|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Natural^(15)N abundance in soils and plants in relation to N cycling in a rangeland in Inner Mongolia显示文摘Aims Natural 15N abundance provides integrated information about nitrogen(N)input,transformation and output,indirectly reflecting N cycling traits within terrestrial ecosystems.However,relationships between natural 15N abundance and N cycling processes are poorly understood in China.Here,our primary objectives were to(i)examine the effects of grazing at varying levels of intensity on d15N of soils and plants in a semi-arid grassland;(ii)detect the relationships between d15N of soils and four major N cycling processes(i.e.mineralization,nitrification,denitrification and ammonia volatilization);and(iii)determine whether d15N of soils can be used as an indicator of N cycling in this semi-arid grassland.Methods The field experiment was conducted within the long-term(17-year)grazing enclosures in a semi-arid grassland in Inner Mongolia.Five grazing intensities(0.00,1.33,2.67,4.00 and 5.33 sheep ha1)were designed.d15N values of topsoils(0–10 cm),surface soils(0–2 cm)and plants were measured in 2006.Differences in d15N of soils and plants between the five grazing intensities were examined.Rates of four soil N cycling processes were measured periodically during the 2005 and 2006 growing seasons.The d15N values of topsoils were linked to the four N cycling processes to investigate their relationships.Important Findings The d15N values of topsoils(5.20–5.96&)were substantially higher than the d15N values of plants(2.51–2.93&)and surface soils(1.44–2.92&)regardless of grazing intensities.The 15N-depleted N losses during microbial decomposition of organic matter in concert with the downward movement of residual substrate over time are the possible causes of higher d15N values in topsoils than in surface soils.In addition,the d15N values of topsoils were positively correlated with the d15N values of both plants and surface soils.Grazing,especially the high-intensity grazing(5.33 sheep ha1),resulted in a significant decrease in d15N of surface soils.However,no statistically significant variations in d15N of topsoils and plants were found in response to grazing.The d15N values of topsoils exhibited significant dependence on the cumulative rates of NH3 volatilization,net nitrification and denitrification in 2005 but not in 2006. | Yuqing Xu Jicheng He Weixin Cheng Xuerong Xing Linghao Li | 2010 | Journal of Plant Ecology2010，3，3： | 12 |
| 2 | Socio-economic driving forces of arable land conversion: A case study of Wuxian City, China显示文摘 | Yichun Xie Yu Mei Tian Guangjin Xing Xuerong | 2005 | Global Environmental Change2005，，3： | 1 |
| 3 | Temperature and soil moisture interactively affected soil net N mineralization in temperate grassland in Northern China显示文摘 | Changhui Wang Shiqiang Wan Xuerong Xing Lei Zhang Xingguo Han | 2005 | Soil Biology and Biochemistry2005，，5： | 1 |
| 4 | Fabrication of amorphous PdNiCuP nanoparticles as efficient bifunctional and highly durable electrocatalyst for methanol and formic acid oxidation显示文摘Highly active and durable electrocatalytic materials towards small molecules electro-oxidation reaction are critical to the large-scale commercial applications of direct liquid fuel cells.Unfortunately,current nanocrystalline electrocatalysts normally suffer from low catalytic efficiency,severe CO poisoning and rapid activity decay.Herein,we report a novel amorphous Pd Ni Cu P catalyst synthesized with laser liquid ablation as a potential settlement to this issue.The as-obtained amorphous Pd Ni Cu P catalyst exhibits enhanced electrocatalytic performance with the mass activity of 1.61 A mg^(-1)and 737.8 m A mg^(-1)towards methanol oxidation reaction(MOR)and formic acid oxidation reaction(FAOR),respectively.Moreover,amorphous Pd Ni Cu P displays excellent operation stability and CO-poisoning resistance in both alkaline and acidic medium.P was proposed to play the decisive role for forming the amorphous structure and maintaining the catalytic stability in MOR and FAOR processes.This work provided insights for the ration design of active and durable amorphous electrocatalysts applied in direct liquid fuel cells. | Yunwei Liu Chang Liu Zelin Chen Xuerong Zheng Rui Jiang Xing Tong Yida Deng Wenbin Hu | 2022 | Journal of Materials Science & Technology2022，，27： | 0 |
| 5 | Facile fabrication of ultrafine nickel-iridium alloy nanoparticles/graphene hybrid with enhanced mass activity and stability for overall water splitting显示文摘Developing active and durable electrocatalysts for overall water splitting is desirable but challenging to realize sustainable hydrogen production.Here,we report a facile and general method to prepare ultrafine nickel(Ni)-iridium(Ir)alloy nanoparticles/graphene hybrids for overall water splitting.The optimized hybrid with 4.9 wt%Ir exhibits much higher catalytic activity and durability than commercial 20 wt%Ir/C for both oxygen evolution reaction(OER)and hydrogen evolution reaction(HER).Theoretical simulations reveal that the incorporation of Ir in metallic Ni lattice regulates hydrogen adsorption free energy to the optimum level,thus improving HER activity,while in situ generated amorphous Ir-Ni hydr(oxy)oxides around metallic Ni-Ir core have been demonstrated to be the active species under OER conditions,which switches OER rate-determining step to energy-favorable pathway.The overall water splitting electrolyzer assembled by the optimized electrocatalyst shows a low cell voltage of only 1.52 V and excellent stability to deliver a current density of 10 m A cm-2.This work provides a powerful strategy toward general synthesis of ultrafine alloy nanoparticles for high-performance overall water splitting. | Shen Zhang Xing Zhang Xuerong Shi Feng Zhou Ruihu Wang Xiaoju Li | 2020 | Journal of Energy Chemistry2020，29，10： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员