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| 1 | Unraveling a genetic roadmap for improved taste in the domesticated apple显示文摘Although taste is an important aspect of fruit quality, an understanding of its genetic control remains elusive in apple and other fruit crops. In this study, we conducted genomic sequence analysis of 497 Malus accessions and revealed erosion of genetic diversity caused by apple breeding and possible independent domestication events of dessert and cider apples. Signatures of selection for fruit acidity and size, but not for fruit sugar content, were detected during the processes of both domestication and improvement. Furthermore, we found that single mutations in major genes affecting fruit taste, including Ma1, MdTDT, and MdSOT2, dramatically decrease malate, citrate, and sorbitol accumulation, respectively, and correspond to important domestication events. Interestingly, Ma1 was identified to have pleiotropic effects on both organic acid content and sugar:acid ratio, suggesting that it plays a vital role in determining fruit taste. Fruit taste is unlikely to have been negatively affected by linkage drag associated with selection for larger fruit that resulted from the pyramiding of multiple genes with minor effects on fruit size. Collectively, our study provides new insights into the genetic basis of fruit quality and its evolutionary roadmap during apple domestication, pinpointing several candidate genes for genetic manipulation of fruit taste in apple. | Liao Liao Weihan Zhang Bo Zhang Ting Fang Xiao-Fei Wang Yarning Cai Collins Ogutu Lei Gao Gang Chen Xiaoqing Nie Jinsheng Xu Quanyan Zhang Yiran Ren Jianqiang Yu Chukun Wang Cecilia H.Deng Baiquan Ma Beibei Zheng Chun-Xiang You Da-Gang Hu Richard Espley Kui Lin-Wang Jia-Long Yao Andrew C.Allan Awais Khan Schuyler S.Korban Zhangjun Fei Ray Ming Yu-Jin Hao Li Li Yuepeng Han | 2021 | Molecular Plant2021，14，9： | 5 |
| 2 | Development of T. aestivum L.eH. californicum Alien Chromosome Lines and Assignment of Homoeologous Groups of Hordeum californicum Chromosomes显示文摘Hordeum californicum(2n=2x=14, HH) is resistant to several wheat diseases and tolerant to lower nitrogen. In this study, a molecular karyotype of H. californicum chromosomes in the Triticum aestivum L. cv. Chinese Spring(CS)eH. californicum amphidiploid(2n=6x=56, AABBDDHH) was established. By genomic in situ hybridization(GISH) and multicolor fluorescent in situ hybridization(FISH) using repetitive DNA clones(pTa71, pTa794 and pSc119.2) as probes, the H. californicum chromosomes could be differentiated from each other and from the wheat chromosomes unequivocally. Based on molecular karyotype and marker analyses, 12 wheatealien chromosome lines, including four disomic addition lines(DAH1, DAH3, DAH5 and DAH6), five telosomic addition lines(MtH7L,MtH1 S, MtH1 L, DtH6 S and DtH6L), one multiple addition line involving H. californicum chromosome H2, one disomic substitution line(DSH4) and one translocation line(TH7S/1BL), were identified from the progenies derived from the crosses of CSeH. californicum amphidiploid with common wheat varieties. A total of 482 EST(expressed sequence tag) or SSR(simple sequence repeat) markers specific for individual H. californicum chromosomes were identified, and 47, 50, 45, 49, 21, 51 and 40 markers were assigned to chromosomes H1, H2, H3, H4, H5, H6 and H7, respectively. According to the chromosome allocation of these markers, chromosomes H2,H3, H4, H5, and H7 of H. californicum have relationship with wheat homoeologous groups 5, 2, 6, 3, and 1, and hence could be designated as 5Hc, 2Hc, 6Hc, 3Hcand 1Hc, respectively. The chromosomes H1 and H6 were designated as 7Hcand 4Hc, respectively, by referring to SSR markers located on rye chromosomes. | Yuhui Fang Jingya Yuan Zhangjun Wang Haiyan Wang Jin Xiao Zhixi Yang Ruiqi Zhang Zengjun Qi Weigang Xu Lin Hu Xiu-E Wang | 2014 | Journal of Genetics and Genomics2014，41，8： | 2 |
| 3 | Nested hollow architectures of nitrogen-doped carbon-decorated Fe,Co,Ni-based phosphides for boosting water and urea electrolysis显示文摘Tailoring the nanostructure/morphology and chemical composition is important to regulate the electronic configuration of electrocatalysts and thus enhance their performance for water and urea electrolysis.Herein,the nitrogen-doped carbon-decorated tricomponent metal phosphides of FeP4 nanotube@Ni-Co-P nanocage(NC-FNCP)with unique nested hollow architectures are fabricated by a self-sacrifice template strategy.Benefiting from the multi-component synergy,the modification of nitrogen-doped carbon,and the modulation of nested porous hollow morphology,NC-FNCP facilitates rapid electron/mass transport in water and urea electrolysis.NC-FNCP-based anode shows low potentials of 248 mV and 1.37 V(vs.reversible hydrogen electrode)to attain 10 mA/cm^(2) for oxygen evolution reaction(OER)and urea oxidation reaction(UOR),respectively.In addition,the overall urea electrolysis drives 10 mA/cm^(2) at a comparatively low voltage of 1.52 V(vs.RHE)that is 110 mV lower than that of overall water electrolysis,as well as exhibits excellent stability over 20 h.This work strategizes a multi-shell-structured electrocatalyst with multi-compositions and explores its applications in a sustainable combination of hydrogen production and sewage remediation. | Jie Zhang Shoushuang Huang Ping Ning Peijun Xin Zhiwen Chen Qing Wang Kajsa Uvdal Zhangjun Hu | 2022 | Nano Research2022，15，3： | 2 |
| 4 | Single-wavelength-excited fluorogenic nanoprobe for accurate realtime ratiometric analysis of broad pH fluctuations in mitophagy显示文摘Mitophagy has a critical role in maintaining cellular homeostasis through acidic lysosomes engulfing excess or impaired mitochondria,thereby pH fluctuation is one of the most significant indicators for tracking mitophagy.Then such precise pH tracking demands the fluorogenic probe that has tailored contemporaneous features,including mitochondrial-specificity,excellent biocompatibility,wide pH-sensitive range of 8.0–4.0,and especially quantitative ability.However,available molecular probes cannot simultaneously meet all the requirements since it is extremely difficult to integrate multiple functionalities into a single molecule.To fully address this issue,we herein integrate two fluorogenic pH sensitive units,a mitochondria-specific block,cellpenetrating facilitator,and biocompatible segments into an elegant silica nano scaffold,which greatly ensures the applicability for real-time tracking of pH fluctuations in mitophagy.Most significantly,at a single wavelength excitation,the integrated pHsensitive units have spectra-distinguishable fluorescence towards alkaline and acidic pH in a broad range that covers mitochondrial and lysosomal pH,thus enabling a ratiometric analysis of pH variations during the whole mitophagy.This work also provides constructive insights into the fabrication of advanced fluorescent nanoprobes for diverse biomedical applications. | Xin Zhang Juan Chen Jiwen Hu Anna du Rietz Xiongyu Wu Ruilong Zhang Zhongping Zhang Kajsa Uvdal Zhangjun Hu | 2022 | Nano Research2022，15，7： | 1 |
| 5 | Well-defined sur- face ion-imprinted magnetic microspheres for facile onsite monitoring of lead ions at trace level in water 显示文摘 | Cui Yang Liu Jiaqi Hu Zhangjun | 2012 | Anal Methods2012，4，： | 1 |
| 6 | 有机电子器件中的纳米接触实现高效空穴注入显示文摘电极与半导体之间的欧姆接触是实现高效有机电子器件的关键.本文通过将DNA/表面活性剂复合物与双极性电子聚合物混合,获得了一种可印刷的杂化界面传输材料.研究发现DNA/表面活性剂复合物与导电聚合物之间可以进行有效的电荷转移,而纳米尺寸的发光二极管证明传输材料与导电聚合物间的纳米接触有助于电荷的传输和注入.该新型材料可应用于高效有机发光二极管、太阳能电池和场效应晶体管. | Qingzhen Bian Chiara Musumeci Chuanfei Wang reas Skallberg Yongzhen Chen Zhangjun Hu EPeter Münger Kajsa Uvdal Mats Fahlman Olle Inganas | 2021 | Science Bulletin2021，66，9： | 1 |
| 7 | Phosphorus-doped Fe_(7)S_(8)@C nanowires for efficient electrochemical hydrogen and oxygen evolutions:Controlled synthesis and electronic modulation on active sites显示文摘Developing low-cost,efficient,and stable non-precious-metal electrocatalysts with controlled crystal structure,morphology and compositions are highly desirable for hydrogen and oxygen evolution reactions.Herein,a series of phosphorus-doped Fe_(7)S_(8)nanowires integrated within carbon(P-Fe_(7)S_(8)@C)are rationally synthesized via a one-step phosphorization of one-dimensional(1D)Fe-based organicinorganic nanowires.The as-obtained P-Fe_(7)S_(8)@C catalysts with modified electronic configurations present typical porous structure,providing plentiful active sites for rapid reaction kinetics.Density functional calculations demonstrate that the doping Fe_(7)S_(8)with P can effectively enhance the electron density of Fe_(7)S_(8)around the Fermi level and weaken the Fe-H bonding,leading to the decrease of adsorption free energy barrier on active sites.As a result,the optimal catalyst of P-Fe_(7)S_(8)-600@C exhibits a relatively low overpotential of 136 mV for hydrogen evolution reaction(HER)to reach the current density of 10 mA/cm^(2),and a significantly low overpotential of 210 mV for oxygen evolution reaction(OER)at 20 mA/cm^(2)in alkaline media.The work presented here may pave the way to design and synthesis of other prominent Fe-based catalysts for water splitting via electronic regulation. | Thanh-Tung Le Xiao Liu Peijun Xin Qing Wang Chunyan Gao Ye Wu Yongjiang Zhangjun Hu Shoushuang Huang Zhiwen Chen | 2021 | Journal of Materials Science & Technology2021，，15： | 0 |
| 8 | Microseismic Concentration Zones before and after the February 12,2014 M_S 7.3 Yutian Earthquake and the Possible Indication of an Earthquake Risk Zone显示文摘Since 2001, there have occurred in succession the 2001 Kunlun Mountains M S8. 1earthquake,the 2008 Wenchuan M S8. 0 earthquake,the 2010 Yushu M S7. 1 earthquake and the 2012 Lushan M S7. 0 earthquake in the periphery of the Bayan Har block. By comparison of the characteristics of seismic strain release variations before and after the Kunlun Mountains M S8. 1 earthquake in the same time length in the geodynamical related regions,we found that the seismic strain release was obviously enhanced after the earthquake in the Longmenshan area,Batang area,and the NS-trending valleys at the west of the Hot Spring Basin. The Wenchuan earthquake occurred in the first area,and the Yushu earthquake is related to the second area. After the earthquake rupture occurred on the East Kunlun fault zone on the northern boundary of the Bayan Har Block,crustal materials on the south side of the fault zone migrated to the southeast,leading to a concentration of tectonic deformation in the Longmenshan thrust belt, e ventually rupturing on the Longmenshan thrust belt. This earthquake case illustrates that seismicity enhancement zones are possibly prone to long-term destructive earthquakes. After the M S7. 3 earthquake in Yutian,Xinjiang on February 12,2014,earthquake frequency and seismic strain release markedly increased in the junction area between the eastern Qilian Mountain tectonic belt and the Altun Tagh fault zone,where more attention should be paid to the long-term seismic risk. | Hu Chaozhong Chen Dan Yang Panxin Xiong Renwei Li Zhangjun | 2015 | Earthquake Research in China2015，29，2： | 0 |
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