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| 1 | Terahertz surface plasmonic waves: a review显示文摘Terahertz science and technology promise many cutting-edge applications.Terahertz surface plasmonic waves that propagate at metal–dielectric interfaces deliver a potentially effective way to realize integrated terahertz devices and systems.Previous concerns regarding terahertz surface plasmonic waves have been based on their highly delocalized feature.However,recent advances in plasmonics indicate that the confinement of terahertz surface plasmonic waves,as well as their propagating behaviors,can be engineered by designing the surface environments,shapes,structures,materials,etc.,enabling a unique and fascinating regime of plasmonic waves.Together with the essential spectral property of terahertz radiation,as well as the increasingly developed materials,microfabrication,and time-domain spectroscopy technologies,devices and systems based on terahertz surface plasmonic waves may pave the way toward highly integrated platforms for multifunctional operation,implementation,and processing of terahertz waves in both fundamental science and practical applications.We present a review on terahertz surface plasmonic waves on various types of supports in a sequence of properties,excitation and detection,and applications.The current research trend and outlook of possible research directions for terahertz surface plasmonic waves are also outlined. | Xueqian Zhang Quan Xu Lingbo Xia Yanfeng Li Jianqiang Gu Zhen Tian Chunmei Ouyang Jiaguang Han Weili Zhang | 2020 | Advanced Photonics2020，2，1： | 7 |
| 2 | Study on the quantitative structureactivity relation-ship of C-10 substituted artemisinin(QHS)’s derivatives using rough set theory显示文摘The structure-activity relationship study of C-10 substituted artemisinin (QHS) derivatives that are used as antimalarial was performed with the RS (rough sets) method. An RS process is a concise nonlinear process, and it has broad application foreground in the data mining of nonlinear life courses. In this work, initially the parameters of C-10 substituted QHS’s derivatives were computed with the quantum chemistry method, and the information table was constructed from the parameters (condition attributes) and biological activity (decision attributes). Based on the analysis of rough set theory, the core and reduction of attributes sets were obtained. Then the decision rules were extracted and the struc-ture-activity relationship was analyzed. As a nonlinear system, RS theory can extract the special rela-tion in the database. It has the advantage of being nonlinear over multiple linear regression (MLR), principal component analysis (PCA), partial least square (PLS), etc., and the advantage of obtaining results with unambiguous physical meanings over artificial neuron networks (ANNs), etc. The result obtained in this study is instructive to the study of pharmacodynamics, resistance mechanism of QHS and development of QHS’s derivatives. | LIU Hao QU LingBo GAO HongBin WANG JinXiang HAN LiPing XIANG BingRen | 2008 | Science China Chemistry2008，51，10： | 5 |
| 3 | Follicular hyperandrogenism and insulin resistance in polycystic ovary syndrome patients with normal circulating testosterone levels显示文摘Polycystic ovary syndrome(PCOS) is a common reproductive disease with high heterogeneity. The role of excess androgen in PCOS etiology remains disputed, since around 20%-50% of PCOS women do not display hyperandrogenemia. The microenvironment of the ovary critically influences follicular development. In the present study, we assessed the role of androgen in PCOS by investigating whether excessive follicular fluid androgen was present in PCOS patients with normal serum androgen levels and influenced by follicular fluid insulin resistance(IR).Follicular fluid samples of 105 women with PCOS and 105 controls were collected. Levels of steroid hormones,glucose and insulin in the follicular fluid were examined and compared with data from serum biochemistry tests. We found that 64.9%(63/97) of PCOS patients with normal serum androgen levels displayed abnormally high follicular fluid androgen level. The follicular fluid androgen level was positively correlated with follicular fluid IR within a certain range and follicular fluid estrogen-to-testosterone(E2/T) ratio was significantly reduced in these patients.These results indicated that there existed a subgroup of PCOS patients who displayed excessive follicular fluid androgen and IR despite their normal circulating testosterone(T) levels. Our study highlights the importance of ovary hyperandrogenism and IR in the etiology of PCOS. | Andi Li Lu Zhang Jiajia Jiang Nan Yang Ying Liu Lingbo Cai Yugui Cui Feiyang Diao Xiao Han Jiayin Liu Yujie Sun | 2018 | The Journal of Biomedical Research2018，32，3： | 2 |
| 4 | Comprehensive characterization of oil refinery effluent derived humic substances using various spectroscopic approaches显示文摘 | Li Lingbo Yan Song Han Congbi Shan Guangbo | 2005 | ChemospHere2005，60，4： | 1 |
| 5 | Comprehensive characterization of oil refinery effluent-derived humic sub- stances using various speetroscopic approaches 显示文摘 | Li Lingbo Yan Song Han Congbi | 2005 | Chemosphere2005，60，4： | 1 |
| 6 | Intrinsic in-plane nodal chain and generalized quaternion charge protected nodal link in photonics显示文摘Nodal lines are degeneracies formed by crossing bands in three-dimensional momentum space.Interestingly,these degenerate lines can chain together via touching points and manifest as nodal chains.These nodal chains are usually embedded in two orthogonal planes and protected by the corresponding mirror symmetries.Here,we propose and demonstrate an in-plane nodal chain in photonics,where all chained nodal lines coexist in a single mirror plane instead of two orthogonal ones.Nodal lines are degeneracies formed by crossing bands in three-dimensional momentum space.Interestingly,these degenerate lines can chain together via touching points and manifest as nodal chains.These nodal chains are usually embedded in two orthogonal planes and protected by the corresponding mirror symmetries.Here,we propose and demonstrate an in-plane nodal chain in photonics,where all chained nodal lines coexist in a single mirror plane instead of two orthogonal ones.The chain point is stabilized by the intrinsic symmetry that is specific to electromagnetic waves at theГpoint of zero frequency.By adding another mirror plane,we find a nodal ring that is constructed by two higher bands and links with the in-plane nodal chain.The nodal link in momentum space exhibits non-Abelian characteristics on a C_(2)T-invariant plane,where admissible transitions of the nodal link structure are determined by generalized quaternion charges.Through near-field scanning measurements of bi-anisotropic metamaterials,we experimentally mapped out the in-plane nodal chain and nodal link in such systems.The chain point is stabilized by the intrinsic symmetry that is specific to electromagnetic waves at the r point of zero frequency.By adding another mirror plane,we find a nodal ring that is constructed by two higher bands and links with the in-plane nodal chain.The nodal link in momentum space exhibits non-Abelian characteristics on a C2T-invariant plane,where admissible transitions of the nodal link structure are determined by generalized quaternion charges.Through near-field scanning measurements of bi-anisotropic metamaterials,we experimentally mapped out the in-plane nodal chain and nodal link in such systems. | Dongyang Wang Biao Yang Qinghua Guo Ruo-Yang Zhang Lingbo Xia Xiaoqiang Su Wen-Jie Chen Jiaguang Han Shuang Zhang C.T.Chan | 2021 | Light(Science & Applications)2021，10，5： | 0 |
| 7 | Synthesis of a novel magnetic biomass-MOF composite for the efficient removal of phosphates:Adsorption mechanism and characterization study显示文摘The adverse effects of eutrophication have prompted the use of various remediation techniques for phosphate(PO_(4)^(3-))removal owing to it being the major causative agent.Herein,the influence of different solvents and ratios of 2-aminoterepthalicacid on the efficiency of magnetic biomass metal-organic framework composites based on the in situ growth of NH_(2)-MIL-101(Fe)onto magnetized peanut husks towards PO_(4)^(3-)removal was assessed via the adsorption technique.The magnetic biocomposite labelled as MPN@NH2-MIL-101(Fe)exhibited the best efficiency owing to its mesoporous structures and presence of abundant oxygen and nitrogen possessing functional groups.Adsorption results confirmed MPN@NH2-MIL-101(Fe)to have a high adsorption capacity of(14.0±0.3)mg·L^(-1)at a PO43-concentration of 20 mg·L^(-1)with an associated high stability within pH 2-10.The adsorption kinetics for the process was well described by both Elovich and pseudo-second-order kinetic models and was mediated by both internal diffusion and liquid film diffusion.The Temkin and Freundlich models fitted the equilibrium data well signifying occurrence of both physical and chemical adsorption on a heterogeneous surface.It is concluded that MPN@NH2-MIL-101(Fe)is a promising adsorbent for the effective removal of phosphate from a water body. | Aaron Albert Aryee Chenping Gao Runping Han Lingbo Qu | 2023 | Chinese Journal of Chemical Engineering2023，62，10： | 0 |
| 8 | Mechanisms and reusability potentials of zirconium-polyaziridine-engineered tiger nut residue towards anionic pollutants显示文摘Access to fresh water,its availability,and its quality are a global challenge to humanity,largely due to human activities in the environment.Thus,global water security has been jeopardized,requiring urgent remediation to safeguard our very existence.Hence,a novel and facilely engineered zirconium and polyethylenimine adsorbent based on tiger nut residue (TNR) was prepared,and its adsorptive capabilities towards a model dyestuff and nutrient were invested through a batch adsorption method.The developed adsorbent,zirconium-polyethylenimine-engineered tiger nut residue (TNR@PEI–Zr) was characterised by scanning electron microscopy,Fourier-transform infrared spectroscopy,X-ray diffraction analysis,and X-ray photoelectron spectroscopy to understand its morphology and surface chemistry and predict its adsorption mechanism.TNR@PEI–Zr had a p H point of zero charge (pH_(zpc)) of 6.7.The introduction of salts inhibited the removal efficiency of Alizarin red (AR) and phosphate (PO_(4)^(3–)) in the order of HCO_(3)^(-)>SO_(4)^(2–)>Cl^(-).Increasing temperatures (293–313 K) favoured the adsorption process at pH 3.The Langmuir model suited the adsorption processes of both AR and PO_(4)^(3–),implying homogenous and monolayer removal of pollutants with a maximal capacity of 537.8 mg·g^(-1)and 100.5 mg·g^(-1)at a dose of 0.01 g,respectively.The rate-determining steps of AR and PO_(4)^(3–)followed a pseudo-secondorder kinetic model and were thermodynamically spontaneous with an increase in randomness at the solid-solution interface.The adsorbent’s recyclability was notable and outperformed most adsorbents in terms of removal efficiency.TNR@PEI–Zr was found to be stable,and its use in practical wastewater decontamination was effective,ecologically acceptable and free of secondary pollution problems. | Alexander Nti Kani Evans Dovi Aaron Albert Aryee Runping Han Zhaohui Li Lingbo Qu | 2023 | Chinese Journal of Chemical Engineering2023，60，8： | 0 |
| 9 | Fine-tuning hydroxylamines as single-nitrogen sources for Pd(0)-catalyzed diamination of o-bromo(or chloro)-biaryls显示文摘Transition metal-catalyzed diamination by hydroxylamines is a common approach for making three-membered aziridines,while its use for building the larger N-heterocycles is still underdeveloped.Herein,we report an efficient Pd(0)-catalyzed intermolecular[4+1]annulation of o-bromo(or chloro)-biaryls with bifunctional secondary hydroxylamines for the one-step assembly of synthetically useful carbazoles.Noteworthily,a linchpin for this domino reaction was the judicious selection of both the amino-sources and Pd(0)-catalysts for enabling the prerequisite oxidative addition of aryl halides to Pd(0)-species in the presence of hydroxylamines with a labile N-O bond. | Pin Ding Lingbo Han Jiaxing Bai Jingjing Liu Xinjun Luan | 2022 | Science China Chemistry2022，65，4： | 0 |
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