|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Abundance and Distribution of Fatty Acids in Sediments of the South Mid-Atlantic Ridge显示文摘Sediment samples obtained from the South Mid-Atlantic Ridge were studies by gas chromatography-mass spectrometer(GC-MS) for the abundance and distributions of total fatty acids(TFAs). Approximately 34 fatty acids were identified, with the chain-lengths ranging from C12 to C30. The total concentrations of TFAs(∑TFA) ranged from 7.15 to 30.09 μg g-1 dry sediment, and ∑TFA was weakly correlated with bitumen content(R2 = 0.69). The ∑TFA of samples around hydrothermal areas were significantly higher than that of samples away from hydrothermal areas, indicating intense primary production and large biomass in the hydrothermal areas, and suggesting a close relationship between hydrothermal activity and ∑TFA of samples. The characteristics of the TFA composition in the present study are rich in monounsaturated fatty acids and lacking in polyunsaturated fatty acids, and the ratios between the concentrations of monounsaturated fatty acids and ΣTFAs in samples close to the hydrothermal areas, are about 0.8, but for samples far from the hydrothermal areas, they are only about 0.5. Several fatty acids(e.g., a/i C15:0 and C16:1ω7), which are signature biomarkers for sulfur-metabolizing bacteria, show the same distribution trend as ∑TFA of samples, further highlighting the close relationship between fatty acid content and hydrothermal activity and/or hydrothermal communities. The metabolic activities of hydrothermal communities, especially those of microorganisms, are likely the main source of fatty acids in samples. | HUANG Xin ZENG Zhigang CHEN Shuai YIN Xuebo WANG Xiaoyuan MA Yao YANG Baoju RONG Kunbo SHU Yunchao JIANG Tao | 2015 | Journal of Ocean University of China2015，14，2： | 4 |
| 2 | Component characteristics of polycyclic aromatic compounds in sediments of the South Mid-Atlantic Ridge显示文摘10 samples of sediments obtained from the South Mid-Atlantic Ridge were measured for the abundances and distributions of polycyclic aromatic compounds(PAHs). The total concentrations of PAHs(∑PAHs) ranged from 2.768 to 9.826 μg/g dry sediment. The ∑PAHs was higher in sample 22V-TVG10 and sample 26V-TVG05 which were close to hydrothermal fields, with the lowest value in sample 22V-TVG14 which was farthest from hydrothermal fields, suggesting a probable hydrothermal origin of ∑PAHs of samples. Approximately nine kinds of PAHs were identified, and low molecular mass tricyclic and tetracyclic aromatic compounds were predominant in the samples. The concentrations of fluoranthene which were typical as hydrothermal alteration compounds were the highest among PAHs with dry weight between 0.913–3.157 μg/g. The phenanthrene homologue was most abundant in the samples, and the ratios between parent phenanthrene and methylphenanthrene which probably reflected the degree of hydrothermal alteration ranged from 0.097 to 1.602. The sample 22V-TVG10 possessing a maximum ratio value showed the intense influence of the hydrothermal alteration on this sample, which might further imply that PAHs in sediments were mainly derived from the hydrothermal alteration. | HUANG Xin ZENG Zhigang CHEN Shuai YIN Xuebo WANG Xiaoyuan MA Yao YANG Baoju RONG Kunbo SHU Yunchao JIANG Tao | 2014 | Acta Oceanologica Sinica2014，33，11： | 2 |
| 3 | Detailed modeling of aluminum particle combustion——From single particles to cloud combustion in Bunsen flames显示文摘A numerical model for aluminum cloud combustion which includes the effects of interphase heat transfer,phase change,heterogeneous surface reactions,homogeneous combustion,oxide cap growth and radiation within the Euler–Lagrange framework is proposed.The model is validated in single particle configurations with varying particle diameters.The combustion process of a single aluminum particle is analyzed in detail and the particle consumption rates as well as the heat release rates due to the various physical/chemical sub-models are presented.The combustion time of single aluminum particles predicted by the model are in very good agreement with empirical correlations for particles with diameters larger than 10μm.The prediction error for smaller particles is noticeably reduced when using a heat transfer model that is capable of capturing the transition regime between continuum mechanics and molecular dynamics.The predictive capabilities of the proposed model framework are further evaluated by simulating the aluminum/air Bunsen flames of Mc Gill University for the first time.Results show that the predicted temperature distribution of the flame is consistent with the experimental data and the double-front structure of the Bunsen flame is reproduced well.The burning rates of aluminum in both single particle and particle cloud configurations are calculated and compared with empirical correlations.Results show that the burning rates obtained from the present model are more reasonable,while the correlations,when embedded in the Euler–Lagrange context,tend to underestimate the burning rate in the combustion stage,particularly for the considered fuel-rich flames. | Jiarui ZHANG Oliver T.STEIN Tien D.LUU Ali SHAMOONI Zhixun XIA Zhenbing LUO Likun MA Yunchao FENG Andreas KRONENBURG | 2022 | Chinese Journal of Aeronautics2022，35，5： | 2 |
| 4 | One-pot synthesis of 2,5-bis(hydroxymethyl)furan from biomass derived 5-(chloromethyl)furfural in high yield显示文摘5-(Chloromethyl)furfural(CMF),as a new platform molecular,has become a hot topic in the field of biorefinery.Herein,the one-pot conversion of CMF to 2,5-bis(hydroxymethyl)furan(BHMF)in the water phase was demonstrated for the first time.A 91%BHMF yield was obtained over Ru/Cu Oxcatalyst,and BHMF was mainly produced by the consecutive hydrolysis and hydrogenation of CMF with 5-hydroxymethylfurfural(HMF)as an intermediate.Kinetic studies revealed that the conversion of HMF to BHMF was the rate-determining step.Remarkably,the characterizations and density functional theory(DFT)calculations further revealed the lower electron density of Ru NPs in Ru/Cu Oxcatalyst,resulting in a larger adsorption energy and a smaller free energy difference for the formation of alcohols.The present findings offered a new pathway for biomass-derived diol production through CMF as a potential source. | Binglin Chen Yunchao Feng Sen Ma Weizhen Xie Guihua Yan Zheng Li Jonathan Sperry Shuliang Yang Xing Tang Yong Sun Lu Lin Xianhai Zeng | 2023 | Journal of Energy Chemistry2023，，1： | 1 |
| 5 | Rapid fabrication of bonded diamond composite using the spark plasma sintering reaction synthesis method显示文摘 | Ma Yunchao Guo Jifeng Liang Baoyan | 2010 | Int J Refractory Metals Hard Mater2010，29，3： | 1 |
| 6 | Experimental exploration of five-qubit quantum error-correcting code with superconducting qubits显示文摘Quantum error correction is an essential ingredient for universal quantum computing.D espite tremendous experimental efforts in the study of quantum error correction,to date,there has been no demonstration in the realis ation of universal quantum error-correcting code,with the subsequent verification of all key features including the identification of an arbitrary physical error,the capability for transversal manipulation of the logical state and state decoding.To address this challenge,we experimentally realise the [5,1,3]code,the so-called smallest perfect code that permits corrections of generic single-qubit errors.In the experiment,having optimised the encoding circuit,we employ an array of superconducting qubits to realise the [5,1,3] code for several typical logical states including the magic state,an indispensable resource for realising non-Clifford gates.The encoded states are prepared with an average fidelity of 57.1(3)% while with a high fidelity of 98.6(1)% in the code space.Then,the arbitrary single-qubit errors introduced manually are identified by measuring the stabilisers.We further implement logical Pauli operations with a fidelity of 97.2(2)% within the code space.Finally,we realise the decoding circuit and recover the input state with an overall fidelity of 74.5(6)%,in total with 92 gates.Our work demonstrates each key aspect of the [5,1,3] code and verifies the viability of experimental realisation of quantum error-correcting codes with superconducting qubits. | Ming Gong Xiao Yuan Shiyu Wang Yulin Wu Youwei Zhao Chen Zha Shaowei Li Zhen Zhang Qi Zhao Yunchao Liu Futian Liang Jin Lin Yu Xu Hui Deng Hao Rong He Lu Simon C.Benjamin Cheng-Zhi Peng Xiongfeng Ma Yu-Ao Chen Xiaobo Zhu Jian-Wei Pan | 2022 | National Science Review2022，9，1： | 1 |
| 7 | AFExplorer:Visual analysis and interactive selection of audio features显示文摘Acoustic quality detection is vital in the manufactured products quality control field since it represents the conditions of machines or products.Recent work employed machine learning models in manufactured audio data to detect anomalous patterns.A major challenge is how to select applicable audio features to meliorate model’s accuracy and precision.To relax this challenge,we extract and analyze three audio feature types including Time Domain Feature,Frequency Domain Feature,and Cepstrum Feature to help identify the potential linear and non-linear relationships.In addition,we design a visual analysis system,namely AFExplorer,to assist data scientists in extracting audio features and selecting potential feature combinations.AFExplorer integrates four main views to present detailed distribution and relevance of the audio features,which helps users observe the impact of features visually in the feature selection.We perform the case study with AFExplore according to the ToyADMOS and MIMII Dataset to demonstrate the usability and effectiveness of the proposed system. | Lei Wang Guodao Sun Yunchao Wang Ji Ma Xiaomin Zhao Ronghua Liang | 2022 | Visual Informatics2022，6，1： | 1 |
| 8 | Effect of carbon dioxide concentration on the combustion characteristics of boron agglomerates in oxygen-containing atmospheres显示文摘In ramjet combustion chambers,carbon dioxide(CO_(2))produced by the combustion of carbonaceous fuel enters the chamber together with boron agglomerates.In order to investigate the effect of CO_(2)concentration present in an oxygen-containing atmosphere on the combustion characteristics and oxidation mechanisms of boron agglomerates,we used a laser ignition system,an X-ray diffractometer(XRD),and a thermogravimetric-differential scanning calorimetry(TG-DSC)combined thermal analysis system.Single-particle boron was tested in the laser-ignition experiments as the control group.The ignition experiment results showed that with a fixed O2 concentration of 20%,when the particle temperature reaches the melting point of boron,increasing CO_(2)content causes the combustion process of boron agglomerates to transition from single-particle molten droplet combustion to porous-particle combustion.Furthermore,XRD analysis results indicated that the condensed-phase combustion products(CCPs)of boron particles in a mixed atmosphere of O2 and CO_(2)contained B4C,which is responsible for the porous structure of the particles.At temperatures below 1200℃,the addition of CO_(2)has no obvious promotion effect on boron exothermic reaction.However,in the laser-ignition experiment,when the oxygen concentration was fixed at 20%while the CO_(2)concentration increased from 0%to 80%,the maximum temperature of boron agglomerates rose from 2434 to 2573 K,the self-sustaining combustion time of single-particle boron decreased from 396 to 169 ms,and the self-sustaining combustion time of boron agglomerates decreased from 198 to 40 ms.This study conclusively showed that adding CO_(2)to an oxygen-containing atmosphere facilitates boron reaction and consumption pathways,which is beneficial to promoting exothermic reaction of boron agglomerates at relatively high temperatures. | Lian DUAN Zhixun XIA Yunchao FENG Binbin CHEN Jiarui ZHANG Likun MA | 2023 | Journal of Zhejiang University-Science A(Applied Physics & Engineering)2023，24，11： | 0 |
| 9 | A Nitrogen, Sulfur co-Doped Porphyrin-based Covalent Organic Framework as an Efficient Catalyst for Oxygen Reduction显示文摘Oxygen reduction reaction(ORR) is a significant reaction for energy conversion systems(such as fuel cells, metal-air batteries, etc.). It is an urgent need to develop cheap, durable and highly-active catalysts for efficient ORR. Hence, we report a metal-free nitrogen and sulfur co-doped porphyrin-based covalent organic framework(COF) as a high-efficiency ORR catalyst[the onset potential(Eo) is 0.79 V and the half-wave potential(E1/2) is 0.70 V]. The double doping of N and S atoms causes uneven charge distribution around carbon atoms, which can act as catalytic active centers, improving ORR activity. Compared with single-atom doping, double atoms doping exhibits a higher activity due to the synergistic effect between different elements. These results demonstrate that reasonable design of stable metal-free COFs with a high electrochemical activity can promote their wide applications. | YU Xiaoming MA Yunchao LI Cuiyan GUAN Xinyu FANG Qianrong QIU Shilun | 2022 | Chemical Research in Chinese Universities2022，38，1： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员