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| 1 | In vivo theranostics with near-infraredemitting carbon dots—highly efficient photothermal therapy based on passive targeting after intravenous administration显示文摘Carbon dots that exhibit near-infrared fluorescence(NIR CDs)are considered emerging nanomaterials for advanced biomedical applications with low toxicity and superior photostability and targeting compared to currently used photoluminescence agents.Despite progress in the synthesis of NIR CDs,there remains a key obstacle to using them as an in vivo theranostic agent.This work demonstrates that the newly developed sulfur and nitrogen codoped NIR CDs are highly efficient in photothermal therapy(PTT)in mouse models(conversion efficiency of 59%)and can be readily visualized by photoluminescence and photoacoustic imaging.The real theranostic potential of NIR CDs is enhanced by their unique biodistribution and targeting.Contrary to all other nanomaterials that have been tested in biomedicine,they are excreted through the body’s renal filtration system.Moreover,after intravenous injection,NIR CDs are accumulated in tumor tissue via passive targeting,without any active species such as antibodies.Due to their accumulation in tumor tissue without the need for intratumor injection,high photothermal conversion,excellent optical and photoacoustic imaging performance,and renal excretion,the developed CDs are suitable for transfer to clinical biomedical practice. | Xin Bao Ye Yuan Jingqin Chen Bohan Zhang Di Li Ding Zhou Pengtao Jing Guiying Xu Yingli Wang Kateřina Holá Dezhen Shen Changfeng Wu Liang Song Chengbo Liu Radek Zbořil Songnan Qu | 2018 | Light(Science & Applications)2018,7,1: | 13 |
| 2 | Thermoelectric properties of p-type (Bi_(0.15)Sb_(0.85))_2Te_3-PbTe graded thermoelectric materials with different barriers显示文摘The p-type (Bi0.15Sb0.85)2Te3 and PbTe are typical thermoelectric materials used for low and middle temperature range and functional graded materials (FGM) is an inevitable way to widen the working temperature range. Here two segments graded thermoelectric materials (GTM) consisting of (Bi0.15Sb0.85)2Te3, PbTe and different barriers were fabricated by the common hot pressure method. Metals Fe, Mg and Ni were used as barriers between the two segments. The diffusion of different barriers between the barriers and bases were analyzed by electron microprobe analysis (EMA). The phase and crystal structures were determined by X-ray diffraction analysis (XRD). The thermoelectric properties were measured at 303 K along the direction parallel to the pressing direction. The results show that the compositional diffusion occurs when there is no barrier at the interface of the two segments, and the diffusion of Pb is most obvious; as the barrier material, the diffusion of metals Fe, Mg and Ni between different bases is not very obvious, and the thermoelectric properties of GTM is much better than that of the original segment. | Guiying Xu Yanping Gao Changchun Ge Weiping Shen | 2005 | Journal of University of Science and Technology Beijing2005,12,4: | 3 |
| 3 | “Reinforced concrete”-like flexible transparent electrode for organic solar cells with high efficiency and mechanical robustness显示文摘Flexible transparent electrodes(FTEs) with robust mechanical stability are crucial for the industrial application of flexible organic solar cells(OSCs). However, their production remains challenging owing to the difficulty in balancing the conductivity,transmittance, and adhesion of FTEs to substrates. Herein, we present the so-called “reinforced concrete” strategy which finetunes the structure of silver nanowires(Ag NWs)-based FTEs with polydopamine(PDA) possessing good adhesion properties and moderate reducibility. The PDA reduces Ag+to form silver nanoparticles(Ag NPs) which grow like “rivets” at the Ag NW junction sites;PDA stabilizes the Ag NW skeleton and improves the adhesion between the Ag NWs and polyethylene terephthalate(PET) substrate and interface layer. The obtained Ag NW:PDA:Ag NP FTE exhibits excellent optoelectronic properties and high mechanical stability. The resulting flexible OSCs exhibit 17.07% efficiency, high flexibility during 10,000 bending test cycles, and robust peeling stability. In addition, this “reinforced concrete”-like FTE provides great advantages for the production of large-area flexible OSCs, thereby paving a new way toward their commercial application. | Yang Chen Juanyong Wan Guiying Xu Xiaoxiao Wu Xinqi Li Yunxiu Shen Fu Yang Xuemei Ou Yaowen Li Yongfang Li | 2022 | Science China Chemistry2022,65,6: | 1 |
| 4 | The measurement of responsivity of infrared photodetectors using a cavity blackbody显示文摘For the measurement of responsivity of an infrared photodetector,the most-used radiation source is a blackbody.In such a measurement system,distance between the blackbody,the photodetector and the aperture diameter are two parameters that contribute most measurement errors.In this work,we describe the configuration of our responsivity measurement system in great detail and present a method to calibrate the distance and aperture diameter.The core of this calibration method is to transfer direct measurements of these two parameters into an extraction procedure by fitting the experiment data to the calculated results.The calibration method is proved experimentally with a commercially extended InGaAs detector at a wide range of blackbody temperature,aperture diameter and distance.Then proof procedures are further extended into a detector fabricated in our laboratory and consistent results were obtained. | Nong Li Dongwei Jiang Guowei Wang Weiqiang Chen Wenguang Zhou Junkai Jiang Faran Chang Hongyue Hao Donghai Wu Yingqiang Xu Guiying Shen Hui Xie Jingming Liu Youwen Zhao Fenghua Wang Zhichuan Niu | 2023 | Journal of Semiconductors2023,44,10: | 0 |
| 5 | Cationic and temperature-sensitive liposomes loaded with eugenol for the application to silk显示文摘Silk has been widely used in the clothing industry due to their soft and smooth features,good biocompatibility,good heat dissipation,warmth and ultraviolet resistance.The application of fragrance to silk can significantly improve the performance of silk.However,there are two key scientific problems that need to be solved:slowing down the release rate of fragrances and increasing the scent lasting time of silk.In this study,cationic and temperature-sensitive liposomes were designed and prepared to encapsulate eugenol.These fragrance-loaded liposomes significantly slowed down the release rate of the fragrance and controlled the release rate of the fragrance in a thermo-sensitive manner.The liposomes adhered to the silk through electrostatic adsorption interaction.The positive charge on the fragranceloaded liposomes neutralized much negative charge on silk and thereby increasing the adhesion efficiency. | Zhiguo Lu Xiangyu Wang Tianlu Zhang Luyao Zhang Jun Yang Yan Li Jie Shen Jianze Wang Yunwei Niu Zuobing Xiao Guiying Liu Xin Zhang | 2020 | Chinese Chemical Letters2020,31,12: | 0 |
| 6 | Photoluminescene study acceptor defects in lightly doped n type GaSb single crystals显示文摘Lightly Te-doped GaSb samples grown by the liquid encapsulated Czochralski(LEC) method have been studied by Hall measurements and low-temperature PL spectroscopy. The results suggest that acceptor-related antisite is the dominant defect in n-type GaSb with low Te-doping concentration. As the Te concentration increases, gallium vacancy related defects become the main acceptor. A new band of around 665 meV is observed in the GaSb sample with the lowest Te-doping concentration. The variation of the acceptor defects and their influence on the electronic and optical property on the n-GaSb single crystal are discussed based on the results. | Guiying Shen Youwen Zhao Yongbiao Bai Jingming Liu Hui Xie Zhiyuan Dong Jun Yang Ding Yu | 2019 | Journal of Semiconductors2019,40,4: | 0 |
| 7 | Reactive nano-essential oils for sustained release of essential oils and application to wallpaper显示文摘Essential oils are a volatile and aromatic substance with a variety of active biological activities.However,the excessive volatility and inconvenience of the use of essential oils limit their applications.In this study,we developed a reactive mesoporous silica nanoparticle(rMSNs)based on cyanuric chloride modification for essential oil encapsulation and commodity adhesion.The large pore volume and specific surface area of rMSNs facilitate the nanoparticles adhering to a large amount of essential oil and achieve the sustained release of essential oil,thus prolonging the fragrance retention time of essential oils.The reactive nanoessential oils can form covalent bonds with the wallpaper,thereby remarkably improving the adhesion of the reactive nano-essential oils on the wallpaper and preventing the reactive nano-essential oil from deadhering from the wallpaper.The active nano essential oil simultaneously overcomes the intense volatility of the essential oil and inconvenience in use,has a simple preparation process and low cost,and has great application potential. | Qiulian Hao Huan Peng Ruichen Zhao Jianze Wang Zhiguo Lu Jingwen Wang Jie Shen Yunwei Niu Zuobing Xiao Guiying Liu Jifu Hao Xin Zhang | 2022 | Chinese Chemical Letters2022,33,1: | 0 |
| 8 | Electrical and optical property of annealed Te-doped GaSb显示文摘GaSb is the most suitable substrate in the epitaxial growth of mixed semiconductors of GaSb system.In this work,Te-doped GaSb bulk crystals with different doping concentration have been annealed at 550℃ for100 h in ambient antimony.The annealed samples have been studied by Hall effect measurement,infrared(IR)optical transmission,Glow discharge mass spectroscopy(GDMS) and photoluminescence(PL) spectroscopy.After annealing,Te-doped GaSb samples exhibit a decrease of carrier concentration and increase of mobility,along with an improvement of below gap IR transmission.Native acceptor related electrical compensation analysis suggests a formation of donor defect with deeper energy level.The mechanism of the variation of the defect and its influence on the material properties are discussed. | Jie Su Tong Liu Jingming Liu Jun Yang Guiying Shen Yongbiao Bai Zhiyuan Dong Fangfang Wang Youwen Zhao | 2017 | Journal of Semiconductors2017,38,4: | 0 |
| 9 | Easily Obtaining Excellent Performance High-voltage LiCoO_(2)via Pr_(6)O_(11)Modification显示文摘Developing an effective method to synthesize high-performance high-voltage LiCoO_(2) is essential for its industrialization in lithium batteries(LIBs).This work proposes a simple mass-produced strategy for the first time,that is,negative temperature coefficient thermosensitive Pr_(6)O_(11) nanoparticles are uniformly modified on LiCoO_(2) to prepare LiCoO_(2)@Pr_(6)O_(11)(LCO@PrO)via a liquid-phase mixing combined with annealing method.Tested at 274 mA g−1,the modified LCO@PrO electrodes deliver excellent 4.5 V high-voltage cycling performance with capacity retention ratios of 90.8%and 80.5%at 25 and 60℃,being much larger than those of 22.8%and 63.2%for bare LCO electrodes.Several effective strategies were used to clearly unveil the performance enhancement mechanism induced by Pr_(6)O_(11) modification.It is discovered that Pr_(6)O_(11) can improve interface compatibility,exhibit improved conductivity at elevated temperature,thus enhance the Li^(+)diffusion kinetics,and suppress the phase transformation of LCO and its resulting mechanical stresses.The 450 mAh LCO@PrO‖graphite pouch cells show excellent LIB performance and improved thermal safety characteristics.Importantly,the energy density of such pouch cell was increased even by~42%at 5 C.This extremely convenient technology is feasible for producing high-energy density LIBs with negligible cost increase,undoubtedly providing important academic inspiration for industrialization. | Yongcong Huang Chenjie Xu Jingguo Gao Liao Shen Qian Liu Guiying Zhao Qingshui Xie Yingbin Lin Jiaxin Li Zhigao Huang | 2023 | Energy & Environmental Materials2023,6,2: | 0 |
| 10 | Structural Characterization of Carbon-implanted GaSb显示文摘Ion implantation induced damage in GaSb and its removal by rapid thermal annealing(RTA)have been investigated by Raman spectroscopy.The evolution of the Raman modes as a function of implantation fluence,annealing temperature and time has been analyzed.Results indicate that a lattice quality that is close to as-grown GaSb has been obtained by annealing the implanted samples at 500℃for 45 s.However,consequent surface analyses by scanning electron microscope(SEM)and atomic force microscope(AFM)show that a heavily perturbed layer contains voids due to the outdifiusion of Sb atoms on the surface remains.Mechanism of the damage recovery and the structure of the implanted layer are discussed based on the experimental results. | SHEN Guiying ZHAO Youwen HE Jianjun | 2023 | Journal of Wuhan University of Technology(Materials Science)2023,38,5: | 0 |
| 11 | Performance improvement of c-Si solar cell by a combination of SiNx/SiOx passivation and double P-diffusion gettering treatment显示文摘SiN_x/SiO_x passivation and double side P-diffusion gettering treatment have been used for the fabrication of c-Si solar cells. The solar cells fabricated have high open circuit voltage and short circuit current after the double P-diffusion treatment. In addition to better surface passivation effect, SiN_x/SiO_x layer has lower reflectivity in long wavelength range than conventional SiN_x film. As a consequence, such solar cells exhibit higher conversion efficiency and better internal quantum efficiency, compared with conventional c-Si solar cells. | Xiaoyu Chen Youwen Zhao Zhiyuan Dong Guiying Shen Yongbiao Bai Jingming Liu Hui Xie Jiangbian He | 2017 | Journal of Semiconductors2017,38,11: | 0 |
| 12 | Thermoelectric Properties of N-typer Bi_2Te_3-PbTe Graded Thermoelectric Materials with Different Barriers显示文摘In order to investigate the adaptability of thermoelectric materials system with different barriers to functional graded thermoelectric materials, n-type Bi2Te3 and PbTe two segments graded thermoelectric materials (GTM) with different barriers were fabricated by conventional hot pressing method. Metals Cu, Al, Fe, Co and Ni were used as barriers between two segments. The effects of different barriers on thermoelectric properties of GTM were investigated. The phase and crystal structures were determined by x-ray diffraction analysis (XRD). The distributions of different compositions were analyzed by electron microprobe analysis (EMA). The thermoelectric properties were measured at 303 K along the direction parallel to the pressing direction. The electric conductivity of samples was measured at 303 K by the four-probe technique. To measure the Seebeck coefficient, heat was applied to the samples, which were placed between two Cu discs. The thermoelectric electromotive force (E) was measured upon applying small temperature differences (△T< 275 K) between the both ends of the samples. The Seebeck coefficient of the samples was determined from the E/△T. | Guiying Xu, Changchun Ge, Yanping Gao, Weiping Shen Laboratory of Special Ceramics and Powder Metallurgy, University of Science and Technology Beijing. Beijing 100083, China | 2001 | Journal of University of Science and Technology Beijing2001,8,4: | 0 |