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| 1 | Aerosol and boundary-layer interactions and impact on air quality显示文摘Air quality is concerned with pollutants in both the gas phase and solid or liquid phases. The latter are referred to as aerosols, which are multifaceted agents affecting air quality, weather and climate through many mechanisms. Unlike gas pollutants, aerosols interact strongly with meteorological variables with the strongest interactions taking place in the planetary boundary layer(PBL). The PBL hosting the bulk of aerosols in the lower atmosphere is affected by aerosol radiative effects. Both aerosol scattering and absorption reduce the amount of solar radiation reaching the ground and thus reduce the sensible heat fluxes that drive the diurnal evolution of the PBL. Moreover, aerosols can increase atmospheric stability by inducing a temperature inversion as a result of both scattering and absorption of solar radiation, which suppresses dispersion of pollutants and leads to further increases in aerosol concentration in the lower PBL.Such positive feedback is especially strong during severe pollution events. Knowledge of the PBL is thus crucial for understanding the interactions between air pollution and meteorology. A key question is how the diurnal evolution of the PBL interacts with aerosols, especially in vertical directions, and affects air quality.We review the major advances in aerosol measurements, PBL processes and their interactions with each other through complex feedback mechanisms, and highlight the priorities for future studies. | Zhanqing Li Jianping Guo Aijun Ding Hong Liao Jianjun Liu Yele Sun Tijian Wang Huiwen Xue Hongsheng Zhang Bin Zhu | 2017 | National Science Review2017，4，6： | 37 |
| 2 | Influence of Atmospheric Particulate Matter on Ozone in Nanjing,China:Observational Study and Mechanistic Analysis显示文摘Particulate matter with diameters of 2.5 μm or smaller(PM_(2.5)) and ozone(O_3) are major pollutants in the urban atmosphere. PM_(2.5) can affect O_3 by altering the photolysis rate and heterogeneous reactions. However, these two processes and their relative importance remain uncertain. In this paper, with Nanjing in China as the target city, we investigate the characteristics and mechanism of interactions between particles and O_3 based on ground observations and numerical modeling.In 2008, the average concentrations of PM_(2.5) and O_3 at Caochangmen station are 64.6 ± 47.4 μg m^(-3) and 24.6 ± 22.8 ppb,respectively, while at Pukou station they are 94.1 ± 63.4 μg m^(-3) and 16.9 ± 14.9 ppb. The correlation coefficient between PM_(2.5) and O_3 is -0.46. In order to understand the reaction between PM_(2.5) and O_3, we construct a box model, in which an aerosol optical property model, ultraviolet radiation model, gas phase chemistry model, and heterogeneous chemistry model,are coupled. The model is employed to investigate the relative contribution of the aforementioned two processes, which vary under different particle concentrations, scattering capability and VOCs/NOxratios(VOCs: volatile organic compounds;NOx: nitric oxide and nitrogen dioxide). Generally, photolysis rate effect can cause a greater O_3 reduction when the particle concentrations are higher, while heterogeneous reactions dominate O_3 reduction with low-level particle concentrations.Moreover, in typical VOC-sensitive regions, O_3 can even be increased by heterogeneous reactions. In Nanjing, both processes lead to O_3 reduction, and photolysis rate effect is dominant. Our study underscores the importance of photolysis rate effect and heterogeneous reactions for O_3, and such interaction processes should be fully considered in future atmospheric chemistry modeling. | Yawei QU Tijian WANG Yanfeng CAI Shekou WANG Pulong CHEN Shu LI Mengmeng LI Cheng YUAN Jing WANG Shaocai XU | 2018 | Advances in Atmospheric Sciences2018，35，11： | 33 |
| 3 | Methane emissions from terrestrial plants over China and their effects on methane concentrations in lower troposphere显示文摘Methane (CH4) is the most important greenhouse gas and reactive trace gas in the atmosphere. Recently, it has been reported that terrestrial plants can emit CH4 under aerobic conditions, which may call for reevaluation of the inventory of CH4 emissions in China. In this paper, those emissions over China and their effects on CH4 concentrations in lower troposphere were investigated. Firstly, based on the work of Keppler et al., the aerobic plant CH4 emission model (PLANTCH4) for China was established. And by using the database of normalized difference vegetation index (NDVI) derived from NOAA/ AVHRR, the distribution of net primary productivity (NPP) over China was simulated, and thereby, for the first time, the amount and distribution of the newly identified source in China were estimated. Secondly, with the aid of the three-dimensional atmospheric chemistry model system (MM5-CALGRID), the effects of the emissions were studied. The results show that the annual aerobic plant CH4 emissions over China amount to 11.83 Tg, i.e. nearly 24% of Chinese total CH4 emissions. And the major fraction (about 43%) comes from forests. When those emissions are considered in modeling, computed countrywide mean surface concentration of CH4 is 29.9% higher than without them, with a maximum increase of 69.61 μg·m-3 in the south of Yunnan Province. In conclusion, to study CH4 emissions from terrestrial plants over China may have important implications for correctly estimating the contribution of China to global CH4 budget, and may call for a reconsideration of the role of CH4 in global and regional environment and climate change. | XIE Min LI Shu JIANG Fei WANG TiJian | 2009 | Chinese Science Bulletin2009，54，2： | 6 |
| 4 | INVESTIGATIONS OF MAIN FACTORS AFFECTING TROPOSPHERIC NITRATE AEROSOL USING A COUPLING MODEL显示文摘Factors affecting tropospheric nitrate aerosol formation were investigated through a number of sensitivity studies using the thermodynamic equilibrium model ISORROPIA and the condensed gas-phase chemistry model. Re-sults indicate that the equilibrium concentration of nitrate aerosol varies with solar zenith angle, air temperature, relative humidity, initial SO2 concentration, initial NO2 concentration and initial NH3 concentration. NH3 concentration and solar zenith angle play the most important roles, followed by relative humidity and NO2 concentration. It seems that the rela-tions between nitrate aerosol and these four factors, as well as air temperature, are strong and highly nonlinear due to the coupling effect. The influence of SO2 concentration on nitrate aerosol is near-linear and weak. | Tijian Wang Shu Li Fei Jiang Lijie Gao | 2006 | China Particuology2006，4，6： | 5 |
| 5 | Review of Chinese atmospheric science research over the past 70 years: Atmospheric physics and atmospheric environment显示文摘Since the founding of the People’s Republic of China 70 years ago,the subject of atmospheric physics and atmospheric environment has developed rapidly in China,providing important support for the development of atmospheric science and guarantee for the development of national economy.In this paper,the general advancement of atmospheric physics and atmospheric environment in last 70 years was described.The main research progress of atmospheric physics and atmospheric environment in the past 40 years of reform and opening-up was reviewed,the outstanding research achievements since the 21 st century were summarized,the major problems and challenges are pointed out,and the key directions and suggestions for future development are put forward. | Tijian WANG Taichang GAO Hongsheng ZHANG Maofa GE Hengchi LEI Peichang ZHANG Peng ZHANG Chunsong LU Chao LIU Hua ZHANG Qiang ZHANG Hong LIAO Haidong KAN Zhaozhong FENG Yijun ZHANG Xiushu QIE Xuhui CAI Mengmeng LI Lei LIU Shengrui TONG | 2019 | Science China Earth Sciences2019，62，12： | 5 |
| 6 | Dynamic impact experiment and response characteristics analysis for 1:2 reduced-scale model of hydraulic support显示文摘It is significant to research the impact resistance properties of hydraulic support due to its key support role in the fully mechanized mining face.However,it is difficult for the entire hydraulic support to implement the impact experiment underground and analyze the response characteristic.Therefore,a dynamic impact experiment for the entire hydraulic support was proposed in this paper,where a 1:2 reducedscale model of hydraulic support was designed and its response characteristics under dynamic impact load were analyzed.Firstly,a comprehensive monitoring scheme was proposed to achieve an effective monitoring for dynamic response of hydraulic support.Secondly,a multi-scale impact experiment was carried out for the entire hydraulic support and dynamic behaviors of hydraulic support under the multi-scale impact load were revealed by experimental data.Then a dynamic impact experiment of the entire hydraulic support was simulated in ADAMS with the same experiment conditions,and the experimental and simulation data were verified mutually.Finally,the characteristics of energy conversion and dissipation of the entire experiment system after impact were analyzed.The experiment results showed that the impact resistance properties of hydraulic support largely depended on the initial support conditions and different vertical rigidities affected energy distribution proportion of the entire support system. | Huaiwei Ren Desheng Zhang Shixin Gong Kai Zhou Chenyang Xi Ming He Tijian Li | 2021 | International Journal of Mining Science and Technology2021，31，3： | 5 |
| 7 | Modeling heterogeneous chemical processes on aerosol surface显示文摘To explore the possible impact of heterogeneous chemical processes on atmospheric trace components,a coupled box model including gas-phase chemical processes,aerosol thermodynamic equilibrium processes,and heterogeneous chemical processes on the surface of dust,black carbon(BC) and sea salt is set up to simulate the effects of heterogeneous chemistry on the aerosol surface,and analyze the primary factors affecting the heterogeneous processes.Results indicate that heterogeneous chemical processes on the aerosol surface in the atmosphere will affect the concentrations of trace gases such as H2O2,HO2,O3,NO2,NO3,HNO3 and SO2,and aerosols such as SO42-,NO3- and NH4+.Sensitivity tests suggest that the magnitude of the impact of heterogeneous processes strongly depends on aerosol concentration and the surface uptake coefficients used in the box model.However,the impact of temperature on heterogeneous chemical processes is considerably less.The 'renoxification' of HNO3 will affect the components of the troposphere such as nitrogen oxide and ozone. | Junjun Deng Tijian Wang Li Liu Fei Jiang | 2010 | Particuology2010，8，4： | 4 |
| 8 | Impact of Tropospheric Ozone on Summer Climate in China显示文摘The spatial distribution, radiative forcing, and climatic effects of tropospheric ozone in China during summer were investigated by using the regional climate model Reg CM4. The results revealed that the tropospheric ozone column concentration was high in East China, Central China, North China, and the Sichuan basin during summer. The increase in tropospheric ozone levels since the industrialization era produced clear-sky shortwave and clear-sky longwave radiative forcing of 0.18 and 0.71 W m^(–2), respectively, which increased the average surface air temperature by 0.06 K and the average precipitation by 0.22 mm day^(–1) over eastern China during summer. In addition, tropospheric ozone increased the land–sea thermal contrast, leading to an enhancement of East Asian summer monsoon circulation over southern China and a weakening over northern China. The notable increase in surface air temperature in northwestern China, East China, and North China could be attributed to the absorption of longwave radiation by ozone, negative cloud amount anomaly, and corresponding positive shortwave radiation anomaly. There was a substantial increase in precipitation in the middle and lower reaches of the Yangtze River. It was related to the enhanced upward motion and the increased water vapor brought by strengthened southerly winds in the lower troposphere. | Shu LI Tijian WANG Prodromos ZANIS Dimitris MELAS Bingliang ZHUANG | 2018 | Journal of Meteorological Research2018，32，2： | 3 |
| 9 | Phase-matching-induced near-chirp-free solitons in normal-dispersion fiber lasers显示文摘Direct generation of chirp-free solitons without external compression in normal-dispersion fiber lasers is a long-term challenge in ultrafast optics.We demonstrate near-chirp-free solitons with distinct spectral sidebands in normaldispersion hybrid-structure fiber lasers containing a few meters of polarization-maintaining fiber.The bandwidth and duration of the typical mode-locked pulse are 0.74 nm and 1.95 ps,respectively,giving the time-bandwidth product of 0.41 and confirming the near-chirp-free property.Numerical results and theoretical analyses fully reproduce and interpret the experimental observations,and show that the fiber birefringence,normal-dispersion,and nonlinear effect follow a phase-matching principle,enabling the formation of the near-chirp-free soliton.Specifically,the phasematching effect confines the spectrum broadened by self-phase modulation and the saturable absorption effect slims the pulse stretched by normal dispersion.Such pulse is termed as birefringence-managed soliton because its two orthogonal-polarized components propagate in an unsymmetrical“X”manner inside the polarization-maintaining fiber,partially compensating the group delay difference induced by the chromatic dispersion and resulting in the selfconsistent evolution.The property and formation mechanism of birefringence-managed soliton fundamentally differ from other types of pulses in mode-locked fiber lasers,which will open new research branches in laser physics,soliton mathematics,and their related applications. | Dong Mao Zhiwen He Yusong Zhang Yueqing Du Chao Zeng Ling Yun Zhichao Luo Tijian Li Zhipei Sun Jianlin Zhao | 2022 | Light(Science & Applications)2022，11，2： | 3 |
| 10 | Recent Progress in Atmospheric Chemistry Research in China: Establishing a Theoretical Framework for the “Air Pollution Complex”显示文摘Atmospheric chemistry research has been growing rapidly in China in the last 25 years since the concept of the“air pollution complex”was first proposed by Professor Xiaoyan TANG in 1997.For papers published in 2021 on air pollution(only papers included in the Web of Science Core Collection database were considered),more than 24000 papers were authored or co-authored by scientists working in China.In this paper,we review a limited number of representative and significant studies on atmospheric chemistry in China in the last few years,including studies on(1)sources and emission inventories,(2)atmospheric chemical processes,(3)interactions of air pollution with meteorology,weather and climate,(4)interactions between the biosphere and atmosphere,and(5)data assimilation.The intention was not to provide a complete review of all progress made in the last few years,but rather to serve as a starting point for learning more about atmospheric chemistry research in China.The advances reviewed in this paper have enabled a theoretical framework for the air pollution complex to be established,provided robust scientific support to highly successful air pollution control policies in China,and created great opportunities in education,training,and career development for many graduate students and young scientists.This paper further highlights that developing and low-income countries that are heavily affected by air pollution can benefit from these research advances,whilst at the same time acknowledging that many challenges and opportunities still remain in atmospheric chemistry research in China,to hopefully be addressed over the next few decades. | Tong ZHU Mingjin TANG Meng GAO Xinhui BI Junji CAO Huizheng CHE Jianmin CHEN Aijun DING Pingqing FU Jian GAO Yang GAO Maofa GE Xinlei GE Zhiwei HAN Hong HE Ru-Jin HUANG Xin HUANG Hong LIAO Cheng LIU Huan LIU Jianguo LIU Shaw Chen LIU Keding LU Qingxin MA Wei NIE Min SHAO Yu SONG Yele SUN Xiao TANG Tao WANG Tijian WANG Weigang WANG Xuemei WANG Zifa WANG Yan YIN Qiang ZHANG Weijun ZHANG Yanlin ZHANG Yunhong ZHANG Yu ZHAO Mei ZHENG Bin ZHU Jiang ZHU | 2023 | Advances in Atmospheric Sciences2023，40，8： | 2 |
| 11 | Bioaccessibility and health risk of arsenic and heavy metals (Cd, Co, Cr, Cu, Ni, Pb, Zn and Mn) in TSP and PM2.5 in Nanjing, China显示文摘 | Xin Hu Yun Zhang Zhuhong Ding Tijian Wang Hongzhen Lian Yuanyuan Sun Jichun Wu | 2012 | Atmospheric Environment2012，，： | 2 |
| 12 | Simulation of Non-Homogeneous CO2 and Its Impact on Regional Temperature in East Asia显示文摘Carbon dioxide(CO_2) is an important greenhouse gas that influences regional climate through disturbing the earth's energy balance. The CO_2 concentrations are usually prescribed homogenously in most climate models and the spatiotemporal variations of CO_2 are neglected. To address this issue,a regional climate model(RegCM4) is modified to investigate the non-homogeneous distribution of CO_2 and its effects on regional longwave radiation flux and temperature in East Asia. One-year simulation is performed with prescribed surface CO_2 fluxes that include fossil fuel emission, biomass burning, air-sea exchange, and terrestrial biosphere flux. Two numerical experiments(one using constant prescribed CO_2 concentrations in the radiation scheme and the other using the simulated CO_2 concentrations that are spatially non-homogeneous) are conducted to assess the impact of non-homogeneous CO_2 on the regional longwave radiation flux and temperature. Comparison of CO_2 concentrations from the model with the observations from the GLOBALVIEW-CO_2 network suggests that the model can well capture the spatiotemporal patterns of CO_2 concentrations. Generally, high CO_2 mixing ratios appear in the heavily industrialized eastern China in cold seasons, which probably relates to intensive human activities. The accommodation of non-homogeneous CO_2 concentrations in the radiative transfer scheme leads to an annual mean change of -0.12 W m^(-2) in total sky surface upward longwave flux in East Asia. The experiment with non-homogeneous CO_2 tends to yield a warmer lower troposphere.Surface temperature exhibits a maximum difference in summertime, ranging from -4.18 K to 3.88 K, when compared to its homogeneous counterpart. Our results indicate that the spatial and temporal distributions of CO_2 have a considerable impact on regional longwave radiation flux and temperature, and should be taken into account in future climate modeling. | Xiaodong XIE Xiaoxian HUANG Tijian WANG Mengmeng LI Shu LI Pulong CHEN | 2018 | Journal of Meteorological Research2018，32，3： | 2 |
| 13 | Positive and negative regulation of transcription in vitro: enhancer-binding protein AP-2 is inhibited by SV40 T antigen 显示文摘 | Mitchell PJ Wang C Tijian R | 1987 | Cell1987，50，6： | 1 |
| 14 | Characterization of visibility and its affecting factors over Nanjing, China显示文摘 | Junjun Deng Tijian Wang Ziqiang Jiang Min Xie Renjian Zhang Xiaoxian Huang Jialei Zhu | 2011 | Atmospheric Research2011，，3： | 1 |
| 15 | Lead contamination and transfer in urban environmental compartments analyzed by lead levels and isotopic compositions显示文摘 | Xin Hu Yuanyuan Sun Zhuhong Ding Yun Zhang Jichun Wu Hongzhen Lian Tijian Wang | 2014 | Environmental Pollution2014，，： | 1 |
| 16 | Urban air quality and regional haze weather forecast for Yangtze River Delta region 显示文摘 | WANG Tijian JIANG Fei DENG Junjun | 2012 | Atmospheric Environment2012，58，： | 1 |
| 17 | Impacts of biogenic emissions of VOC and NOx on tropospheric ozone during summertime in eastern China 显示文摘 | Qin' geng Wanga Zhiwei Hanb Tijian Wangc etc | 2008 | Science of the Total Environment2008，395，： | 1 |
| 18 | The relation of osteoporosis and Calcium, phosphorous, Zinc content in human hair element显示文摘 | Suen Tijian Shang Xiaohong Dong jin | 1998 | J Shanxi Medical University1998，29，2： | 1 |
| 19 | Impacts of biogenie emissions of VOC and NOx on tropospheric ozone during summertime in eastern China显示文摘 | Qin' geng Wanga Zhiwei Hanb Tijian Wangc etc | 2008 | Science of the Total Environment2008，395，： | 1 |
| 20 | Positive and negative regulation of transcription in vitro:enhancer-binding protein AP-2 is inhibited by SV40 T antigen显示文摘 | Mitchell J P Wang C Tijian R | 1987 | Cell1987，50，6： | 1 |
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