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| 1 | Integrated System of Solar Cells with Hierarchical NiCo2O4 Battery-Supercapacitor Hybrid Devices for Self-Driving Light-Emitting Diodes显示文摘An integrated system has been provided with a-Si/H solar cells as energy conversion device,NiCo2O4 battery-supercapacitor hybrid(BSH)as energy storage device,and light emitting diodes(LEDs)as energy utilization device.By designing three-dimensional hierarchical NiCo2O4 arrays as faradic electrode,with capacitive electrode of active carbon(AC),BSHs were assembled with energy density of 16.6 Wh kg-1,power density of 7285 W kg-1,long-term stability with 100% retention after 15,000 cycles,and rather low self-discharge.The NiCo2O4//AC BSH was charged to 1.6 V in 1 s by solar cells and acted as reliable sources for powering LEDs.The integrated system is rational for operation,having an overall efficiency of 8.1% with storage efficiency of 74.24%.The integrated system demonstrates a stable solar power conversion,outstanding energy storage behavior,and reliable light emitting.Our study offers a precious strategy to design a self-driven integrated system for highly efficient energy utilization. | Yuliang Yuan Yangdan Lu BeiEr Jia Haichao Tang Lingxiang Chen YuJia Zeng Yang Hou Qinghua Zhang Qinggang He Lei Jiao Jianxing Leng Zhizhen Ye Jianguo Lu | 2019 | Nano-Micro Letters2019，11，3： | 5 |
| 2 | Nickel single atom overcoordinated active sites to accelerate the electrochemical reaction kinetics for Li-S cathode显示文摘Lithium-sulfur(Li-S)batteries with high theoretical energy density are promising advanced energy storage devices.However,shuttling of dissolute lithium polysulfide(LiPSs)and sluggish conversion kinetics impede their applications.Herein,single nickel(Ni)atoms on two-dimensional(2D)nitrogen(N)-doped carbon with Ni-N_(4)-O overcoordinated structure(SANi-N_(4)-O/NC)are prepared and firstly used as a sulfur host of Li-S batteries.Due to the efficient polysulfides traps and highly LiPSs conversion effect of SANi-N_(4)-O/NC,the electrochemical performance of Li-S batteries obviously improved.The batteries can well operate even under high sulfur loading(5.8 mg cm^(-2))and lean electrolyte(6.1μL mg^(-1))condition.Meanwhile,density functional theory(DFT)calculations demonstrate that Ni single atom’s active sites decrease the energy barriers of conversion reactions from Li_(2)S_(8)to Li2S due to the strong interaction between SANi-N_(4)-O/NC and LiPSs.Thus,the kinetic conversion of LiPSs was accelerated and the shuttle effect is suppressed on SANi-N_(4)-O/NC host.This study provides a new design strategy for a 2D structure with single-atom overcoordinated active sites to facilitate the fast kinetic conversion of LiPSs for Li-S cathode. | Juan Zhu Xinyue Wang Tian Ke Mingji Jia Biyu Jin Yuanyuan Li Qiwei Yang Lanhui Ren Yongyuan Ren Dangguo Cheng Jianguo Lu Xiang Gao Qinggang He Yang Hou Xiaoli Zhan Qinghua Zhang | 2023 | Journal of Energy Chemistry2023，，3： | 2 |
| 3 | Nitrogen-doped carbon nanotube-encapsulated nickel nanoparticles assembled on graphene for efficient CO2 electroreduction显示文摘Exploring 3 D hybrid nanocarbons encapsulated with metal nanoparticles(NPs)are recently considered as emerging catalysts for boosting CO2 electroreduction reaction(CRR)under practical and economic limits.Herein,we report a one-step pyrolysis strategy for fabricating N-doped carbon nanotube(CNT)-encapsulated Ni NPs assembled on the surface of graphene(N/NiNPs@CNT/G)to efficiently convert CO2 into CO.In such 3 D hybrid,the particle size of Ni NPs that coated by five graphitic carbon layers is less than 100 nm,and the amount of N dopants introduced into graphene with countable CNTs is determined to 7.27 at%.Thanks to unique CNT-encapsulated Ni NPs structure and N dopants,the achieved N/NiNPs@CNT/G hybrid displays an exceptional CRR activity with a high Faradaic efficiency of 97.7%and large CO partial current density of 7.9 mA/cm2 at-0.7 V,which outperforms those reported metallic NPs loaded carbon based CRR electrocatalysts.Further,a low Tafel slope of 134 mV/dec,a turnover frequency of 387.3 CO/h at-0.9 V,and tiny performance losses during long-term CRR operation are observed on N/NiNPs@CNT/G.Experimental observations illustrate that the Ni NPs encapsulated by carbon layers along with N dopants are of great importance in the conversion of CO2 into CO with high current density. | Tingting Wang Jian Yang Jiayi Chen Qinggang He Zhongjian Li Lecheng Lei Jianguo Lu Michael K.H.Leung Bin Yang Yang Hou | 2020 | Chinese Chemical Letters2020，31，6： | 1 |
| 4 | Microstructures and ablation properties of 3D 4-directional C f /ZrC–SiC composite in a plasma wind tunnel environment显示文摘 | Yan Ma Qinggang Li Shaoming Dong Zhi Wang Guopu Shi Haijun Zhou Zhen Wang Ping He | 2014 | Ceramics International2014，，7： | 1 |
| 5 | 肝细胞肝癌经肝动脉化疗栓塞后破裂:2例报告及系统回顾(英文)显示文摘Objective: Rupture of hepatocellular carcinoma (HCC) following transarterial embolization/chemoembolization (TAE/TACE) is a rare but life-threatening complication. The aim of the study was to explore the incidence, risk factors, clinical characteristics, treatment, and outcomes of this complication. Methods: We described two cases and reviewed all cases of ruptured HCC after TAE/TACE reported in the literature. Results: Our search yielded 32 cases of ruptured HCC after TAE/TACE. The overall incidences were 0.45% per patient and 0.21% per session. The mean age of the patients was 57.4 years (range 28-90 years, n=26, No. of cases with available information). Males accounted for 81% of cases (21/26). The 50% of the cases had histories of primary hypertension, diabetes or peripheral artery disease (6/12). Mean diameter of the tumors was 11.4 cm (range 3-20 cm, n=27). The 100% of cases had superficial or exophytic tumors (23/23). Portal vein thrombosis was presented in 61.5% of patients (8/13). The median interval between TAE/TACE and rupture was 2 days (range 0 hour-30 days, n=31). Management choices included emergency TAE, surgery, and conservative treatment. The overall median survival time was 7 days (n=19). Conclusion: Rupture of HCC following TAE/TACE is relatively rare but potentially life-threatening. The management is difficult and prognosis is poor. Large tumor size, superficial or exophytic tumors as well as portal vein thrombosis and comorbidities such as primary hypertension, diabetes or peripheral artery disease may be predisposing factors for rupture. | Ping Sun Zifang Song Qinggang Hu Jun Xiong Shaobo Hu Ruiqing He Qichang Zheng | 2013 | The Chinese-German Journal of Clinical Oncology2013，12，2： | 1 |
| 6 | Remarkable improvement of cyclic stability in Li-O2 batteries using ruthenocene as a redox mediator显示文摘Nonaqueous Li-O2 batteries attract attention for their theoretical specific energy density.However,due to the difficulty of decomposition of Li2 O2,Li-O2 batteries have high charge overpotential and poor cycling life.So all kinds of catalysts have been studied on the cathode.Compared to heterogeneous solid catalysts,soluble catalysts achieve faster and more effective transport of electrons by reversible redox pairs.Here,we first report ruthenocene(Ruc) as a mobile redox mediator in a Li-O2 battery.0.01 mol/L Ruc in the electrolyte effectively reduces the charging voltage by 610 mV.Additionally,Ruc greatly increases the cycling life by four-fold(up to 83 cycles) with a simple ketjen black(KB) cathode.The results of SEM,XPS and XRD confirm that less discharge product residue accumulated after recharge.To verify the reaction mechanisms of the mediato r,free energy profiles of the possible reaction pathways based on DFT are provided. | Cuicui Zhu Yiping Wang Ling Shuai Yizhao Tang Ming Qiu Jian Xie Jia Liu Wen Wen Hengquan Chen Suifei Nan Mei Dou Qinggang He | 2020 | Chinese Chemical Letters2020，31，7： | 1 |
| 7 | 重离子在MRAM中引起的辐照效应研究显示文摘Nonvolatile memories play a critical role for storing significant data,the programs of micro control system and scientific observation data[1].Unfortunately,conventional charge non-volatile memories,EEPROM or PROM are hardly to suitable the new missions nowadays,such as the requirements of more than 10 years on-orbit service and ultra-deep space exploration missions,etc.Representation of novel NVRAM technologies of magnetoresistive random access memories(MRAM)utilize magnetic bits of a magnetic tunnel junction(MTJ)[2]to store binary data have inherently endurance to the direct ionization induced by the charge particle.Therefore,it is an ideal candidate general-purpose memory to be used in space-borne microelectronics. | Zhao Peixiong Liu Jie Liu Tianqi Ji Qinggang Cai Chang Li Dongqing He Ze Ye Bing Mo Lihua Zhai Pengfei Sun Youmei Hou Mingdong | 2018 | IMP & HIRFL Annual Report2018，，1： | 0 |
| 8 | Extracting Lotus Fields Using the Spectral Characteristics of GF-1 Satellite Data显示文摘The lotus(Nelumbo nucifera Gaertn.)is an aquatic plant that grows in shallow water and has long been cultivated in South China.It can improve the incomes of farmers and plays an important role in alleviating poverty in rural China.However,a modern method is required to accurately estimate the area of lotus fields.Lotus has spectral characteristics similar to those of rice,grassland,and shrubs.The features surrounding areas where it is grown are complex,small,and fragmented.Few studies have examined the remote sensing extraction of lotus fields,and automatic extraction and mapping are still challenging methods.Here,we compared the spectral characteristics of lotus fields and other ground objects and devised a remote sensing method for the rapid extraction of lotus fields.Using this method,the extraction accuracy of lotus was 96.3%.The Kappa coefficient was 0.926,which is higher than those of the unsupervised K-means classification,Mahalanobis distance,and support vector machine supervised classification,and demonstrates the potential of this method for extracting and mapping lotus fields by remote sensing. | Dongping Zha Haisheng Cai Xueling Zhang Qinggang He Liting Chen Chunqing Qiu Shufang Xia | 2022 | Phyton-International Journal of Experimental Botany2022，91，10： | 0 |
| 9 | Regulating adsorption ability toward polysulfides in a porous carbon/Cu_(3)P hybrid for an ultrastable high-temperature lithium-sulfur battery显示文摘Lithium-sulfur batteries(LSBs)can work at high temperatures,but they suffer from poor cycle life stability due to the“shuttle effect”of polysulfides.In this study,pollen-derived porous carbon/cuprous phosphide(PC/Cu_(3)P)hybrids were rationally synthesized using a one-step carbonization method using pollen as the source material,acting as the sulfur host for LSBs.In the hybrid,polar Cu_(3)P can markedly inhibit the“shuttle effect”by regulating the adsorption ability toward polysulfides,as confirmed by theoretical calculations and experimental tests.As an example,the camellia pollen porous carbon(CPC)/Cu_(3)P/S electrode shows a high capacity of 1205.6 mAh g^(−1) at 0.1 C,an ultralow capacity decay rate of 0.038%per cycle after 1000 cycles at 1 C,and a rather high initial Coulombic efficiency of 98.5%.The CPC/Cu_(3)P LSBs can work well at high temperatures,having a high capacity of 545.9 mAh g^(−1) at 1 C even at 150℃.The strategy of the PC/Cu_(3)P hybrid proposed in this study is expected to be an ideal cathode for ultrastable high-temperature LSBs.We believe that this strategy is universal and worthy of in-depth development for the next generation energy storage devices. | Yichuan Guo Rabia Khatoon Jianguo Lu Qinggang He Xiang Gao Xiaopeng Yang Xun Hu Yang Wu Jiale Lian Zhoupeng Li Zhizhen Ye | 2021 | Carbon Energy2021，3，6： | 0 |
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