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| 1 | Label-free fiber nanograting sensor for real-time in situ early monitoring of cellular apoptosis显示文摘The achievement of functional nanomodules for subcellular label-free measurement has long been pursued in order to fully understand cellular functions.Here,a compact label-free nanosensor based on a fiber taper and zinc oxide nanogratings is designed and applied for the early monitoring of apoptosis in individual living cells.Because of its nanoscale dimensions,mechanical flexibility,and minimal cytotoxicity to cells,the sensing module can be loaded in cells for long term in situ tracking with high sensitivity.A gradual increase in the nuclear refractive index during the apoptosis process is observed,revealing the increase in molecular density and the decrease in cell volume.The strategy used in our study not only contributes to the understanding of internal environmental variations during cellular apoptosis but also provides a new platform for nonfluorescent fiber devices for investigation of cellular events and understanding fundamental cell biochemical engineering. | Danran Li Nina Wang Tianyang Zhang Guangxing Wu Yifeng Xiong Qianqian Du Yunfei Tian Weiwei Zhao Jiandong Ye Shulin Gu Yanqing Lu Dechen Jiang Fei Xu | 2022 | Advanced Photonics2022，4，1： | 5 |
| 2 | Acetate-assistant efficient cation-exchange of halide perovskite nanocrystals to boost the photocatalytic CO_(2) reduction显示文摘The judicious implantation of active metal cations into the surface of semiconductor nanocrystal(NC)through cation-exchange is one of the facile and viable strategies to enhance the activity of catalysts for photocatalytic CO_(2)reduction,by shortening the transfer pathway of photogenerated carriers and increasing the active sites simultaneously.However,cation-exchange is hard to achieve for halide perovskite NCs owing to the stable octahedron of[PbX6]4−with strong interaction between halogen and lead.Herein,we report a facile method to overcome this obstacle by replacing partial Br−with acetate(Ac−)to generate CsPbBr_(3) NC(coded as CsPbBr_(3−x)Ac_(x)).A small amount of Ac−instead of Br−does not change the crystal structure of halide perovskite.Owing to the weaker interaction between acetate and lead in comparison with bromide,the corresponding octahedron structure containing acetate in CsPbBr_(3−x)Ac_(x) can be easily opened to realize efficient cation-exchange with Ni^(2+) ions.The resulting high loading amount of Ni^(2+) as active site endows CsPbBr_(3−x)Ac_(x) with an improved performance for photocatalytic CO_(2)reduction under visible light irradiation,exhibiting a significantly increased CO yield of 44.09μmol·g^(−1)·h^(−1),which is over 8 and 3 times higher than those of traditional pristine CsPbBr_(3) and nickel doped CsPbBr_(3) NC,respectively.This work provides a critical solution for the efficient metal doping of low-cost halide perovskite NCs to enhance their photocatalytic activity,promoting their practical applications in the field of photocatalysis. | Jialin Cheng Yanfei Mu Liyuan Wu Zhaolei Liu Ke Su Guangxing Dong Min Zhang Tongbu Lu | 2022 | Nano Research2022，15，3： | 3 |
| 3 | Taxonomic and functional variations in the microbial community during the upgrade process of a full-scale landfill leachate treatment plant-from conventional to partial nitrification-denitrification显示文摘Because of the low access to biodegradable organic substances used for denitrification,the partial nitrification-denitrification process has been considered as a low-cost,sustainable alternative for landfill leachate treatment.In this study,the process upgrade from conventional to partial nitrificationdenitrification was comprehensively investigated in a full-scale landfill leachate treatment plant(LLTP).The partial nitrification-denitrification system was successfully achieved through the optimizing dissolved oxygen and the external carbon source,with effluent nitrogen concentrations lower than 150 mg/L.Moreover,the upgrading process facilitated the enrichment of Nitrosomonas(abundance increased from 0.4%to 3.3%),which was also evidenced by increased abundance of amoA/B/C genes carried by Nitrosomonas.Although Nitrospira(accounting for 0.1%-0.6%)was found to stably exist in the reactor tank,considerable nitrite accumulation occurred in the reactor(reaching 98.8 mg/L),indicating high-efficiency of the partial nitrification process.Moreover,the abundance of Thauera,the dominant denitrifying bacteria responsible for nitrite reduction,gradually increased from 0.60%to 5.52%during the upgrade process.This process caused great changes in the microbial community,inducing continuous succession of heterotrophic bacteria accompanied by enhanced metabolic potentials toward organic substances.The results obtained in this study advanced our understanding of the operation of a partial nitrification-denitrification system and provided a technical case for the upgrade of currently existing full-scale LLTPs. | Binbin Sheng Depeng Wang Xianrong Liu Guangxing Yang Wu Zeng Yiqing Yang Fangang Meng | 2020 | Frontiers of Environmental Science & Engineering2020，14，6： | 3 |
| 4 | Syngas production by dry reforming of the mixture of glycerol and ethanol with CaCO3显示文摘The reduction of CO2 emission is crucial for the mitigation of climate change.A considerable amount of industrial CO2 can be absorbed in the form of carbonates through high-temperature sorption processes.In this regard,the efficient conversion of carbonates to value-added products will provide an economically viable method for the sustainable usage of carbon compounds.Herein,we report a promising solution involving the use of a glycerol and ethanol mixture as a hydrogen donor in the dry reforming process with CaCO3 to produce syngas.A series of metal active components,including Ni,Fe,Co,Cu,Pt,Pd,Ru,and Rh,was used to promote this reaction.Ni showed comparable performance with that of Pd,but outperformed Co,Fe,Cu,Rh,Ru,and Pt.Approximately 100%conversion of glycerol and ethanol,~92%selectivity of synthesis gas(H2 and CO),and a H2/CO ratio of^1.2 were achieved over CaCO3 containing10 wt%Ni(10Ni-CaCO3).Meanwhile,the CO2 concentration was less than 5 vol%,indicating that most of the CO2 captured by the carbonate can be transformed into chemicals;however,they cannot simply be emitted.The CO2 released from the decomposition of CaCO3 not only adjusted the ratio of H2 to CO but also eliminated cokes to guarantee the CO2 absorption-conversion cyclic stability in the absence of steam and at high temperatures. | Chengxiong Dang Shijie Wu Guangxing Yang Yonghai Cao Hongjuan Wang Feng Peng Hao Yu | 2020 | Journal of Energy Chemistry2020，29，4： | 1 |
| 5 | Sub-50 nm optical imaging in ambient air with 10× objective lens enabled by hyper-hemi-microsphere显示文摘Optical microsphere nanoscope has great potential in the inspection of integrated circuit chips for semiconductor industry and morphological characterization in biology due to its superior resolving power and label-free characteristics.However,its resolution in ambient air is restricted by the magnification and numerical aperture(NA)of microsphere.High magnification objective lens is required to be coupled with microsphere for nano-imaging beyond the diffraction limit.To overcome these challenges,in this work,high refractive index hyper-hemi-microspheres with tunable magnification up to 10×are proposed and realized by accurately tailoring their thickness with focused ion beam(FIB)milling.The effective refractive index is put forward to guide the design of hyper-hemi-microspheres.Experiments demonstrate that the imaging resolution and contrast of a hyper-hemi-microsphere with a higher magnification and larger NA excel those of a microsphere in air.Besides,the hyper-hemi-microsphere could resolve~50 nm feature with higher image fidelity and contrast compared with liquid immersed high refractive index microspheres.With a hyper-hemi-microsphere composed microscale compound lens configuration,sub-50 nm optical imaging in ambient air is realized by only coupling with a 10×objective lens(NA=0.3),which enhances a conventional microscope imaging power about an order of magnitude. | Guangxing Wu Yan Zhou Minghui Hong | 2023 | Light(Science & Applications)2023，12，3： | 1 |
| 6 | Production of high-purity hydrogen from paper recycling black liquor via sorption enhanced steam reforming显示文摘Environmentally friendly and energy saving treatment of black liquor(BL),a massively produced waste in Kraft papermaking process,still remains a big challenge.Here,by adopting a NieCaOeCa_(12)Al_(14)O_(33) bifunctional catalyst derived from hydrotalcite-like materials,we demonstrate the feasibility of producing high-purity H_(2)(~96%)with 0.9 mol H_(2) mol^(-1) C yield via the sorption enhanced steam reforming(SESR)of BL.The SESRBL performance in terms of H_(2) production maintained stable for 5 cycles,but declined from the 6th cycle.XRD,Raman spectroscopy,elemental analysis and energy dispersive techniques were employed to rationalize the deactivation of the catalyst.It was revealed that gradual sintering and agglomeration of Ni and CaO and associated coking played important roles in catalyst deactivation and performance degradation of SESRBL,while deposition of Na and K from the BL might also be responsible for the declined performance.On the other hand,it was demonstrated that the SESRBL process could effectively reduce the emission of sulfur species by storing it as CaSO_(3).Our results highlight a promising alternative for BL treatment and H_(2) production,thereby being beneficial for pollution control and environment governance in the context of mitigation of climate change. | Hanke Li Shijie Wu Chengxiong Dang Guangxing Yang Yonghai Cao Hongjuan Wang Feng Peng Hao Yu | 2021 | Green Energy & Environment2021，6，5： | 0 |
| 7 | A method of convolutional neural network based on frequency segmentation for monitoring the state of wind turbine blades显示文摘Wind turbine blades are prone to failure due to high tip speed,rain,dust and so on.A surface condition detecting approach based on wind turbine blade aerodynamic noise is proposed.On the experimental measurement data,variational mode decomposition filtering and Mel spectrogram drawing are conducted first.The Mel spectrogram is divided into two halves based on frequency characteristics and then sent into the convolutional neural network.Gaussian white noise is superimposed on the original signal and the output results are assessed based on score coefficients,considering the complexity of the real environment.The surfaces of Wind turbine blades are classified into four types:standard,attachments,polishing,and serrated trailing edge.The proposed method is evaluated and the detection accuracy in complicated background conditions is found to be 99.59%.In addition to support the differentiation of trained models,utilizing proper score coefficients also permit the screening of unknown types. | Weijun Zhu Yunan Wu Zhenye Sun Wenzhong Shen Guangxing Guo Jianwei Lin | 2023 | Theoretical & Applied Mechanics Letters2023，13，6： | 0 |
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