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| 1 | Restoration and Rational Use of Degraded Saline Reed Wetlands:A Case Study in Western Songnen Plain, China显示文摘The protection, restoration and sustainable use are key issues of all the wetlands worldwide. Ecological, agronomic, and engineering techniques have been integrated in the development of a structurally sound, ecologically beneficial engineering restoration method for restoring and utilizing a degraded saline wetland in the western Songnen Plain of China. Hydrological restoration was performed by developing a system of biannual irrigation and drainage using civil engineering measures to bring wetlands into contact with river water and improve the irrigation and drainage system in the wetlands. Agronomic measures such as plowing the reed fields, reed rhizome transplantation, and fertilization were used to restore the reed vegetation. Biological measures, including the release of crab and fish fry and natural proliferation, were used to restore the aquatic communities. The results of the restoration were clear and positive. By the year 2009, the reed yield had increased by 20.9 times. Remarkable ecological benefits occurred simultaneously. Vegetation primary-production capacity increased, local climate regulation and water purification enhanced, and biodiversity increased. This demonstration of engineering techniques illustrates the basic route for the restoration of degraded wetlands, that the biodiversity should be reconstructed by the comprehensive application of engineering, biological, and agronomic measures based on habitat restoration under the guidance of process-oriented strategies. The complex ecological system including reeds, fish and crabs is based on the biological principles of coexistence and material recycling and provides a reasonable ecological engineering model suitable for the sustainable utilization of degraded saline reed wetlands. | WEN Bolong LIU Xingtu LI Xiujun YANG Fuyi LI Xiaoyu | 2012 | Chinese Geographical Science2012，22，2： | 10 |
| 2 | Ultrasmall Fe-doped carbon dots nanozymes for photoenhanced antibacterial therapy and wound healing显示文摘Pathogenic bacteria pose a devastating threat to public health.However,because of the growing bacterial antibiotic resistance,there is an urgent need to develop alternative antibacterial strategies to the established antibiotics.Herein,iron-doped carbon dots(Fe-CDs,~3 nm)nanozymes with excellent photothermal conversion and photoenhanced enzyme-like properties are developed through a facile one-pot pyrolysis approach for synergistic efficient antibacterial therapy and wound healing.In particular,Fe doping endows CDs with photoenhanced peroxidase(POD)-like activity,which lead to the generation of heat and reactive oxygen species(ROS)for Gram-positive and Gram-negative bacteria killing.This study demonstrates Fe-CDs have significant wound healing efficiency of Fe-CDs by preventing infection,promoting fibroblast proliferation,angiogenesis,and collagen deposition.Furthermore,the ultrasmall size of Fe-CDs possesses good biocompatibility favoring clinical translation.We believe that the nanozyme-mediated therapeutic platform presented here is expected to show promising applications in antibacterial. | Yunhang Liu Bolong Xu Mingzhu Lu Shanshan Li Juan Guo Fangzhou Chen Xiaolu Xiong Zhe Yin Huiyu Liu Dongsheng Zhou | 2022 | Bioactive Materials2022，7，6： | 7 |
| 3 | Surface engineering at the interface of core/shell nanoparticles promotes hydrogen peroxide generation显示文摘Hydrogen peroxide(H_2O_2), an environmentally friendly oxidant, has already been widely used in many chemical synthesis and industrials as an alternative to replace traditional oxidants including chlorinated oxidizers and strong acids. However, the conventional synthesis method confronts intense energy cost,tedious separation procedures and high cost, which is not competitive with traditional oxidants. Although direct H_2O_2 synthesis from H_2 and O_2 is a green and atomically economic reaction, satisfactory activity and desirable selectivity still remain formidable challenges. Herein, for the first time, a class of Pd@NiO-x nanoparticles(NPs)(x = 1, 2, 3 and 4) with a unique core@shell interface structure has been created to achieve high activity, selectivity and stability for the direct H_2O_2 synthesis. A precise thermal annealing on Pd@Ni-x NPs revealed that the resulting Pd@Ni O-x NPs exhibited the volcano-like activity toward direct H_2O_2 synthesis as a function of annealing temperature and time. By tuning the composition of Pd@Ni O-x NPs and the reaction condition, the efficiency of H_2O-2 synthesis could be well optimized with 5 wt%Pd@NiO-3/TiO_2 exhibiting the highest productivity(89 mol/(kg_(cat) h)) and selectivity(91%) to H_2O_2 as well as excellent stability, making it one of the best catalysts for direct H_2O_2 synthesis reported to date. | Yonggang Feng Qi Shao Bolong Huang Junbo Zhang Xiaoqing Huang | 2018 | National Science Review2018，5，6： | 7 |
| 4 | ZnWO_4 nanocrystals/reduced graphene oxide hybrids:Synthesis and their application for Li ion batteries显示文摘ZnWO4,as an environment-friendly and economic material,has the potential for Li ion batteries(LIB)application.In this paper,a facile method has been developed to synthesize ZnWO4supported on the reduced graphene oxide(RGO)to improve its LIB performance.The cuboid-like ZnWO4nanocrystals are prepared by directly adding Na2WO4 powders into the graphene oxide/Zn aqueous solution followed by a hydrothermal treatment.The high-resolution TEM,XRD and XPS characterizations were employed to demonstrate structural information of the as-prepared ZnWO4/RGO hybrids carefully.Besides,we also discussed the LIB properties of the hybrids based on the detailed galvanostatic charge-discharge cycling tests.As a result,the specific capacity of the as-prepared ZnWO4/RGO hybrids reached more than 477.3 mA h g 1after 40 cycles at a current density of 100 mA g 1(only less than 159 mA g 1for bare ZnWO4).During the whole cyclic process,the coulombic efficiency steadily kept the values higher than 90%. | WANG Xiao LI BoLong LIU DaPeng XIONG HuanMing | 2014 | Science China Chemistry2014，57，1： | 6 |
| 5 | RRx-001 ameliorates inflammatory diseases by acting as a potent covalent NLRP3 inhibitor显示文摘The NLRP3 inflammasome plays a crucial role in innate immune-mediated inflammation and contributes to the pathogenesis of multiple autoinflammatory,metabolic and neurodegenerative diseases,but medications targeting the NLRP3 inflammasome are not available for clinical use.RRx-001 is a well-tolerated anticancer agent currently being investigated in phase III clinical trials,but its effects on inflammatory diseases are not known.Here,we show that RRx-001 is a highly selective and potent NLRP3 inhibitor that has strong beneficial effects on NLRP3-driven inflammatory diseases.RRx-001 inhibits the activation of the canonical,noncanonical,and alternative NLRP3 inflammasomes but not the AIM2,NLRC4 or Pyrin inflammasomes.Mechanistically,RRx-001 covalently binds to cysteine 409 of NLRP3 via its bromoacetyl group and therefore blocks the NLRP3-NEK7 interaction,which is critical for the assembly and activation of the NLRP3 inflammasome.More importantly,RRx-001 treatment attenuates the symptoms of lipopolysaccharide(LPS)-induced systemic inflammation,dextran sulfate sodium(DSS)-induced colitis and experimental autoimmune encephalomyelitis(EAE)in mice.Thus,our study identifies RRx-001 as a new potential therapeutic agent for NLRP3-driven diseases. | Yun Chen Hongbin He Bolong Lin Yun Chen Xianming Deng Wei Jiang Rongbin Zhou | 2021 | Cellular & Molecular Immunology2021，18，6： | 5 |
| 6 | Effects of Anthropogenic Disturbance on Sediment Organic Carbon Mineralization Under Different Water Conditions in Coastal Wetland of a Subtropical Estuary显示文摘The changes in soil organic carbon(C) mineralization as affected by anthropogenic disturbance directly determine the role of soils as C source or sink in the global C budget. The objectives of this study were to investigate the effects of anthropogenic disturbance(aquaculture pond, pollutant discharge and agricultural activity) on soil organic C mineralization under different water conditions in the Minjiang River estuary wetland, Southeast China. The results showed that the organic C mineralization in the wetland soils was significantly affected by human disturbance and water conditions(P < 0.001), and the interaction between human disturbance activities and water conditions was also significant(P < 0.01). The C mineralization rate and the cumulative mineralized carbon dioxide-carbon(CO_2-C)(at the 49th day) ranked from highest to lowest as follows: Phragmites australis wetland soil > aquaculture pond sediment > soil near the discharge outlet > rice paddy soil. This indicated that human disturbance inhibited the mineralization of C in soils of the Minjiang River estuary wetland, and the inhibition increased with the intensity of human disturbance. The data for cumulative mineralized CO_2-C showed a good fit(R^2 > 0.91) to the first-order kinetic model C_t = C_0(1 – exp(–kt)). The kinetic parameters C_0, k and C_0 k were significantly affected by human disturbance and water conditions. In addition, the total amount of mineralized C(in 49 d) was positively related to C_0, C_0 k and electrical conductivity of soils. These findings indicated that anthropogenic disturbance suppressed the organic C mineralization potential in subtropical coastal wetland soils, and changes of water pattern as affected by human activities in the future would have a strong influence on C cycling in the subtropical estuarine wetlands. | MOU Xiaojie LIU Xingtu SUN Zhigao TONG Chuan HUANG Jiafang WAN Siang WANG Chun WEN Bolong | 2018 | Chinese Geographical Science2018，28，3： | 4 |
| 7 | Partially hydroxylated ultrathin iridium nanosheets as efficient electrocatalysts for water splitting显示文摘Ultrathin two-dimensional(2D)materials have attracted considerable attention for their unique physicochemical properties and promising applications;however,preparation of freestanding ultrathin 2D noble metal remains a significant challenge.Here,for the first time,we report use of a wet-chemical method to synthesize partially hydroxylated ultrathin Ir nanosheets(ir-NSs)of only five to six atomic layers*thickness.Detailed analysis indicates that the growth confinement effect of carbon monoxide and the partially hydroxylated surface play a critical role in formation of the ultrathin structure.The ultrathin Ir-NSs exhib让excellent performance for both the hydrogen evolution reaction and oxygen evolution reaction in a wide pH range,outperforming the state-of the-art Pt/C and IrO2,respectively.Density-functional theory calculations reveal that the partial hydroxylation not only enhances the surface electron transfer between Ir-sites and intermediate O-species,but also guarantees efficient irdtial activation ofbond cleavage of H-O-H for first-step H2O splitting.This;ultimately,breaks through barriers to full water splitting,with efficient electron transfer essentially maintained. | Zifang Cheng Bolong Huang Yecan Pi Leigang Li Qi Shao Xiaoqing Huang | 2020 | National Science Review2020，7，8： | 4 |
| 8 | Characterization of Water Quality in Xiao Xingkai Lake:Implications for Trophic Status and Management显示文摘Increasing cases of lake eutrophication globally have raised concerns among stakeholders,and particularly in China.Evaluating the causes of eutrophication in waterways is essential for effective pollution prevention and control.Xiao Xingkai Lake is part of and connected to Xingkai(Khanka)Lake,a boundary lake between China and Russia.In this study,we investigated the spatio-temporal variabilities in water quality(i.e.,dissolved oxygen(DO),total nitrogen(TN),total phosphorus(TP),chemical oxygen demand(CODMn)and ammonium-nitrogen(NH4+-N))in Xiao Xingkai Lake,from 2012 to 2014,after which a Trophic Level Index was used to evaluate trophic status,in addition to the factors influencing water quality variation in the lake.The DO,TN,TP,CODMn and NH4+-N concentrations were 0.44-15.57,0.16-5.11,0.01-0.45,0.16-48.31,and 0.19-0.78 mg/L,respectively.Compared to the Environmental Quality Standards for surface water(GB 3838-2002)in China,the lake transitioned to an oligotrophic status in 2013 and 2014 from a mesotrophic status in 2012,TN and TP concentrations were the key factors influencing water quality of Xiao Xingkai Lake.Non-para-metric test results showed that sampling time and sites had significant effects on water quality.Water quality was worse in summer and in tourism and aquaculture areas,followed by agricultural drainage areas.Furthermore,lake water trophic status fluctuated between medium eutrophic and light eutrophic status from September 2012 to September 2014,and was negatively correlated with water level.Water quality in tourism and aquaculture sites were medium eutrophic,while in agricultural areas were light eutrophic.According to the results,high water-level fluctuations and anthropogenic activities were the key factor driving variability in physicochemical parameters associated with water quality in Xiao Xingkai Lake. | YU Shuling LI Xiaoyu WEN Bolong CHEN Guoshuang HARTLEYC Anne JIANG Ming LI Xiujun | 2021 | Chinese Geographical Science2021，31，3： | 4 |
| 9 | Rh-doped PdAg nanoparticles as efficient methanol tolerance electrocatalytic materials for oxygen reduction显示文摘Direct methanol fuel cells(DMFCs)have received extensive attention on their high efficiency,high reliability,and no carbon emission.Unfortunately,the poor methanol tolerance and sluggish oxygen reduction reaction(ORR)at cathode have seriously hindered their further development.Herein we report the synthesis of a new class of Rh-doped PdAg alloy nanoparticles(NPs)for boosting ORR activity with high methanol tolerance capacity concurrently.The ORR mass activity of typical Rh_4Pd_(40)Ag_(56)NPs is 4.2 times higher than that of commercial Pt catalyst.Moreover,it shows a great methanol tolerance capability by maintaining 92.4%in ORR mass activity in alkaline solution with 0.1 mol L^(à1)methanol,against a big decrease of almost 100%for commercial Pt.Even after 30,000 potential cycles with 1.0 mol L^(à1)methanol,Rh_4Pd_(40)Ag_(56)NPs still retain ORR mass activity of up to 68.3%.DFT calculations reveal that excellent ORR performance with excellent methanol tolerance originates the active d-band-pinning engineering for an efficient site-independent electron-transfer.A generalized d-band mediated fine electron-transfer tuning path has blueprinted for effectively minimizing intrinsic ORR barriers with high current density.The present work highlights the key role of Rh doping in enhancing the ORR activity and methanol tolerance ability of PdAg NPs for future high-performance DMFCs. | Yingjun Sun Bolong Huang Nuoyan Xu Yingjie Li Mingchuan Luo Chunji Li Yingnan Qin Lei Wang Shaojun Guo | 2019 | Science Bulletin2019，64，1： | 4 |
| 10 | Soil Carbon, Nitrogen and Phosphorus Concentrations and Stoichiometries Across a Chronosequence of Restored Inland Soda Saline-Alkali Wetlands, Western Songnen Plain, Northeast China显示文摘Soil carbon(C), nitrogen(N) and phosphorus(P) concentrations and stoichiometries can be used to evaluate the success indicators to the effects of wetland restoration and reflect ecosystem function. Restoration of inland soda saline-alkali wetlands is widespread, however, the soil nutrition changes that follow restoration are unclear. We quantified the recovery trajectories of soil physicochemical properties, including soil organic carbon(SOC), total nitrogen(TN), and total phosphorus(TP) pools, for a chronosequence of three restored wetlands(7 yr, 12 yr and 21 yr) and compared these properties to those of degraded and natural wetlands in the western Songnen Plain, Northeast China. Wetland degradation lead to the loss of soil nutrients. Relative to natural wetlands, the mean reductions of in SOC, TN, and TP concentrations were 89.6%, 65.5% and 52.5%, respectively. Nutrients recovered as years passed after restoration. The SOC, TN, and TP concentrations increased by 2.36 times, 1.15 times, and 0.83 times, respectively in degraded wetlands that had been restored for 21 yr, but remained 29.2%, 17.3%, and 12.8% lower, respectively, than those in natural wetlands. The soil C∶N(RC N), C∶P(R CP), and N∶P(R NP) ratios increased from 5.92 to 8.81, 45.36 to 79.19, and 7.67 to 8.71, respectively in the wetland that had been restored for 12 yr. These results were similar to those from the natural wetland and the wetland that had been restored for 21 yr(P > 0.05). Soil nutrients changes occurred mainly in the upper layers(≤ 30 cm), and no significant differences were found in deeper soils(> 30 cm). Based on this, we inferred that it would take at least 34 yr for SOC, TN, and TP concentrations and 12 yr for RC N, R CP, and RN P in the top soils of degraded wetlands to recover to levels of natural wetlands. Soil salinity negatively influenced SOC(r =-0.704, P < 0.01), TN(r =-0.722, P < 0.01), and TP(r =-0.882, P < 0.01) concentrations during wetland restoration, which indicates that reducing salinity is beneficial to SOC, TN, and TP recovery. Moreover, plants were an important source of soil nutrients and vegetation restoration was conducive to soil nutrient accumulation. In brief, wetland restoration increased the accumulation of soil biogenic elements, which indicated that positive ecosystem functions changes had occurred. | YANG Yanli MOU Xiaojie WEN Bolong LIU Xingtu | 2020 | Chinese Geographical Science2020，30，5： | 4 |
| 11 | Multiple structural defects in ultrathin NiFe-LDH nanosheets synergistically and remarkably boost water oxidation reaction显示文摘Modifying electrocatalysts nanostructures and tuning their electronic properties through defects-oriented synthetic strategies are:essential to improve the oxygen evolution reaction(OER)performance of electrocatalysts.Current synthetic strategies about.electrocatalysts mainly target the single or double structural defects,while the researches about the synergistic effect of multiple'structural defects are rare.In this work,the ultrathin NiFe layered double hydroxide nanosheets with a holey structure,oxygen;vacancies and Ni^(3+)defects on nickel foam(NiFe-LDH-NSs/NF)are prepared by employing a simple and green H202-assisted etching 1 method.The synergistic effect ofthe above three defects leads to the exposure of.more active sites and significant improvement of:the intrinsic activity.The optimized catalyst exhibits an excellent OER performance with an extraordinarily low overpotential of 170 mV;at to mA·cm^(-2) and a small Tafel slope of 39.3 mV·dec^(-1) in 1 M KOH solution.Density functional theory calculations reveal this OER;performance arises from pseudo re-oxidized metal-stable Ni^(3+)near oxygen vacancies(O_(vac)),which suppresses 3d-e_(g) of Ni-site and!elevates d-band center towards the competitively low electron-transferbarrier.This work provides a new insight to fabricate advanced electrocatalysts for renewable energy conversion technologies. | Zhongyin Zhao Qi Shao Jiangyan Xue Bolong Huang Zheng Niu Hongwei Gu Xiaoqing Huang Jianping Lang | 2022 | Nano Research2022，15，1： | 3 |
| 12 | Mesoporous carbon nanomaterials induced pulmonary surfactant inhibition,cytotoxicity,inflammation and lung fibrosis显示文摘Environmental exposure and health risk upon engineered nanomaterials are increasingly concerned. The family of mesoporous carbon nanomaterials(MCNs) is a rising star in nanotechnology for multidisciplinary research with versatile applications in electronics,energy and gas storage, and biomedicine. Meanwhile, there is mounting concern on their environmental health risks due to the growing production and usage of MCNs. The lung is the primary site for particle invasion under environmental exposure to nanomaterials. Here, we studied the comprehensive toxicological profile of MCNs in the lung under the scenario of moderate environmental exposure. It was found that at a low concentration of 10 μg/mL MCNs induced biophysical inhibition of natural pulmonary surfactant. Moreover, MCNs at similar concentrations reduced viability of J774 A.1 macrophages and lung epithelial A549 cells.Incubating with nature pulmonary surfactant effectively reduced the cytotoxicity of MCNs.Regarding the pro-inflammatory responses, MCNs activated macrophages in vitro, and stimulated lung inflammation in mice after inhalation exposure, associated with lung fibrosis.Moreover, we found that the size of MCNs played a significant role in regulating cytotoxicity and pro-inflammatory potential of this nanomaterial. In general, larger MCNs induced more pronounced cytotoxic and pro-inflammatory effects than their smaller counterparts. Our results provided valuable information on the toxicological profile and environmental health risks of MCNs, and suggested that fine-tuning the size of MCNs could be a practical precautionary design strategy to increase safety and biocompatibility of this nanomaterial. | Yunan Chen Yi Yang Bolong Xu Shunhao Wang Bin Li Juan Ma Jie Gao Yi Y.Zuo Sijin Liu | 2017 | Journal of Environmental Sciences2017，29，12： | 3 |
| 13 | New interpretation of laser gyro drifts显示文摘Discuss and develop some contents which are relevant to the IEEE Std 647TM-2006 in this paper. The IEEE Std only involves Allan variance, and decomposes it into five primary noise terms, in which, however, the noise nature of the so called 'rate random walk noise' and the 'rate ramp' is doubted by the IEEE Std editors. Here we use a mathematical identity to entirely affirm the first query and partially the second query as mentioned above. Besides, we argue that only the classical variance can be used in navigation, not the Allan variance. In order to seek the true nature of all drift terms in the variance, we adopt our original work that represents the noises as damped oscillations, to obtain the power spectral density (PSD) of the noises which is then transformed back into time domain. When the damped time constant is much longer than the sampling interval, the re-sulting slow variation term may be expanded into three terms: ordinary bias instability, rate random walk, and rate ramp. Therefore, these 'noise terms' are not independent, and they are more of deterministic errors than random noises, and can be explained quantitatively. The resulting fast variation drift may be expanded into two terms. The first term is the same as angle random noise, while the second term adds to the true quantization noise term to form a new combined term called 'quantiza-tion noise term'. As the result of our research, not only the IEEE Std editors’ suspicions above are answered completely, but a new theory to analyze the laser gyro drifts is also presented, with several supporting examples to explain and verify the theory. | GAO BoLong,ZHANG Mei & ZHANG Wen College of Opto-electric Science and Engineering,National University of Defense Technology,Changsha 410073,China | 2010 | Science China(Technological Sciences)2010，53，5： | 3 |
| 14 | Activated Carbon from Rice Husk with One-Step KOH Mechanical Mixing Activation as Adsorbent for Treating Phenolic Wastewater显示文摘This study investigates how large-surface-area biocarbons with high phenolic adsorption capacities can be obtained from cheap and abundant rice husk(RH).The RH is directly mixed with potassium hydroxide(KOH)and activated in a flowing N_(2) atmosphere,and the effects of the pyrolysis temperature and KOH to RH ratio on the structure of the obtained activated carbon adsorbents and their adsorption of p-nitrophenol and phenol are studied.The results show that the optimum pyrolysis temperature of RH is 750℃,whereby the highest surface area of 2047 m^(2)/g and best adsorption performance are obtained with a KOH to RH ratio of 3:1.Moreover,the obtained biocarbons achieve a maximum adsorption capacity of 175 mg/g for phenol and 430 mg/g for p-nitrophenol,which are higher than most previously reported data. | Jiang Bolong Jiang Nan Shi Shunjie Cui Yanyan | 2022 | China Petroleum Processing & Petrochemical Technology2022，24，4： | 2 |
| 15 | Annealing behavior of a modified 5083 aluminum alloy显示文摘 | Shuangping Lin Zuoren Nie Hui Huang Bolong Li | 2009 | Materials and Design2009，，3： | 2 |
| 16 | Series-Type Switched-Inductor Z-Source Inverter显示文摘To solve the disadvantages of the traditional Z-source inverter(ZSI),this paper investigates a series-type switched-inductor Z-source inverter(SSI-ZSI)topology.It not only preserves the advantages of the traditional ZSI,but also improves the voltage gain.On the condition of the same voltage gain,the capacitor voltage stress is reduced,the soft start characteristic can be achieved and the inverter can be immune to the damage of the inrush current.The circuit structure and operating principle are analyzed in detail;the simulation model and the experimental platform are built.The simulation and experimental results verify the rationality and superiority of the circuit topology. | Xupeng Fang Yingying Tian Xiaokang Ding Bolong Ma | 2020 | CES Transactions on Electrical Machines and Systems2020，4，1： | 2 |
| 17 | MOF-Transformed In_(2)O_(3-x)@C Nanocorn Electrocatalyst for Efficient CO_(2)Reduction to HCOOH显示文摘For electrochemical CO_(2) reduction to HCOOH,an ongoing challenge is to design energy efficient electrocatalysts that can deliver a high HCOOH current density(JHCOOH)at a low overpotential.Indium oxide is good HCOOH production catalyst but with low con-ductivity.In this work,we report a unique corn design of In_(2)O_(3-x)@C nanocatalyst,wherein In_(2)O_(3-x)nanocube as the fine grains dispersed uniformly on the carbon nanorod cob,resulting in the enhanced conductivity.Excellent performance is achieved with 84%Faradaic efficiency(FE)and 11 mA cm^(−2)JHCOOH at a low potential of−0.4 V versus RHE.At the current density of 100 mA cm^(−2),the applied potential remained stable for more than 120 h with the FE above 90%.Density functional theory calculations reveal that the abundant oxygen vacancy in In_(2)O_(3-x) has exposed more In^(3+) sites with activated electroactivity,which facilitates the formation of HCOO*intermediate.Operando X-ray absorp-tion spectroscopy also confirms In^(3+) as the active site and the key intermediate of HCOO*during the process of CO_(2) reduction to HCOOH. | Chen Qiu Kun Qian Jun Yu Mingzi Sun Shoufu Cao Jinqiang Gao Rongxing Yu Lingzhe Fang Youwei Yao Xiaoqing Lu Tao Li Bolong Huang Shihe Yang | 2022 | Nano-Micro Letters2022，14，10： | 2 |
| 18 | A Case Study on the Rapid Rain-to-Snow Transition in Late Spring 2018 over Northern China:Effects of Return Flows and Topography显示文摘Phase changes in the precipitation processes of early winter and late spring in midlatitude regions represent challenges when forecasting the timing and magnitude of snowfall.On 4 April 2018,a heavy snow process occurred in Beijing and northwestern Hebei Province,becoming the most delayed occurrence of heavy spring snow ever recorded over Beijing in the last 30 years.This paper uses observational and numerical simulation data to investigate the causes for the rapid rain-to-snow(RRTS)phase transition during this process.The following results are obtained.(1)Return flows(RFs),an interesting type of easterly wind,including those at 1000,925,and 800 hPa,played an important role in this heavy snow process and presented a characteristic'sandwich'structure.The RFs,complex topography,and snow particles that dominated the clouds,were the three key factors for the RRTS transition.(2)The RRTS transition in the plains was directly related to the RF at 925 hPa,which brought about advective cooling initiated approximately 4-6 h before the onset of precipitation.Then,the RF played a role of diabatic cooling when snow particles began to fall at the onset of precipitation.(3)The RRTS transition in the northern part of the Taihang Mountains was closely related to the relatively high altitude that led to a lower surface temperature owing to the vertical temperature lapse rate.Both immediately before and after the onset of precipitation,the snow particles in clouds entrained the middle-level cold air downward,causing the melting layer(from surface to the 0℃-isotherm level)to become very thin;and thus the snow particles did not have adequate time to melt before falling to the ground.(4)The rapid RRTS over the Yanqing mountainous area in the northwest of Beijing could have involved all the three concurrent mechanisms:the advective cooling of RF,the melting cooling of cloud snow particles,and the high-altitude effect.Compared with that in the plain area with less urbanization the duration of the RRTS in the plain area with significant urbanization was extended by approximately 2 h. | Wenlong ZHANG Xiaopeng CUI Bolong DUAN Bo YU Runxia GUO Haiwen LIU | 2022 | Journal of Meteorological Research2022，36，1： | 2 |
| 19 | Graphdiyne-based metal atomic catalysts for synthesizing ammonia显示文摘Development of novel catalysts for nitrogen reduction at ambient pressures and temperatures with ultrahigh ammonia(NH_(3))yield and selectivity is challenging.In this work,an atomic catalyst with separated Pd atoms on graphdiyne(Pd-GDY)was synthesized,which shows fascinating electrocatalytic properties for nitrogen reduction.The catalyst has the highest average NH_(3)yield of 4.45±0.30 mgNH_(3)mg Pd^(-1)h^(-1),almost tens of orders larger than for previously reported catalysts,and 100%reaction selectivity in neutral media.Pd-GDY exhibits almost no decreases in NH_(3)yield and Faradaic efficiency.Density functional theory calculations show that the reaction pathway prefers to perform at the(Pd,C1,C2)active area because of the strongly coupled(Pd,C1,C2),which elevates the selectivity via enhanced electron transfer.By adjusting the p–d coupling accurately,reduction of self-activated nitrogen is promoted by anchoring atom selection,and side effects are minimized. | Huidi Yu Yurui Xue Lan Hui Chao Zhang Yan Fang Yuxin Liu Xi Chen Danyan Zhang Bolong Huang Yuliang Li | 2021 | National Science Review2021，8，8： | 2 |
| 20 | Clinical treatment of depressive patients with Anshendingzhi decoction显示文摘OBJECTIVE: To determine the effects of Anshendingzhi decoction(ASDZD) on depression, to com-pare ASDZD with Danzhixiaoyao pill(DZXYP), and to provide evidence for the clinical treatment of depression with Traditional Chinese Medicine.METHODS: Seventy-eight patients with depression were enrolled from 2011 to 2013 in this double-blinded study. Patients were randomly divided into two groups: ASDZD(treatment group, n=39)and DZXYP(control group, n=39). Hamilton Depressive Scale and TCM Syndrome Differentiation Scale were used to assess depression and efficacy before treatment and 2, 4, and 6 weeks after treatment.The Treatment Emergent Symptoms Scale(TESS)was used to evaluate adverse reactions, observe,and record treatment outcomes.RESULTS: ASDZD was significantly more effective than DZXYP. There were significant differences between the two groups in terms of recovered patients, overall response rate, and TESS score(all P<0.05).CONCLUSION: ASDZD is an effective treatment for depression. ASDZD could improve clinical symptoms and warrants further clinical research and application. | Jianyu Yang Lijuan Jiang Yang Li Qingwen Zhu Dong Liu Wugeng Xue Bolong Cao Yingke Liu Xing Wang | 2014 | Journal of Traditional Chinese Medicine2014，34，6： | 2 |
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