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| 1 | Soluble Graphene Through Edge-Selective Functionalization显示文摘Thermally expanded graphite was functionalized with 4-bromophenyl addends using the in situ diazonium formation procedure,and after mild sonication treatment in N,N’-dimethylformamide,thin graphene layers were exfoliated from the bulk graphite.These chemically-assisted exfoliated graphene(CEG)sheets had higher solubility than pristine graphene without any stabilizer additive.More than 70%of these soluble flakes had less than 5 layers.Energy filtered transmission electron microscopy(EFTEM)elemental mapping provided evidence of the edge-selective diazonium functionalization with graphene.A majority of the Br signals came from the edges of the CEG indicating that the basal planes were not highly functionalized.The CEG was also characterized by X-ray photoelectron spectroscopy,atomic force microscopy,Raman spectroscopy,and transmission electron microscopy. | Zhengzong Sun Shin-ichiro Kohama Zengxing Zhang Jay RLomeda James M.Tour | 2010 | Nano Research2010，3，2： | 8 |
| 2 | Magnetically levitated/piezoelectric/triboelectric hybrid generator as a power supply for the temperature sensor显示文摘The combination of new intelligent materials and structure technology is becoming an effective way in energy havesting and self-powered sensing. In this work, we demonstrate a magnetically levitated/piezoelectric/triboelectric hybrid generator, which does not use complex structure and has high steady output performance. It includes three parts: magnetically levitated generator(MLG), piezoelectric generator(PNG), triboelectric nanogenerator(TENG). The peak power of each is 135 μW, 22 mW and3.6 mW, which are obtained at 1 MΩ, 10 kΩ and 1 kΩ, respectively. The hybrid generator can completely light up light-emitting diodes(LEDs) under the vibration frequency of 20 Hz and the vibration amplitude of 10 mm. It also can charge a 470 μF capacitor.On this basis, we have integrated the hybrid generaor as a power supply into a self-powered tempreature sensing system. The combination of three generators can not only broaden the operating range, but also increase the operating length and sensitivity.This work will extend the application of self-powered sensor in automatic production line and promote the development of industrial control technology. | ZHANG ZengXing HE Jian HAN JianQiang XU HongYan MU JiLiang WEN Tao WANG DaWei TIAN ZhuMei CHEN ZeTian XUE ChenYang | 2017 | Science China(Technological Sciences)2017，60，7： | 3 |
| 3 | A stretchable triboelectric generator with coplanar integration design of energy harvesting and strain sensing显示文摘The rapid development of flexible triboelectric nanogenerators(TENGs)has become an alternative to batteries for wearable devices.Stretchable,multifunctional,and low-cost are the primary development directions for these wearable devices based on TENG.Herein,a stretchable triboelectric generator with coplanar integration was designed for energy harvesting and force sensing.The industrial conductive silicone and silicone were used to fabricate the TENG with a thickness of less than 0.9 mm.When the elongation was less than 150%,TENG exhibited excellent linear characteristics in the resistance-tensile strain correspondence,and the coefficient of determination was 0.99.This stretchable TENG with a sufficient contact area of 9 cm^(2) could generate a short-circuit current of 2μA when it was in contact with the skin.Lastly,an intelligent tension monitoring wearable device that can effectively measure the tensile force was developed.Such a stretchable,coplanar integration-based,and low-cost wearable device has excellent applicability in wearable electronics. | WU Bin ZHANG ZengXing XUE XiaoBin HAO CongCong ZHANG WenJun BI RuiYu WANG Qiang XUE ChenYang | 2022 | Science China(Technological Sciences)2022，65，1： | 3 |
| 4 | Coil-levitated hybrid generator for mechanical energy harvesting and wireless temperature and vibration monitoring显示文摘The development of wireless monitoring is currently restricted by the short lifetime of batteries,requiring frequent replacement.Utilization of abundant mechanical energy from the surrounding environment has attracted increasing attention in real-time monitoring.Herein,a coil-levitated hybrid generator was developed for the efficient harvesting of mechanical energy from mechanical motion.The novel coil-levitated structure adapted to the metal and magnetic environment.The output currents were systematically analyzed at different operation modes based on the unique combination of triboelectrification,electromagnetic induction,and piezoelectric effect.Under the excitation of vibration frequency and amplitude of 8 Hz and 5 mm respectively,the as-constructed triboelectric nanogenerator delivered a peak power density of 11.40 W/m3 at 10 MΩ.Meanwhile,the middle electromagnetic part and bottom piezoelectric generator provided peak power densities of 6.97 and 79.93 W/m2 at 10000Ω,respectively.More importantly,the battery charging experiment was verified,in which a 30 mA h Li-ion battery can be charged from 2.57 to 3.27 V in about 90 min.In sum,a self-powered temperature and vibration monitoring system was successfully developed based on hybrid generator,promising for realizing wireless monitoring of mechanical equipment without any external power supply. | XUE XiaoBin ZHANG ZengXing WU Bin HE ShanShan WANG Qiang ZHANG WenJun BI RuiYu CUI Juan ZHENG YongQiu XUE ChenYang | 2021 | Science China(Technological Sciences)2021，64，6： | 2 |
| 5 | A study of the neuroprotective effect of the phenolic glucoside gastrodin during cerebral ischemiain vivoandin vitro显示文摘 | ZengX H Zhang SM ZhangL | 2006 | PlantaMed2006，72，15： | 1 |
| 6 | ZnO tetrapods designed as multiterminal sensors to distinguish false responses and increase sensitivity显示文摘 | Zhang Zengxing Sun Lianfeng Zhao Yuanchun | 2008 | Nano Lett2008，8，2： | 1 |
| 7 | Two-dimensional complementary gate-programmable PN junctions for reconfigurable rectifier circuit显示文摘The unique features of ambipolar two-dimensional materials open up a great opportunity to build gate-programmable devices for reconfigurable circuit applications,e.g.,PN junctions for rectifier circuits.However,current-reported rectifier circuits usually consist of one gate-programmable PN junction as the rectifier and one resistor as the load,which are not conductive to voltage output and large-scale integration.Here we propose an approach of complementary gate-programmable PN junctions to assemble reconfigurable rectifier circuit,which include two symmetric back-to-back black phosphorus(BP)/hexagonal boron nitride(h-BN)/graphene heterostructured semi-gate field-effect transistors(FETs)and perform complementary NP and PN junction like complementary metal-oxide-semiconductor(CMOS)circuit.The investigation exhibits that the circuit can effectively reconfigure the circuit with/without rectifying ability,and can process alternating current(AC)signals with the frequency prior 1 KHz and reconfiguration speed up to 25μs.We also achieve the reconfigurable rectifier circuit memory via complementary semi-floating gate FETs configuration.The complementary configuration here should be of low output impedance and low static power consumption,being beneficial for effective voltage output and large-scale integration. | Zhe Sheng Yue Wang Wennan Hu Haoran Sun Jianguo Dong Rui Yu David Wei Zhang Peng Zhou Zengxing Zhang | 2023 | Nano Research2023，16，1： | 0 |
| 8 | Van der Waals contacted WSe_(2) ambipolar transistor for in-sensor computing显示文摘Image sensors with an in-sensor computing architecture have shown great potential in meeting the energy-efficient requirements of emergent data-intensive applications,where images are processed within the photodiode arrays.It demands the composed photodiodes are reconfigurable,which are usually achieved by ambipolar two-dimensional(2D)semiconductors.To improve the ambipolar charges injection,here we report a top-gated field-effect transistor(FET)design that is of bottom van der Waals contact via transferring ambipolar 2D WSe_(2) onto Pd/Cr source/drain electrodes.The devices exhibit nearly negligible effective barrier heights for both holes and electrons based on thermionic emission mode,and show an almost balanced on/off ratio in the p-branch and n-branch.By replacing the top gate with two aligned semi-gates,the devices can effectively function as reconfigurable photodiodes.They can be switched between PIN and NIP configurations via controlling the two semi-gates,exhibiting good linearity in terms of short-circuit current(ISC)and incident light power density.The photodiode arrays are also demonstrated for in-sensor optoelectronic convolutional image processing,showing significant potential for in-sensor computing image processors. | Yue Wang Haoran Sun Zhe Sheng Jianguo Dong Wennan Hu Dongsheng Tang Zengxing Zhang | 2023 | Nano Research2023，16，11： | 0 |
| 9 | Surface plasmon resonance metal-coupled biomass carbon modified TiO_(2) nanorods for photoelectrochemical water splitting显示文摘Exploring efficient and stable photoanode materials is a necessary link to realize the practical application of solar-driven photoelectrochemical(PEC)water splitting.Hence,we prepared rutile TiO_(2) nanorods,with a width of 50 nm,which was growth in situ on carbon cloth(TiO_(2)@CC)by hydrothermal reaction.And then,Ag nanoparticles(NPs)and biomass N,S-C NPs were chosen for the additional modification of the fabricated TiO_(2) nanorods to produce broccoli-like Ag-N,S-C/TiO_(2)@CC nanocomposites.According to the result of ultraviolet-visible diffuse reflectance spectroscopy(UV-vis)and PEC water splitting performance tests,Ag-N,S-C/TiO_(2)@CC broadens the absorption region of TiO_(2)@CC from the ultraviolet region to the visible regio n.Under AM 1.5 G solar light irradiation,the photocurrent density of Ag-N,S-C/TiO_(2)@CC is 89.8μA·cm^(-2),which is 11.8 times higher than TiO_(2)@CC.Under visible light irradiation,the photocurrent density of Ag-N,S-C/TiO_(2)@CC reaches to 12.6μA·cm^(-2),which is 21.0 times higher than TiO_(2)@CC.Moreover,Ag-N,S-C/TiO_(2)@CC shows a photocurrent responses in full pH range.It can be found that Ag NPs and N,S-C NPs play key roles in broaden the absorption range of TiO_(2) nanorods to the visible light region and,promote the occurrence of PEC water oxidation reaction due to the surface plasmon resonance effect of Ag NPs and the synergistic effect of N,S-C NPs.The mechanism demonstrated that Ag-N,S-C/TiO_(2)@CC can separate the photogenerated electron-hole pairs effectively and transfer the photogenerated electrons to the photocathode(Pt plate)in time.This research provides a new strategy for exploration surface plasma metal coupled biomass carbon materials in the field of PEC water splitting. | Yingzhen Zhang Yonggang Lei Tianxue Zhu Zengxing Li Shen Xu Jianying Huang Xiao Li Weilong Cai Yuekun Lai Xiaojun Bao | 2022 | Chinese Journal of Chemical Engineering2022，35，1： | 0 |
| 10 | Boron nitride-enabled printing of a highly sensitive and flexible iontronic pressure sensing system for spatial mapping显示文摘Recently,flexible iontronic pressure sensors(FIPSs)with higher sensitivities and wider sensing ranges than conventional capacitive sensors have been widely investigated.Due to the difficulty of fabricating the nanostructures that are commonly used on electrodes and ionic layers by screen printing techniques,strategies for fabricating such devices using these techniques to drive their mass production have rarely been reported.Herein,for the first time,we employed a 2-dimensional(2D)hexagonal boron nitride(h-BN)as both an additive and an ionic liquid reservoir in an ionic film,making the sensor printable and significantly improving its sensitivity and sensing range through screen printing.The engineered sensor exhibited high sensitivity(S_(min)>261.4 kPa^(−1))and a broad sensing range(0.05-450 kPa),and it was capable of stable operation at a high pressure(400 kPa)for more than 5000 cycles.In addition,the integrated sensor array system allowed accurate monitoring of wrist pressure and showed great potential for health care systems.We believe that using h-BN as an additive in an ionic material for screen-printed FIPS could greatly inspire research on 2D materials for similar systems and other types of sensors. | Zekun Yang Qikai Duan Junbin Zang Yunlong Zhao Weihao Zheng Ran Xiao Zhidong Zhang Liangwei Hu Guirong Wu Xueli Nan Zengxing Zhang Chenyang Xue Libo Gao | 2023 | Microsystems & Nanoengineering2023，9，3： | 0 |
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