations in an eigenmatrix are introduced,the topological state expands and extends to extra defects at the topological interface without breaking chiral symmetry.We apply the proposed method in electrical pumping semiconductor laser arrays to verify our theoretical prediction and optimize the output characteristics of the devices.The measured results of the proposed multi-defect SSH laser array show that the output power has been increased by 27%,and the series resistance and far-field divergence have been reduced by half compared to the traditional SSH laser array,establishing a high-performance light source for integrated silicon photonics,infrared light detection and ranging,and so on.Our work demonstrates that the proposed method is capable of improving topological localized interfaces and redistributing zero-energy topological states.Furthermore,our method can be applied to other platforms and inspire optimizations of more devices in broader areas. | JINGXUAN CHEN MINGJIN WANG TING FU YUFEI WANG XUEYOU WANG YINGQIU DAI ZIYUAN LIAO HAIYANG JI WANHUA ZHENG | 2023 | Photonics Research2023，11，9： | 0 |
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