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| 1 | A sensing mechanism for the detection of carbon nanotubes using selective photoluminescent probes based on ionic complexes with organic dyes显示文摘The multifunctional properties of carbon nanotubes(CNTs)make them a powerful platform for unprecedented innovations in a variety of practical applications.As a result of the surging growth of nanotechnology,nanotubes present a potential problem as an environmental pollutant,and as such,an efficient method for their rapid detection must be established.Here,we propose a novel type of ionic sensor complex for detecting CNTs–an organic dye that responds sensitively and selectively to CNTs with a photoluminescent signal.The complexes are formed through Coulomb attractions between dye molecules with uncompensated charges and CNTs covered with an ionic surfactant in water.We demonstrate that the photoluminescent excitation of the dye can be transferred to the nanotubes,resulting in selective and strong amplification(up to a factor of 6)of the light emission from the excitonic levels of CNTs in the near-infrared spectral range,as experimentally observed via excitation-emission photoluminescence(PL)mapping.The chirality of the nanotubes and the type of ionic surfactant used to disperse the nanotubes both strongly affect the amplification;thus,the complexation provides sensing selectivity towards specific CNTs.Additionally,neither similar uncharged dyes nor CNTs covered with neutral surfactant form such complexes.As model organic molecules,we use a family of polymethine dyes with an easily tailorable molecular structure and,consequently,tunable absorbance and PL characteristics.This provides us with a versatile tool for the controllable photonic and electronic engineering of an efficient probe for CNT detection. | Petro Lutsyk Raz Arif Jan Hruby Anatolii Bukivskyi Olexander Vinijchuk Mykola Shandura Viktor Yakubovskyi Yuri Kovtun Graham A Rance Michael Fay Yuri Piryatinski Oleksiy Kachkovsky Anatoli Verbitsky Aleksey Rozhin | 2016 | Light(Science & Applications)2016，5，1： | 2 |
| 2 | Functional analysis of oxidative stress-activated mitogen-activated protein kinase cascade in plants显示文摘 | KOVTUN Y CHIU W L TENA Q SHEEN J | 2000 | Proceedings of the National Academy of Sciences USA2000，97，： | 1 |
| 3 | Role of ultraviolet irradiation and oxidative stress in cataract formation-medical prevention by nutritional antioxidants and metabolic agonists 显示文摘 | Varma SD Kovtun S Hegde KR | 2011 | Eye Contact Lens2011，37，4： | 1 |
| 4 | Comparison of all-inside meniscal re- pair devices with matched inside-out suture repair 显示文摘 | Rosso C Kovtun K Dow W | 2011 | Am J Spoas Med2011，39，12： | 1 |
| 5 | Attenuation and delay of diabetic cataracts by antioxidants: effectiveness of pyruvate after onset of cataract显示文摘 | Varma SD Hegde KR Kovtun S | 2005 | Ophthalmologica2005，219，5： | 1 |
| 6 | Functional analysis of oxidative stress-activated mitogen-activated protein kinases cascade in plants显示文摘 | KOVTUN Y CHIU W L TENA G | 2000 | Proceedings of the National Academy of Sciences USA2000，97，： | 1 |
| 7 | Treatment of habitual shoulder dislocation 显示文摘 | KOVTUN V V FADZHIEV M M | 2000 | Voen Med Zh2000，321，7： | 1 |
| 8 | Functional analysis of oxidative stress-activated mitogen-activated protein kinase cascade in plants显示文摘 | KOVTUN Y CHIU W L TENA G | 2000 | PNAS2000，97，： | 1 |
| 9 | Functional analysis of oxidative stress-activated mitogen-activated protein kinase cascade in plants 显示文摘 | KOVTUN Y CHIU W L TENA G | 2000 | Proc Natl Acad Sci USA2000，97，6： | 1 |
| 10 | Viscosity in strongly in- teracting quantum field theories from black hole physics显示文摘 | Kovtun P K Son D T Starinets A O | 2005 | Physical Review Letters2005，94，11： | 1 |
| 11 | Role of ultraviolet irradiation and oxidative stress in cataract formation-medical prevention by nutritional antioxidants and metabolic agonists显示文摘 | Varma SD Kovtun S Hegde KR | 2011 | Eye Contact Lens2011，37，4： | 1 |
| 12 | Welded structures of 01570 aluminium alloy显示文摘 | Malinkina T I Markachev N A Kovtun V A | 1998 | Welding International1998，12，7： | 1 |
| 13 | Inhibition of glycolysis in the retina by oxidative stress:prevention by pyruvate 显示文摘 | Hegde KR Kovtun S Varma SD | 2010 | Mol Cell Biochem2010，343，12： | 1 |
| 14 | Oxidative damage to lens in culture:reversibility by pyruvate and ethyl pyruvate显示文摘 | Varma SD Hegde KR Kovtun S | | 0，，01： | 1 |
| 15 | New method for preparing alkyl esters of chloroalkanoic acids 显示文摘 | Kovtun VY Kol'tsova ZM Yashunskii VG | 1978 | Zhurnal Prikladnoi Khimii1978，51，8： | 1 |
| 16 | Cholecystostomy in emergent surgery of hepatopancreatobiliary zone organs显示文摘 | Hanzhy VV Kovtun AS Kovals'ky PS | 2007 | Klin Khir2007，，7： | 1 |
| 17 | Suppression of Auxin Signal Transduction by a MAPK Cascade in Higher Plants 显示文摘 | KOVTUN Y CHIU W L ZENG W | 1998 | Nature1998，395，6703： | 1 |
| 18 | Assessing the value of demand sharing in supply chains 显示文摘 | Kovtun V Giloni A Hurvich C | 2014 | Naval Research Logistics2014，61，7： | 1 |
| 19 | Suppression of auxin signal transduction by a MAPK cascade in higher plants显示文摘 | KOVTUN Y CHIU W L ZENG W et ag | 1998 | Nature1998，395，： | 1 |
| 20 | Biocompatible quantum dots for biological applications显示文摘 | Rosenthal SJ Chang JC Kovtun O | | 0，，01： | 1 |
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