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| 1 | Arsenic hyperaccumulator Pteris Vittata L. and its arsenic accumulation显示文摘An arsenic hyperaccumulator Pteris vittata L. (Chinese brake) was first discovered in China by means of field survey and greenhouse cultivation. Field survey showed that Chinese brake had large accumulating capacity to arsenic; the orders of arsenic content in different parts of the fern were as follows: leaves>leafstalks>roots, which is totally different from that of ordinary plants; bioaccumulation coefficients of the above ground parts of the fern decreased as a power function of soil arsenic contents. In the control of pot trials with normal unpolluted soil containing 9mg/kg of arsenic, the bioaccumulation coefficients of the above ground parts and rhizoids of Chinese brake were as high as 71 and 80 respectively. Greenhouse cultivation in the contaminated soil from mining areas has shown that more than 1 times greater arsenic can be accumulated in the leaves of the fern than that of field samples with the largest content of 5070 mg/kg As on a dry matter basis. During greenhouse cultivation, arsenic | Tongbin Chen Chaoyang Wei Zechun Huang Qifei Huang Quanguo Lu Zilian Fan | 2002 | Chinese Science Bulletin2002，47，11： | 108 |
| 2 | Methylation profile of the promoter CpG islands of 14 “drug-resistance”genes in hepatocellular carcinoma显示文摘AIM: To establish the DNA methylation patterns of the promoter CpG islands of 14 'drug-resistance' genes in hepatocellular carcinoma (HCC).METHODS: The methylation specific polymerase chain reaction in conjunction with sequencing verification was used to establish the methylation patterns of the 14 genes in the liver tissues of four healthy liver donors, as well as tumor and the paired non-cancerous tissues of 30 HCC patients.RESULTS: While 11 genes (ATP-binding cassette, sub-family G (WHITE), member 2(ABCG2), activating transcription factor (ATF2), beta-2-microglobulin (B2M), deoxycytidine kinase(DCK, occludin (OCLN, v-raf-1 murine leukemia viral oncogene homolog (RAF/), ralA binding protein 1 (RALBP1),splicing factor (45 kD) (SPF45), S-phase kinase-associated protein 2 (p45) (SKP2), tumor protein p53 (Li-Fraumeni syndrome) (TP53) and topoisomerase (DNA) II beta (TOP2B) maintained the unmethylated patterns, three genes displayed to various extents the hypermethylation state in tumor tissues in comparison with the normal counterparts. The catalase (CAT) was hypermethylated in tumor and the neighboring non-cancerous tissue of one case (3.3%). Both glutathione S-transferase pi (GSTp/) (80%, 24/30 in tumor and 56.7%,17/30 in the paired non-cancerous tissues) and cystic fibrosis transmembrane conductance regulator, ATP-binding cassette (sub-family C, member 7) (CF-FR) (77%, 23/30 in tumor and 50%, 15/30 in the paired non-cancerous tissues) genes were prevalently hypermethylated in HCC as well as their neighboring non-cancerous tissues. No significant difference in the hypermethylation occurrence was observed between the HCC and its neighboring non-cancerous tissues.CONCLUSION: Hypermethylation of promoter CpG islands of both CF-FR and GSTpigenes occurs prevalently in HCC,which may correlate with the low expression of these two genes at the mRNA level and has the profound etiological and clinical implications. It is likely to be specific to the early phase of HCC carcinogenesis. | ShengDing Bang-DongGong JianYu JunGu Hong-YuZhang Zu-BinShang QiFei PengWang Jing-DeZhu | 2004 | World Journal of Gastroenterology2004，10，23： | 14 |
| 3 | Evolution on qualities of leachate and landfill gas in the semi-aerobic landfill显示文摘在半氧气的垃圾堆学习稳定的特征,大规模模仿的垃圾堆基于半被构造氧气的垃圾堆理论。因而,化学的氧需求(货到付款) 的集中,氨氮,和亚硝酸根氮,和 pH 在沥滤吃,以及在垃圾堆的垃圾堆气体作文(甲烷,二氧化碳,和氧) 的成分含量定期被监视 52 个星期。结果证明货到付款和氨集中很快衰退了并且没显示出象厌氧的垃圾堆一样的积累的规则,并且分别地,在 48 个星期以后在大约 300 和 100 mg/L 留下。同时,下降的率分别地到达了 98.9% 和 96.9% 。硝酸盐集中在 24 个星期以后很快增加了并且在 43 个星期以后在 220 280 mg/L 之间波动。pH 在开始的 8 个星期期间并且在以后低于 7 沥滤 ates 看起来碱。二氧化碳是在通过整个稳定过程在高水平仍然是的垃圾堆气体和它的集中的主要作文。二氧化碳,氧,和甲烷的平均内容在 19 vol.% 之间改变了 28 vol.% , 2 vol.% 8 vol.% ,和 5 vol.% 13 vol.% 分别地。相对平衡在 48 个星期以后被到达。在垃圾堆房间的最高的温度能等于摄氏的 75.8 度。 | HUANG Qifei YANG Yufei PANG Xiangrui WANG Qi | 2008 | Journal of Environmental Sciences2008，20，4： | 11 |
| 4 | Effects of grazing on net primary productivity,evapotranspiration and water use efficiency in the grasslands of Xinjiang,China显示文摘Grazing is a main human activity in the grasslands of Xinjiang, China. It is vital to identify the effects of grazing on the sustainable utilization of local grasslands. However, the effects of grazing on net primary productivity(NPP), evapotranspiration(ET) and water use efficiency(WUE) in this region remain unclear. Using the spatial Biome-BGC grazing model, we explored the effects of grazing on NPP, ET and WUE across the different regions and grassland types in Xinjiang during 1979–2012. NPP, ET and WUE under the grazed scenario were generally lower than those under the ungrazed scenario, and the differences showed increasing trends over time. The decreases in NPP, ET and WUE varied significantly among the regions and grassland types. NPP decreased as follows: among the regions, Northern Xinjiang(16.60 g C/(m^2·a)), Tianshan Mountains(15.94 g C/(m^2·a)) and Southern Xinjiang(-3.54 g C/(m^2·a)); and among the grassland types, typical grasslands(25.70 g C/(m^2·a)), swamp meadows(25.26 g C/(m^2·a)), mid-mountain meadows(23.39 g C/(m^2·a)), alpine meadows(6.33 g C/(m^2·a)), desert grasslands(5.82 g C/(m^2·a)) and saline meadows(2.90 g C/(m^2·a)). ET decreased as follows: among the regions, Tianshan Mountains(28.95 mm/a), Northern Xinjiang(8.11 mm/a) and Southern Xinjiang(7.57 mm/a); and among the grassland types, mid-mountain meadows(29.30 mm/a), swamp meadows(25.07 mm/a), typical grasslands(24.56 mm/a), alpine meadows(20.69 mm/a), desert grasslands(11.06 mm/a) and saline meadows(3.44 mm/a). WUE decreased as follows: among the regions, Northern Xinjiang(0.053 g C/kg H_2O), Tianshan Mountains(0.034 g C/kg H_2O) and Southern Xinjiang(0.012 g C/kg H_2O); and among the grassland types, typical grasslands(0.0609 g C/kg H_2O), swamp meadows(0.0548 g C/kg H_2O), mid-mountain meadows(0.0501 g C/kg H_2O), desert grasslands(0.0172 g C/kg H_2O), alpine meadows(0.0121 g C/kg H_2O) and saline meadows(0.0067 g C/kg H_2O). In general, the decreases in NPP and WUE were more significant in the regions with relatively high levels of vegetation growth because of the high grazing intensity in these regions. The decreases in ET were significant in mountainous areas due to the terrain and high grazing intensity. | HUANG Xiaotao LUO Geping YE Feipeng HAN Qifei | 2018 | Journal of Arid Land2018，10，4： | 9 |
| 5 | Mo-modified Pd/Al_2O_3 catalysts for benzene catalytic combustion显示文摘Mo-modified Pd/Al2O3catalysts were prepared by an impregnation method and tested for the catalytic combustion of benzene. The catalysts were characterized by N2 isothermal adsorption, X-ray diffraction(XRD), X-ray photoelectron spectroscopy(XPS), temperatureprogrammed desorption of NH3(NH3-TPD), H2temperature-programmed reduction(H2-TPR), and high-angle annular dark-field scanning transmission electron microscopy(HAADF-STEM). The results showed that the addition of Mo effectively improved the activity and stability of the Pd/Al2O3catalyst by increasing the dispersion of Pd active components, changing the partial oxidation state of palladium and increasing the oxygen species concentration on the surface of catalyst. In the case of the Pd–Mo/Al2O3catalyst,benzene conversion of 90% was obtained at temperatures as low as 190°C, which was 45°C lower than that for similar performance with the Pd/Al2O3catalyst. Moreover, the 1.0% Pd–5% Mo/Al2O3catalyst was more active than the 2.0% Pd/Al2O3catalyst. It was concluded that Pd and Mo have a synergistic effect in benzene catalytic combustion. | Zhanfeng He Zhanrong He Dan Wang Qifei Bo Ting Fan Yi Jiang | 2014 | Journal of Environmental Sciences2014，26，7： | 6 |
| 6 | Advances in metal phosphides for sodium-ion batteries显示文摘Sodium-ion batteries(SIBs)have been extensively studied as the potential alter-native to lithium-ion batteries(LIBs)due to the abundant natural reserves and low price of sodium resources.Nevertheless,Na+ions possess a larger radius than Li+,resulting in slow diffusion dynamics in electrode materials,and thus seeking appropriate anode materials to meet high performance standards has become a trend in the field of SIBs.In this context,owing to the advantages of high theoretical capacity and proper redox potential,metal phosphides(MPs)are considered to be the promising materials to make up for the gap of SIBs anode materials.In this review,the recent development of MPs anode materials for SIBs is reviewed and analyzed comprehensively and deeply,including the synthesis method,advanced modification strategy,electrochemical performance,and Na storage mechanism.In addition,to promote the wide application of the emerg-ing MPs anodes for SIBs,several research emphases in the future are pointed out to overcome challenges toward the commercial application. | Qifei Li Dan Yang Haoliang Chen Xiang Lv Yu Jiang Yuezhan Feng Xianhong Rui Yan Yu | 2021 | SusMat2021，1，3： | 5 |
| 7 | Modeling grassland net primary productivity and water-use efficiency along an elevational gradient of the Northern Tianshan Mountains显示文摘Mountainous ecosystems are considered highly sensitive and vulnerable to natural disasters and climatic changes.Therefore,quantifying the effects of elevation on grassland productivity to understand ecosystem-climate interactions is vital for mountainous ecosystems.Water-use efficiency(WUE)provides a useful index for understanding the metabolism of terrestrial ecosystems as well as for evaluating the degradation of grasslands.This paper explored net primary productivity(NPP)and WUE in grasslands along an elevational gradient ranging from 400 to 3,400 m asl in the northern Tianshan Mountains-southern Junggar Basin(TMJB),Xinjiang of China,using the Biome-BGC model.The results showed that:1)the NPP increased by 0.05 g C/(m2·a)with every increase of 1-m elevation,reached the maximum at the mid-high elevation(1,600 m asl),and then decreased by 0.06 g C/(m2·a)per 1-m increase in elevation;2)the grassland NPP was positively correlated with temperature in alpine meadow(AM,2,700-3,500 m asl),mid-mountain forest meadow(MMFM,1,650-2,700 m asl)and low-mountain dry grassland(LMDG,650-1,650 m asl),while positive correlations were found between NPP and annual precipitation in plain desert grassland(PDG,lower than 650 m asl);3)an increase(from 0.08 to 1.09 g C/(m2·a))in mean NPP for the grassland in TMJB under a real climate change scenario was observed from 1959 to 2009;and 4)remarkable differences in WUE were found among different elevations.In general,WUE increased with decreasing elevation,because water availability is lower at lower elevations;however,at elevations lower than 540 m asl,we did observe a decreasing trend of WUE with decreasing elevation,which may be due to the sharp changes in canopy cover over this gradient.Our research suggests that the NPP simulated by Biome-BGC is consistent with field data,and the modeling provides an opportunity to further evaluate interactions between environmental factors and ecosystem productivity. | QiFei HAN GePing LUO ChaoFan LI Hui YE YaoLiang CHEN | 2013 | Journal of Arid Land2013，5，3： | 5 |
| 8 | Mapping of Regional Soil Salinities in Xinjiang and Strategies for Amelioration and Management显示文摘Information on the spatial distribution of soil salinity can be used as guidance in avoiding the continued degradation of land and water resources by better informing policy makers. However, most regional soil-salinity maps are produced through a conventional direct-linking method derived from historic observations. Such maps lack spatial details and are limited in describing the evolution of soil salinization in particular instances. To overcome these limitations, we employed a method that included an integrative hierarchical-sampling strategy(IHSS) and the Soil Land Inference Model(So LIM) to map soil salinity over a regional area. A fuzzy c-means(FCM) classifier is performed to generate three measures, comprising representative grade, representative area, and representative level(membership). IHSS employs these three measures to ascertain how many representative samples are appropriate. Through this synergetic assessment, representative samples are obtained and their soil-salinity values are measured. These samples are input to So LIM, which is constructed based on fuzzy logic, to calculate the soil-forming environmental similarities between representative samples and other locations. Finally, a detailed soil-salinity map is produced through an averaging function that is linearly weighted, which is used to integrate the soil salinity value and soil similarity. This case study, in the Uyghur Autonomous Region of Xinjiang of China, demonstrates that the employed method can produce soil salinity map at a higher level of spatial detail and accuracy. Twenty-three representative points are determined. The results show that 1) the prediction is appropriate in Kuqa Oasis(R2 = 0.70, RPD = 1.55, RMSE = 12.86) and Keriya Oasis(R2 = 0.75, RPD = 1.66, RMSE = 10.92), that in Fubei Oasis(R2 = 0.77, RPD = 2.01, RMSE = 6.32) perform little better than in those two oases, according to the evaluation criterion. 2) Based on all validation samples from three oases, accuracy estimation show the employed method(R2 = 0.74, RPD = 1.67, RMSE = 11.18) performed better than the multiple linear regression model(R2 = 0.60, RPD = 1.47, RMSE = 14.45). 3) The statistical result show that approximately half(48.07%) of the study area has changed to salt-affected soil, mainly distributed in downstream of oases, around lakes, on both sides of rivers and more serious in the southern than the northern Xinjiang. To deal with this issue, a couple of strategies involving soil-salinity monitoring, water management, and plant diversification are proposed, to reduce soil salinization. Finally, this study concludes that the employed method can serve as an alternative model for soil-salinity mapping on a large scale. | WANG Fei CHEN Xi LUO Geping HAN Qifei | 2015 | Chinese Geographical Science2015，25，3： | 4 |
| 9 | Pollution characteristics of polycyclic aromatic hydrocarbons in common used mineral oils and their transformation during oil regeneration显示文摘The pollution characteristic of polycyclic aromatic hydrocarbons(PAHs) in common used mineral oils, semi-refined oils, refined oils and solid wastes produced during the used mineral oil regeneration process was analyzed. The results showed that total PAHs content in six common used mineral oils was as follows: used engine oil > used quenching oil > used casting oil > used hydraulic oil > used antirust oil > used industrial lubricating oil. Furthermore, this order was dependent on the source of PAHs and oil working temperatures. Additionally, total PAHs content in regenerated oils was as follows: semi-refined oil > refined oil > crude oil, which was related to the catalytic cracking process of crude oil and adsorption refining process of semi-refined oil. The ranking of total PAHs content in regenerated wastes varied depending on the regeneration technology used as follows: waste adsorption sand > acid sludge > waste clay > precipitation sludge > cracked residue. In all types of used mineral oils and regenerated wastes, the maximum and minimum proportions of the total PAHs content were composed of 2–3 ring-PAHs and 5–6 ring-PAHs, respectively. The majority of PAHs in the used mineral oils entered into regenerated wastes during regeneration process, while a small number remained in the regenerated oil. | Xiaohui Wu Bo Yue Yi Su Qi Wan Qifei Huang Qunhui Wang Hongying Cai | 2017 | Journal of Environmental Sciences2017，29，6： | 3 |
| 10 | SrCo_(0.7)Fe_(0.2)Nb_(0.1)O_(3-δ) perovskite stabilized by niobium for oxygen permeation显示文摘The effect of Nb doping on the oxygen permeation and stability of SrCo_(0.8)Fe_(0.2)O_(3-δ)(SCFO) was investigated comprehensively.Cubic perovskite phase was formed in SrCo_(0.7)Fe_(0.2)Nb_(0.1)O_(3-δ)(SCFNO).The SCFNO with a thickness of 1 mm had a high level of oxygen permeation flux of 1.4 ml.min^(-1).cm^(-2) at 850 ℃ under air/He gradient.The bulk diffusion is the rate-limiting step in overall oxygen permeation mechanism for SCFNO when the thickness is higher than 1.0 mm.The partial substitution of Nb for Co suppresses the transition of oxygen vacancies order/disorder proven by DSC measurement and enhances the phase stability under low oxygen partial pressure.During long-term tests under low oxygen pressure,the SCFNO exhibites structural stability and stable oxygen permeation.It is proved that substitution of Nb for Co is an effective way to improve the properties of SCFO. | Wang, Haihai Zhang, Yuwen Geng, Zhen Zhang, Qifei Gai, Yongqian Ding, Weizhong | 2012 | Rare Metals2012，31，4： | 3 |
| 11 | Bacterial community composition and abundance in leachate of semi-aerobic and anaerobic landfills显示文摘The abundance and phylogenetic composition of bacterial community in leachate of semi-aerobic and anaerobic landfill were compared through real-time polymerase chain reaction and denaturing gradient gel electrophoresis. In semi-aerobic landfill scenario, the bacterial 16S rRNA copy numbers in leachate had no significant reduction from initial stage to stable period. In the scenario of anaerobic landfill, the largest bacterial 16S rRNA gene copy number was found in leachate at initial stage, but it reduced significantly at stable period. Moreover, methane-oxidizing bacteria population in stable period was lower than that in initial period in both two landfill processes. However, semi-aerobic landfill leachate had more methanotrophic bacteria populations than that in the anaerobic one. Furthermore, according to the sequences and phylogenetic analysis, obvious difference could be detected in bacterial community composition in different scenarios. Proteobacteria and bacteroidetes took up a dominantly higher proportion in semi-aerobic landfill leachate. To summarize up, different landfill methods and its landfill ages had crucial impacts on bacterial abundance and composition in leachate of semi-aerobic and anaerobic landfills. | Wei Zhang Bo Yue Qi Wang Zechun Huang Qifei Huang Zengqiang Zhang | 2011 | Journal of Environmental Sciences2011，23，11： | 2 |
| 12 | A novel ball-in-ball hollow oxygen-incorporating cobalt sulfide spheres as high-efficient electrocatalyst for oxygen evolution reaction显示文摘Transition-metal chalcogenides with hollow nanostructure,especially cobalt sulfides,are considered as the most pro mising non-precious metal catalysts for oxygen evolution reactio n.However,it is difficult to synthesize oxygen-containing cobalt sulphides with hollow structure due to the different physical/chemical properties between metal sulfides and metal cobalts.Herein,we report a novel oxygencontaining amorphous cobalt sulfide ball-in-ball hollow sphere s(Co-S-O BBHS) synthesized by an anion exchange method.Taking advantage of the ball-in-ball hollow structure,the amorphous Co-S-O BBHS shows supe rior oxygen evolution reaction(OER) electrocatalytic performance with a low overpotentiat of285 mV at 10 mA/cm2,small Tafel slope of 49.67 mV/dec,high Faraday efficiency of 96%,and satisfied durability.Experiments and DFT calculations demonstrate that the introduction of oxygen and sulfur modulates the electronic structure of Co-S-O BBHS,thus enhancing the adsorption of *0(adsorbed 0 species on catalyst surface) intermediate,which greatly boosts the catalytic activity towards OER.This work provides a new strategy for controllable synthe sis of complex hollow structures of transition-metal chalcogenides for OER. | Yurong Li Qifei Guo Yimin Jiang Wei Shen Ming Li Rongxing He | 2021 | Chinese Chemical Letters2021，32，2： | 2 |
| 13 | Negative regulation of transcription factor FoxM1 by p53 enhances oxaliplatin-induced senescence in hepatocellular carcinoma显示文摘 | Kai Qu Xinsen Xu Chang Liu Qifei Wu Jichao Wei Fandi Meng Lei Zhou Zhixin Wang Lei Lei Peijun Liu | 2012 | Cancer Letters2012，，： | 2 |
| 14 | A High-Capacity Ammonium Vanadate Cathode for Zinc-Ion Battery显示文摘Given the advantages of being abundant in resources,environmental benign and highly safe,rechargeable zinc-ion batteries(ZIBs)enter the global spotlight for their potential utilization in large-scale energy storage.Despite their preliminary success,zinc-ion storage that is able to deliver capacity>400 mAh g^-1 remains a great challenge.Here,we demonstrate the viability of NH4V4O10(NVO)as high-capacity cathode that breaks through the bottleneck of ZIBs in limited capacity.The first-principles calculations reveal that layered NVO is a good host to provide fast Zn^2+ions diffusion channel along its[010]direction in the interlayer space.On the other hand,to further enhance Zn^2+ion intercalation kinetics and long-term cycling stability,a three-dimensional(3D)flower-like architecture that is self-assembled by NVO nanobelts(3D-NVO)is rationally designed and fabricated through a microwave-assisted hydrothermal method.As a result,such 3D-NVO cathode possesses high capacity(485 mAh g^-1)and superior long-term cycling performance(3000 times)at 10 A g^-1(~50 s to full discharge/charge).Additionally,based on the excellent 3D-NVO cathode,a quasi-solid-state ZIB with capacity of 378 mAh g^-1is developed. | Qifei Li Xianhong Rui Dong Chen Yuezhan Feng Ni Xiao Liyong Gan Qi Zhang Yan Yu Shaoming Huang | 2020 | Nano-Micro Letters2020，12，5： | 2 |
| 15 | 3D porous V2O5 architectures for high-rate lithium storage显示文摘The discovery of novel electrode materials promises to unleash a number of technological advances in lithium-ion batteries.V2O5 is recognized as a high-performance cathode that capitalizes on the rich redox chemistry of vanadium to store lithium.To unlock the full potential of V2O5,nanotechnology solution and rational electrode design are used to imbue V2O5 with high energy and power density by addressing some of their intrinsic disadvantages in macroscopic crystal form.Here,we demonstrate a facile and environmental-friendly method to prepare nanorods-constructed 3D porous V2O5 architectures(3 D-V2O5)in large-scale.The 3D porous architecture is found to be responsible for the enhanced charge transfer kinetics and Li-ion diffusion rate of the 3D-V2O5 electrode.As the result,the 3D-V2O5 surpasses the conventional bulk V2O5 by showing enhanced discharge capacity and rate capability(delivering 154 and 127 m Ah g^-1 at 15 and 20 C,respectively). | Qifei Li Dong Chen Huiteng Tana Xianghua Zhang Xianhong Rui Yan Yu | 2020 | Journal of Energy Chemistry2020，29，1： | 1 |
| 16 | Improved Pretreatment (Coagulation-Floatation and Ozonation) of Younger Landfill Leachate by Microbubbles显示文摘 | Liu Shu Wang Qunhui Zhai Xuedong Huang Qifei Huang Peikun | 2010 | Water Environment Research2010，，7： | 1 |
| 17 | Hazardous waste generation and management in China: a review 显示文摘 | DUAN Huabo HUANG Qifei WANG Qi | 2008 | Journal of Hazardous Materials2008，158，2： | 1 |
| 18 | Laparoscopic approach for intermittent hydronephrosis caused by primary ureteral fibroepithelial polyps in children显示文摘Objective To summarize the diagnosis and treatment experience of children with intermittent hydronephrosis caused by ureteral fibroepithelial polyp(UFP).Methods From 2017 to 2020,cases of hydronephrosis caused by ureteral polyp in Anhui Provincial Children’s Hospital were retrospectively enrolled for investigation.Demographic data,clinical manifestations,operation details,pathology and outcomes were collected from patients’medical data for analysis.Results All seven cases of UFP were boys,including six cases on the left side of the ureter and one case on the right side,at the median age of 7.1 years(3-14 years),with abdominal intermittent pain as the first symptom.All cases underwent laparoscopic pyeloureteroplasty.All the operations were completed successfully;postoperative pathology indicated the presence of primary UFP.Postoperative follow-ups of 1-30 months showed satisfactory recovery and relief from hydronephrosis.Conclusions Laparoscopic pyeloureteroplasty or ureteroureterostomy is one of the optimal treatments for ureteral polyp at present.The surgical method should be determined according to the number of polyps,the length and the diameter of the affected ureter,and also the status of renal function of the patients. | Han Chu Yongsheng Cao Qifei Deng | 2021 | World Journal of Pediatric Surgery2021，4，1： | 1 |
| 19 | Histology and antitumor activity study of PTX-loaded micelle,a fluorescent drug delivery system prepared by PEG-TPP显示文摘We synthesized PEG-TPP as carrier to encapsulate paclitaxel (PTX) in the form of micelles to overcome its water-solubility problem. PTX-loaded micelles possess a-week stability and appropriate particle size (152.1 ±1.2 nm) which is beneficial for enhanced permeability and retention (EPR) effect. Strong pH dependence of PTX releasing from micelles is verified by in vitro release study. At cellular level, PTX-loaded micelles can target mitochondria effectively which may results a better cytotoxicity of micelles (especially IC50 = 0.123 ± 0.035μmol/L of micelles and 0.298 ± 0.067μmol/L of PTX alone on MCF-7 cells). The fluorescence distributions of both isolated and sliced organs show that the micelles can effectively target tumors. Moreover, we further prove the enhanced therapeutic effects of micelles in tumor-bearing mice comparing with PTX alone. The results show that the biodegradable drug delivery system prepared by PEG-TPP can overcome the poor solubility of paclitaxel and improve its tumor targeting and antitumor activity. | Huilan Li Jieming Li Xinyi He Bo Zhang Chunxia Liu Qifei Li Ying Zhu Wenlong Huang Wei Zhang Hai Qian Liang Ge | 2019 | Chinese Chemical Letters2019，30，5： | 1 |
| 20 | One-Pot Three-Dimensional Printing Robust Self-Supporting MnO_(x)/Cu-SSZ-13 Zeolite Monolithic Catalysts for NH_(3)-SCR显示文摘Honeycomb cordierite coated with Cu-SSZ-13 zeolite is widely used for the selective catalytic reduction of NO_(x) with NH_(3)(NH_(3)-SCR)to reduce pollutants from vehicle emissions.However,conventional honeycomb catalysts fabricated via coating techniques are limited by low zeolite loadings,loss of the deposited zeolites,and complicated preparation processes.Herein,a facile,one-step three-dimensional(3D)printing strategy is developed to construct MnO_(x)/Cu-SSZ-13 monolithic catalysts with excellent catalytic performance for NH_(3)-SCR.Iron-containing halloysite nanotubes(Fe-HNTs)are introduced as printing ink additives to ensure mechanical stability and modulate the NH_(3)-SCR performance of monolithic catalysts in high temperature conditions.In situ incorporation of Mn into the Cu-SSZ-13 zeolite monoliths during the 3D printing process boosts the mechanical strength of the monolithic structures from 2.54 MPa to 4.33 MPa as well as broadens the temperature window(165-550℃)of the catalysts for NH_(3)-SCR with NO_(x) conversion of above 80%.Such robust multicomponent-integrated 3D-printed selfsupporting catalysts not only possess high zeolite loading and excellent catalytic activity,but also avoid complicated manufacturing processes,which contrasts with conventional honeycomb catalysts fabricated by extrusion coupled with coating. | Yingzhen Wei Mengyang Chen Xiaoyu Ren Qifei Wang Jinfeng Han Wenzheng Wu Xiangguang Yang Shuang Wang Jihong Yu | 2022 | CCS Chemistry2022，4，5： | 1 |
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