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| 1 | Features of Sandy Debris Flows of the Yanchang Formation in the Ordos Basin and Its Oil and Gas Exploration Significance显示文摘Sandy debris flow is a new genetic type of sand bodies,which has gained much attention in recent years and its corresponding theory is proved to be a significant improvement and even partial denial to the 'Bouma Sequence' and 'turbidite fan' deep-water sedimentary theories to some point. Oil exploration researchers are highly concerned with sandy debris flows for its key role in controlling oil and gas accumulation processes.In this article,by applying sandy debris flows theory and combining a lot work o... | LI Xiangbo CHEN Qilin LIU Huaqing WAN Yanrong WEI Lihua LIAO Jianbo LONG Liwen | 2011 | Acta Geologica Sinica(English Edition)2011，85，5： | 24 |
| 2 | Current status of diagnosis and treatment of bladder cancer in China-Analyses of Chinese Bladder Cancer Consortium database显示文摘Objective:To investigate current status of diagnosis and treatment of bladder cancer in China.Methods:A database was generated by Chinese Bladder Cancer Consortium(CBCC).From January 2007 to December 2012,14,260 cases from 44 CBCC centers were included.Data of diagnosis,treatment and pathology were collected.Results:The average age was 63.5 year-old and most patients were male(84.3%).The most common histologic types were urothelial carcinoma(91.4%),adenocarcinoma(1.8%),and squamous carcinoma(1.9%).According to 1973 and 2004 WHO grading system,42.0%,41.0%,and 17.0% of patients were grade 1,2,and 3,and 16.0%,48.7%,and 35.3% of patients were papillary urothelial neoplasms of low malignant potential,low,and high grade,respectively.Non-muscle invasive bladder cancer(NMIBC)and muscle invasive bladder cancer(MIBC)were 25.2% and 74.1%,respectively(0.8% not clear).Carcinoma in situ was only 2.4%.Most patients were diagnosed by white-light cystoscopy with biopsy(74.3%).Fluorescence and narrow band imaging cystoscopy had additional detection rate of 1.0% and 4.0%,respectively.Diagnostic transurethral resection(TUR)provided detection rate of 16.9%.Most NMIBCs were treated with TUR(89.2%).After initial TUR,2.6%accepted second TUR,and 45.7%,69.9%,and 58.7% accepted immediate,induced,and maintenance chemotherapy instillation,respectively.Most MIBCs were treated with radical cystectomy(RC,59.7%).Laparoscopic RCs were 35.1%,while open RC 63.4%.Extended and standard pelvic lymph node dissection were 7% and 66%,respectively.Three most common urinary diversions were orthotopic neobladder(44%),ileal conduit(31%),and ureterocutaneostomy(23%).Only 2.3% of patients accepted neo-adjuvant chemotherapy and only 18%of T3 and T4 patients accepted adjuvant chemotherapy.Conclusion:Disease characteristics are similar to international reports,while differences of diagnosis and treatment exist.This study can provide evidences for revisions of the guideline on bladder cancer in China. | Kaiwen Li Tianxin Lin 无 Wei Xue Xin Mu Enci Xu Xu Yang Fubao Chen Guangyong Li Lulin Ma Guoliang Wang Chaozhao Liang Haoqiang Shi Ming Li Mao Tang Xueyi Xue Yisong Lv Yaoliang Deng Chengyang Li Zhiwen Chen Xiaozhou Zhou Fengshuo Jin Xudong Liu Jinxin Wei Lei Shi Xin Gou Weiyang He Liqun Zhou Lin Cai Baiye Jin Guanghou Fu Xiangbo Kong Hongyan Sun Ye Tian Lang Feng Tiejun Pan Yiyi Wu Dongwen Wang Hailong Hao Benkang Shi Yaofeng Zhu Qiang Wei Ping Han Changli Wu Dawei Tian Zhangqun Ye Zheng Liu Zhiping Wang Junqiang Tian Lin Qi Minfeng Chen Wei Li Jinchun Qi Gongxian Wang Longlong Fu Zhaolin Sun Guangheng Luo Zhoujun Shen Zhaowei Zhu Jinchun Xing Zhun Wu Dong Wei Xin Chen Yanqun Na Hongfeng Guo Chunxi Wang Zhihua Lu Chuize Kong Yang Liu Jin Yang Jianyun Hu Xin Gao Jielin Li Changjun Yin Pu Li Shan Chen Zhen Du Jiongming Li Yongji Yan Xu Zhang Shuang Huang Fangjian Zhou Zhiling Zhang Yinghao Sun Shuxiong Zeng Song Cen Jiaquan Zhou Hanzhong Li Jin Wen Jian Huang | 2015 | Asian Journal of Urology2015，2，2： | 21 |
| 3 | Prostate cancer in Asia:A collaborative report显示文摘The incidence of prostate cancer(PCa)within Asian population used to be much lower than in the Western population;however,in recent years the incidence and mortality rate of PCa in some Asian countries have grown rapidly.This collaborative report summarized the latest epidemiology information,risk factors,and racial differences in PCa diagnosis,current status and new trends in surgery management and novel agents for castration-resistant prostate cancer.We believe such information would be helpful in clinical decision making for urologists and oncologists,health-care ministries and medical researchers. | Rui Chen Shancheng Ren 无 Ming Kwong Yiu Ng Chi Fai Wai Sam Cheng Lap Hong Ian Seiji Naito Tadashi Matsuda Elijah Kehinde Ali Kural Jason Yichun Chiu Rainy Umbas Qiang Wei Xiaolei Shi Liqun Zhou Jian Huang Yiran Huang Liping Xie Lulin Ma Changjun Yin Danfeng Xu Kexin Xu Zhangqun Ye Chunxiao Liu Dingwei Ye Xin Gao Qiang Fu Jianquan Hou Jianlin Yuan Dalin He Tiejun Pan Qiang Ding Fengshuo Jin Benkang Shi Gongxian Wang Xiuheng Liu Dongwen Wang Zhoujun Shen Xiangbo Kong Wanhai Xu Yaoliang Deng Haibo Xia Alexa NCohen Xu Gao Chuanliang Xu Yinghao Sun | 2014 | Asian Journal of Urology2014，1，1： | 13 |
| 4 | Identification of sex phero-mones of four economically important species in genus Dendrolimus显示文摘The female-produced sex pheromone of Den-drolimus superans was identified by gas chromatography (GC), coupled GC-mass spectrometry (GC-MS), electroan-tennographic (EAG) studies and field tests as a blend of (Z,E)-5,7-dodecadienal (Z5,E7-12:Ald) and (Z,E)-5,7-dodeca-dien-1-ol (Z5,E7-12:OH). In D. kikuchii, (Z,E)-5,7-dodeca-dien-1-yl acetate (Z5,E7-12:OAc) and Z5,E7-12:OH were found by GC and GC-MS analyses. However, in EAG studies male antennae were more sensitive to Z5,E7-12:OAc and (Z,E)-5,7-dodecadien-l-yl propionate (Z5,E7-12:OPr) than Z5,E7-12:OH. For D. spectabilis, Z5,E7-12:OH had been previously reported as the sex pheromone. However, in our studies, traps baited with Z5,E7-12:OH, Z5,E7-12:OAc and Z5,E7-12:OPr in a ratio of 1:1:1 caught three times more males than those baited with Z5,E7-12:OH alone. Relatively strong EAG responses were elicited from male antennae by Z5,E7-12:OH, Z5,E7-12:OAc and Z5,E7-12:OPr, but in addition to Z5,E7-12:OH, only very small amounts of Z5,E7-12:OAc was found in | Kong Xiangbo Zhao Chenghua Gao Wei | 2001 | Chinese Science Bulletin2001，46，24： | 12 |
| 5 | Genesis of the high gamma sandstone of the Yanchang Formation in the Ordos Basin,China显示文摘Recently, more attention has been paid on the high gamma sandstone reservoirs of the Yanchang Formation in the Ordos Basin, China. These high gamma sandstones have logging characteristics different from conventional sandstones, which influences the identification of sandstone reservoirs. Zhang et al (2010) proposed that the high gamma sandstones of the Yanchang Formation might be the result of re-deposition of homochronous sedimentary tuffs or previous tuffs as a part of the sandstone. However, we present a different viewpoint: 1) few tuffs or tuff debris have been found in the high gamma sandstones of the Yanchang Formation; 2) high gamma (or high Th content) sandstones of Yanchang Formation are not related to either clay minerals or feldspar; 3) the heavy minerals in the sandstone reservoirs of the Yanchang Formation are dominated by zircon, which is characterized by abnormally high Th and U contents, up to 2,163 ppm and 1,362 ppm, respectively. This is sufficient to explain the high gamma anomaly. The conclusion is that the high gamma value of the Yanchang Formation sandstones might be caused by zircon with high Th and U contents in sandstones rather than from the tuff components. | Liu Huaqing Li Xiangbo Liao Jianbo Liu Xianyang | 2013 | Petroleum Science2013，10，1： | 11 |
| 6 | Tectonic Evolution of the Tianhuan Depression and the Western Margin of the Late Triassic Ordos显示文摘The Ordos Basin is one of the most important oil and gas basins in China. Based on surface outcrop, key exploratory wells and seismic reflection data and by using the technology of 'prototype basin recovery', seismic profile 'layer flattening' and 'restoration of balanced section',and other methods, the sedimentary boundary, structure and the evolution history of the Tianhuan depression on the western margin of the Ordos Basin are reestablished. The following results have been obtained. (1) The west boundary of the Late Triassic Ordos Basin was far beyond the scope of the current basin. The basin is connected with the Late Triassic Hexi Corridor Basin, and its western margin did not have tectonic characteristics of a foreland basin. (2) The Tianhuan depression was first formed in the Late Jurassic. At the late stage it was impacted by the late Yanshanian and Himalayan tectonic movement and the depression axis gradually moved eastwards to the present location with a cumulative migration distance of ~30 km. (3) Eastward migration of the depression axis caused adjustment and even destruction of the originally formed oil and gas reservoirs, so that oil and gas remigrated and aggregated, resulting in secondary structural reservoirs formed at high positions on the western flank of the depression. | LI Xiangbo LIU Huaqing WANYAN Rong WEI Lihua LIAO Jianbo FENG Ming MA Yuhu BAI Yunlai | 2009 | Acta Geologica Sinica(English Edition)2009，83，6： | 9 |
| 7 | Overexpression of the Wounding-Responsive Gene AtMYB15 Activates the Shikimate Pathway in Arabidopsis显示文摘MYB 抄写因素基因在许多发展过程和植物的各种各样的防卫回答起重要作用。shikimate 小径是为三芳香的氨基酸和涉及植物的多重回答的另外的芳香的混合物的生产的一条主要 biosynthetic 小径,包括保护对紫外并且防卫。此处,我们在 Arabidopsis 把 R2R3-MYB 基因 AtMYB15 的描述描述为 shikimate 小径的使活跃之物。AtMYB15 蛋白质是原子的局部性并且一个 transcriptional 激活领域在它的 C 终端部分被发现。北污点证明 AtMYB15 是早创伤可诱导的基因。microarray 分析的 Resutls,使用量的即时聚合酶链反应证实,证明在转基因的植物的 AtMYB15 的 overexpression 导致了涉及 shikimate 小径的几乎所有基因的提高的表示。生物信息学分析证明至少一个 AtMYB15 有约束力的交流元素在这些 upregulated 基因的倡导者被检测。而且,在 shikimate 小径的这些基因也被发现被伤害导致。这些数据响应伤害作为 Arabidopsis shikimate 小径的一个可能的直接管理者建议 AtMYB15 的一个重要角色。 | Yanhui Chen Xiangbo Zhang Wei Wu Zhangliang Chen Hongya Gu Li-Jia Qu | 2006 | Journal of Integrative Plant Biology2006，48，9： | 7 |
| 8 | Alpha-2-macroglobulin as a radioprotective agent: a review显示文摘Radiation is an important modality in cancer treatment, and eighty percent of cancer patients need radiotherapy at some point during their clinical management. However, radiation-induced damage to normal tissues restricts the therapeutic doses of radiation that can be delivered to tumours and thereby limits the effectiveness of the treatment. The use of radioprotectors represents an obvious strategy to obtain better tumour control using a higher dose in radiotherapy. However, most of the synthetic radioprotective compounds studied have shown inadequate clinical efficacy owing to their inherent toxicity and high cost. Hence, the development of radioprotective agents with lower toxicity and an extended window of protection has attracted a great deal of attention, and the identification of alternative agents that are less toxic and highly effective is an absolute necessity. Recent studies have shown that alpha-2-macroglobulin(α2M) possesses radioprotective effects. α2M is a tetrameric, disulfide-rich plasma glycoprotein that functions as a nonselective inhibitor of different types of non-specific proteases and as a carrier of cytokines, growth factors, and hormones. α2M induces protein factors whose interplay underlies radioprotection, which supports the idea that α2M is the central effector of natural radioprotection in the rat. Pretreatment with α2M has also induced a significant reduction of irradiation-induced DNA damage and the complete restoration of liver and body weight. Mihailovi? et al. concluded that the radioprotection provided by α2M was in part mediated through cytoprotection of new blood cells produced in the bone marrow; these authors also indicated that an important aspect of the radioprotective effect of amifostine was the result of the induction of the endogenous cytoprotective capability of α2M. The radioprotective effects of α2M are possibly due to antioxidant, antifibrosis, and anti-inflammatory functions, as well as the maintenance of homeostasis, and enhancement of the DNA repair and cell recovery processes. This review is the first to summarise the observations and elucidate the possible mechanisms responsible for the beneficial effects of α2M. The lacunae in the existing knowledge and directions for future research are also addressed. | Xueying Chen Xiangbo Kong Zhaoqiang Zhang Wei Chen Jieyu Chen Huanyang Li Wanting Cao Yaping Ge Silian Fang | 2014 | Chinese Journal of Cancer Research2014，26，5： | 7 |
| 9 | Development of typhoon driven wave nowcasting model in Southeast China Sea显示文摘Using optimal interpolation data assimilation of observed wave spectrum around Northeast coast of Taiwan Island, the typhoon driven wave nowcasting model in Southeast China Sea is setup. The SWAN (simulating waves nearshore) model is used to calculate wave field and the input wind field is the QSCAT/NCEP (Quick Scatterometer/National Centers for Environmental Prediction) data. The two-dimensional wavelet transform is applied to analyze the X-band radar image of nearshore wave field and it reveals that the observed wave spectrum has shoaling characteristics in frequency domain. The reverse calculation approach of wave spectrum in deep water is proposed and validated with experimental tests. The two-dimensional digital low-pass filter is used to obtain the initialization wave field. Wave data during Typhoon Sinlaku is used to calibrate the data assimilation parameters and test the reverse calculation approach. Data assimilation corrects the significant wave height and the low frequency spectra energy evidently at Beishuang Station along Fujian Province coast, where the entire assimilation indexes are positive in verification moments. The nowcasting wave field shows that the present model can obtain more accurate wave predictions for coastal and ocean engineering in Southeast China Sea. | Zheng Jinhai Feng Xiangbo Yan Yixin | 2011 | Engineering Sciences2011，9，1： | 7 |
| 10 | Crystal structure of SARS-CoV-2 main protease in complex with protease inhibitor PF-07321332显示文摘Dear Editor,Since December 2019,the pandemic of coronavirus disease 2019(COVID-19)has taken a heavy toll on global health,creating an urgent need to develop effective strategies for prevention and treatment.The etiological agent,known as severe acute respiratory syndrome coronavirus 2(SARSCoV-2),has infected nearly 229.2 million people worldwide with more than 4.7 million deaths as of September 15,2021.Older age and preexisting health conditions are associated with worse clinical prognosis including higher mortality rates(Zhou et al.,2020).The global race to combat this pandemic has led to rapid deployment of numerous effective vaccines against SARS-CoV-2(Tregoning et al.,2021).However,the emergence of viral variants,including the Delta variant(B.1.617.2),compromised vaccine effectiveness with resurgence of SARS-CoV-2 infection among highly vaccinated population(Keehner et al.,2021).Therefore,development of therapeutics against the more conserved viral targets would be essential to contain the spread of COVID-19 and reduce mortality. | Yao Zhao Chao Fang Qi Zhang Ruxue Zhang Xiangbo Zhao Yinkai Duan Haofeng Wang Yan Zhu Lu Feng Jinyi Zhao Maolin Shao Xiuna Yang Leike Zhang Chao Peng Kailin Yang Dawei Ma Zihe Rao Haitao Yang | 2022 | Protein & Cell2022，13，9： | 6 |
| 11 | Effect of Salt Spray Corrosion on Tribological Properties of HVOF Sprayed NiCr-Cr3C2 Coating with Intermediate Layer显示文摘The objective of the present work was to determine the influence of the neutral salt spray corrosion on the wear resistance of HVOF sprayed NiCr-Cr_3C_2 coating with intermediate layer. Ni-Zn-Al_2O_3 coatings as interlayers were prepared by low pressure cold spray(LPCS) between NiCr-Cr_3C_2 cermet coatings to form a sandwich structure to enhance the corrosion resistance properties. The tribological properties were examined using the UMT-3 fricition and wear tester by line-contact reciprocating sliding under dry and salt spray one week corrosion. The morphology, element distribution, and phase compositions of the coating and worn sufaces were analyzed by using scanning electron microscopy, energy dispersive spectrometry, and X-ray diffraction respectively. The corrosion behavior of the coating was studied by the open-circuit potential, the electrochemical impedance spectroscopy, potentiodynamic polarization, and salt spray corrosion methods. It is found that the sandwich structured coating has better corrosion resistance than the single layer coating. The results show that under dry wear conditions, the wear mechanism is abrasive and adhesive wear, whereas under salt spray corrosion conditions it becomes corrosion wear. The friction coefficient of the sandwich structured coating after salt spray corrosion is slightly lower than the dry friction coefficient, but the weight of the wear loss is lower than that under dry condition. | 白杨 LI Xiangbo XING Lukuo 李焰 | 2017 | Journal of Wuhan University of Technology(Materials Science)2017，32，2： | 6 |
| 12 | Progress and key challenges in catalytic combustion of lean methane显示文摘As a primary type of clean energy,methane is also the second most important greenhouse gas after CO_(2)due to the high global warming potential.Large quantities of lean methane(0.1–1.0 vol%)are emitted into the atmosphere without any treatment during coal mine,oil,and natural gas production,thus leading to energy loss and greenhouse effect.In general,it is challenging to utilize lean methane due to its low concentration and flow instability,while catalytic combustion is a vital pathway to realize an efficient utilization of lean methane owing to the reduced emissions of polluting gases(e.g.,NOxand CO)during the reaction.In particular,to efficiently convert lean methane,it necessitates both the designs of highly active and stable heterogeneous catalysts that accelerate lean methane combustion at low temperatures and smart reactors that enable autothermal operation by optimizing heat management.In this review,we discuss the in-depth development,challenges,and prospects of catalytic lean methane combustion technology in various configurations,with particular emphasis on heat management from the point of view of material design combined with reactor configuration.The target is to describe a framework that can correlate the guiding principles among catalyst design,device innovation and system optimization,inspiring the development of groundbreaking combustion technology for the efficient utilization of lean methane. | Xiangbo Feng Lei Jiang Danyang Li Shaopeng Tian Xing Zhu Hua Wang Chi He Kongzhai Li | 2022 | Journal of Energy Chemistry2022，，12： | 4 |
| 13 | Atypical clinical and pathological findings in a patient with isolated cortical vein thrombosis显示文摘Isolated cortical vein thrombosis often produces a focal lesion. Because of the rapid development of collateral circulation, increased intracranial pressure has never been reported in a patient with isolated cortical vein thrombosis. The diagnosis of isolated cortical vein thrombosis is based mainly on MRI, catheter digital subtraction angiography, and histological findings, but may be challenging. We report a patient who presented with intermittent seizures and left-sided limb weakness. Her symptoms gradually progressed, and she eventually developed signs of increased intracranial pressure. Imaging studies showed a space-occupying lesion in the right frontal lobe of the brain. As we could not diagnose isolated cortical vein thrombosis based on the preoperative findings, surgical excision of the lesion was performed under general anesthesia. Histological examination showed destruction of the brain parenchyma with infiltration of macrophages, proliferation of reactive astrocytes and small vessels, and foci of hemorrhage. Further examination found that a number of small vessels in both the subarachnoid space and brain parenchyma were filled with thrombus, some of which was organized. Elastic fiber staining showed that the obstructed vessels were veins. We diagnosed isolated cortical vein thrombosis with atypical clinical features. | Yan Ding Vance Fredrickson Yicong Lin Yueshan Piao Xiangbo Wang Dehong Lu Cunjiang Li | 2012 | Neural Regeneration Research2012，7，31： | 3 |
| 14 | OS1 functions in the allocation of nutrients between the endosperm and embryo in maize seeds显示文摘Uncovering the genetic basis of seed develop-ment will provide useful tools for improving both crop yield and nutritional value, However, the genetic regulatory networks of maize (Zea mays) seed development remain largely unknown. The maize opaque endosperm and small germ 1 (osl) mutant has opaque endosperm and a small embryo,Here, we cloned OSi1 and show that it encodes a putative transcription factor containing an RWP-RK domain-Transcriptional analysis indicated that OSi1 expression is elevated in early endosperm development, especially in the basal endosperm transfer layer (BETL), conducting zone (CZ), and central starch endospcrm (CSE) cells. RNA sequencing (RNA-Seq) analysis of the osi mutant revealed sharp downregulation of certain genes in specific cell types, including ZmMRP-1 and Megl in BETL cells and a majority of zein-and starch-related genes in CSE cells. Using a haploid induction system, we show that wild-type endosperm could rescue the smaller size of osi embryo, which suggests that nutrients are allocated by tho wild type endosperm. Therefore, our dsta imply that the network regulated by 051 accomplishes a key step in nutrient allocation between endosperm and embryo within maize seeds. Identification of this network will help uncover the mechanisms regulating the nutritional balance between endosperm and embryo. | Weibin Song Jinjie Zhu Haiming Zhao Yingnan Li Jiangtao Liu Xiangbo Zhang Liangliang Huang Jinsheng Lai | 2019 | Journal of Integrative Plant Biology2019，61，6： | 3 |
| 15 | Extraordinary characteristics for one-dimensional parity-time-symmetric periodic ring optical waveguide networks显示文摘In this paper, we design a one-dimensional(1D) parity-time-symmetric periodic ring optical waveguide network(PTSPROWN) and investigate its extraordinary optical characteristics. It is found that quite different from traditional vacuum/dielectric optical waveguide networks, 1D PTSPROWN cannot produce a photonic ordinary propagation mode, but can generate simultaneously two kinds of photonic nonpropagation modes: attenuation propagation mode and gain propagation mode. It creates neither passband nor stopband and possesses no photonic band structure. This makes 1D PTSPROWN possess richer spontaneous PT-symmetric breaking points and causes interesting extremum spontaneous PT-symmetric breaking points to appear, where electromagnetic waves can create ultrastrong extraordinary transmission, reflection, and localization, and the maximum can arrive at 6.6556 × 10^(12) and is more than 7 orders of magnitude larger than the results reported previously.1D PTSPROWN may possess potential in designing high-efficiency optical energy saver devices, optical amplifiers, optical switches with ultrahigh monochromaticity, and so on. | YAN ZHI XIANGBO YANG JIAYE WU SHIPING DU PEICHAO CAO DONGMEI DENG CHENGYI TIMON LIU | 2018 | Photonics Research2018，6，6： | 2 |
| 16 | Development of Al_2O_3/TiN Ceramie Cutting Tool Materials by Artificial Neural Networks显示文摘The artificial neural networks (ANN) which have broad application were proposed to develop multiphase ceramic cutting tool materials. Based on the back propagation algorithm of the forward multilayer perceptron, the models to predict volume content of composition in particle reinforced ceramics are established. The Al2O3/TiN ceramic cutting tool material was developed by ANN, whose mechanical properties fully satisfy the cutting requirements. | Ning FAM, Xiangbo ZE and Zihui GAOSchool of Mechanical Engineering, Jinan University, Jinan 250022, China | 2004 | Journal of Materials Science & Technology2004，20，6： | 2 |
| 17 | Preparation of freestanding palladium nanosheets modified with gold nanoparticles at edges显示文摘电子调整是最通常使用的策略之一改进异构的催化剂的催化表演。我们准备了六角形的 ultrathin Pd nanosheets,边用流电的代替方法由金 nanoparticles (Au@Pd nanosheets ) 修改了。由在 Pd nanosheets 和 Au nanoparticles 之间的电子相互作用的优点, Au@Pd nanosheets 由碳一氧化物在 iodobenzene 的 carbonylation 展出了优秀催化表演。新奇 nanocomposites 能作为模型催化剂被使用在催化作用探索电子效果。 | Xiangbo Zhang Chao Lian Zheng Chen Chen Chen Yadong Li | 2018 | Nano Research2018，11，8： | 2 |
| 18 | Sulfonic groups functionalized Zr-metal organic framework for highly catalytic transfer hydrogenation of furfural to furfuryl alcohol显示文摘The highly selective catalytic transfer hydrogenation(CTH)of furfural(FF)to furfuryl alcohol(FOL)is a significant route of biomass valorization.Herein,a series microporous Zr-metal organic framework(ZrMOF)functionalized by sulfonic groups are prepared.Based on the comprehensive structural characterizations by means of X-ray diffraction(XRD),scanning electron microscopy(SEM),transmission electron microscopy(TEM),N2 physisorption,Thermogravimetric(TG)and Fourier transformed infrared spectroscopy(FTIR),we find that sulfonic acid(–SO_(3)H)functional groups are tethered on the UIO-66 without affecting the structure of the framework.Systematic characterizations(NH_(3)-TPD,CO_(2)-TPD,and in-situ FTIR)demonstrate that modifying of sulfonic groups on UIO-66 results in the formation of stronger Lewis acidic-basic and Brnsted acidis sites.The cooperative role of the versatile Lewis acidic-basic and Brnsted acidic sites in 60%mol fraction of sulfonic acid-containing UIO-66(UIO-S_(0.6))retain high surface area and exhibit excellent catalytic performance of 94.7%FOL yield and 16.9 h^(-1).turnover number(TOF)under mild conditions.Kinetic experiments reveal that the activation energy of the CTH of furfural(FF)over UIO-S_(0.6) catalyst is as low as 50.8 k J mol^(-1).Besides,the hydrogen transfer mechanism is investigated through isotope labeling experiments,exhibiting that theβ-H in isopropanol is transferred to the a-C of FF by forming six-membered intermediates on the Lewis acidic-basic and Brnsted acidic sites of the UIO-S_(0.6),which is the rate-determining step in the formation of FOL. | Jingcheng Wu Dong Liang Xiangbo Song Tingsen Liu Tianyi Xu Shuangyin Wang Yuqin Zou | 2022 | Journal of Energy Chemistry2022，31，8： | 2 |
| 19 | Thermal De- composition of Y3AI5Oa2 Precursor Synthesized by Urea Homo- geneous Co-Precipitation 显示文摘 | Ji Xiangbo Deng Jianguo Kang Bin | 2013 | JAnal Appl Pyrolysis2013，104，11： | 1 |
| 20 | Fine-scale activity patterns of large-and medium-sized mammals in a deciduous broadleaf forest in the Qinling Mountains,China显示文摘The composition of animal species and interactions among them are widely known to shape ecological communities and fine-scale(e.g.,<1 km)monitoring of animal communities is essential for understanding the relationships among animals and plants.Although the co-existence of large-and medium-sized species has been studied across different scales,research on fine-scale interactions of herbivores in deciduous broadleaf forests is limited.Camera trapping of large-and medium-sized mammals was carried out over a 1 year period within a 25 ha deciduous broadleaf forest dynamics plot in the Qinling Mountains,China.Fourteen species of large-and medium-sized mammals,including six carnivores,six ungulates,one primate and one rodent species were found.Kernel density estimations were used to analyse the diel or 24 h activity patterns of all species with more than 40 independent detections and general linear models were developed to explore the spatial relationships among the species.The combination of overlapping diel activity patterns and spatial associations showed obvious niche separation among six species:giant panda(Ailuropoda melanoleuca David),takin(Budorcas taxicolor Hodgson),Reeves’s muntjac(Muntiacus reevesi Ogilby),tufted deer(Elaphodus cephalophus Milne-Edwards),Chinese serow(Capricornis milneedwardsii David)and wild boar(Sus scrofa Linnaeus).Long-term fine-scale monitoring is useful for providing information about the co-existence of species and their interactions.The results demonstrate the importance for fine-scale monitoring of animals and plants for improving understanding of species interactions and community dynamics. | Yuke Zhang Xiangbo He Xuehua Liu Melissa Songer Haishan Dang Quanfa Zhang | 2021 | Journal of Forestry Research2021，32，6： | 1 |
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