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| 1 | 2020 Roadmap on two-dimensional nanomaterials for environmental catalysis显示文摘Environmental catalysis has drawn a great deal ofattention due to its clean ways to produce useful chemicals or carry out some chemical processes.Photocatalysis and electrocatalysis play important roles in these fields.They can decompose and remove organic pollutants from the aqueous environment,and prepare some fine chemicals.Moreover,they also can carry out some important reactions,such as 02 reduction reaction(ORR),O2 evolution reaction(OER),H2 evolution reaction(HER),CO2 reduction reaction(C02 RR),and N2 fixation(NRR).For catalytic reactions,it is the key to develop high-performance catalysts to meet the demand fortargeted reactions.In recentyears,two-dimensional(2 D) materials have attracted great interest in environmental catalysis due to their unique layered structures,which offer us to make use of their electronic and structural characteristics.Great progress has been made so far,including graphene,black phosphorus,oxides,layered double hydroxides(LDHs),chalcogenides,bismuth-based layered compounds,MXenes,metal organic frameworks(MOFs),covalent organic frameworks(COFs),and others.This content drives us to invite many famous groups in these fields to write the roadmap on two-dimensional nanomaterials for environmental catalysis.We hope that this roadmap can give the useful guidance to researchers in future researches,and provide the research directions. | Yulu Yang Mingguang Wu Xingwang Zhu Hui Xu Si Ma Yongfeng Zhi Hong Xia Xiaoming Liu Jun Pan Jie-Yinn Tang Siang-Piao Chai Leonardo Palmisano Francesco Parrino Junli Liu Jianzhong Ma Ze-Lin Wang Ling Tan Yu-Fei Zhao Yu-Fei Song Pardeep Singh Pankaj Raizada Deli Jiang Di Li R.A.Geioushy Jizhen Ma Jintao Zhang Song Hu Rongjuan Feng Gang Liu Minghua Liu Zhenhua Li Mingfei Shao Neng Li Jiahe Peng Wee-Jun Ong Nikolay Kornienko Zhenyu Xing Xiujun Fan Jianmin Ma | 2019 | Chinese Chemical Letters2019，30，12： | 2 |
| 2 | Fast and highly reversible Na^(+)intercalation/extraction in Zn/Mg dual-doped P2-Na_(0.67)MnO_(2)cathode material for high-performance Na-ion batteries显示文摘P2-type layered Na_(0.67)MnO_(2)has been considered to be a promising candidate cathode material for sodium ion batteries.Nevertheless,the undesired phase transitions during operation and the large Na^(+)radius induced sluggish ion diffusion remain the stumbling blocks to realize its high performance.Herein,we propose a Zn/Mg co-doping strategy,which is proved to have bifunctional effects.First,relative to the pristine P2-Na_(0.67)MnO_(2)and the single-ion(Zn/Mg)doped samples,the Zn/Mg dual-doped P2-Na_(0.67)MnO_(2)demonstrates a lower Mn^(3+)/Mn^(4+)ratio and a higher lattice O content,which facilitate the structural stability of the cathode material.More intriguingly,the Zn/Mg co-doping gives rise to enlarged interplanar spacing,which provides spacious ion diffusion channels for fast Na^(+)intercalation/extraction.As a result,the Zn/Mg dual-doped sample exhibits a high Na^(+)diffusion coefficient and a solid-solution reaction during charge/discharge,with a cell volume change determined to be only 0.55%.Taking advantages of the above favorable features,the Zn/Mg dual-doped P2-Na_(0.67)MnO_(2)demonstrates a high rate performance with 67.2 mAh·g^(-1)delivered at 10 C and a decent cycling stability with a capacity retention of 93.8%achieved at 1 C after 100 cycles.This work introduces the Zn/Mg co-doping strategy to simultaneously improve the cycling stability and rate capability of P2-Na_(0.67)MnO_(2),which may offer a promising avenue for further performance enhancement of the layered Na-ion batteries cathode materials. | Xiaoqin Huang Deli Li Haijian Huang Xiao Jiang Zeheng Yang Weixin Zhang | 2021 | Nano Research2021，14，10： | 2 |
| 3 | Complete convergence and almost sure convergence of weighted sums of random variables显示文摘 | Deli Li M. Bhaskara Rao Tiefeng Jiang Xiangchen Wang | 1995 | Journal of Theoretical Probability1995，，1： | 1 |
| 4 | Complete conver- gence and almost sure convergence of weighted sums of random variables显示文摘 | Li Deli Rao M B Jiang T F | 1995 | J Theor Paobab1995，8，： | 1 |
| 5 | Modifi- ers-assisted formation of nickel nanoparticles and their catalytic application to p-nitrophenol reduction 显示文摘 | JIANG Zhifeng XIE Jimin JIANG Deli | 2013 | Cryst Eng Comm2013，15，： | 1 |
| 6 | Complete convergence and almost sure convergence of weighted sums of random variables显示文摘 | Deli Li M. Bhaskara Rao Tiefeng Jiang Xiangchen Wang | 1995 | Journal of Theoretical Probability1995，，1： | 1 |
| 7 | Controllable synthesis of Fluorapatite nanocrystals with various morphologies: Effects of pH value and chelating reagent 显示文摘 | Min Chen Deli Jiang Di Li | 2009 | Alloys Compd2009，485，12： | 1 |
| 8 | Shape-controlled syn- thesis of F-substituted hydroxyapatite microcrystals in the presence of Na2 EDTA and citric acid 显示文摘 | Deli Jiang Di Li Jimin Xie | 2010 | Colloid Interface Sci2010，350，1： | 1 |
| 9 | Relative contributions of biotic and abiotic factors to the spatial variation of litter stock in a mature subtropical forest显示文摘Aims Dead plant material(i.e.litter)is the major source of soil organic matter and thus plays a fundamental role in regulating soil carbon cycling in global forest ecosystems.The storage of litter is jointly determined by its production from plants and decomposition in a given environment.However,only few studies have explored the relative importance of en-vironmental(i.e.abiotic)and plant(i.e.biotic)factors in driving the spa-tial variation of litter mass.The objective of this study is to quantify the relative contributions of biotic and abiotic factors in affecting the spatial variation of aboveground litter stock in a mature subtropical forest.Methods The aboveground litter mass was sampled in 187 grids of a 20-hm forest dynamics plot in a subtropical broad-leave forest in eastern China.The contributions of environmental variables,topographical and species variables on litter stocks were quantified by the boosted regression tree analysis.Important Findings The mean aboveground litter stock was 367.5 g m^(−2) in the Tiantong dynamics forest plot across all the 187 grids.The litter stock ranged from 109.2 to 831.3 g m^(−2) and showed a large spatial variation with the coefficient of variance as 40.8%.The boosted regression tree analysis showed that slope elevation and soil moisture were the most influential variables on the spatial variation of litter stock.The relatively influence of abiotic factors(environmental and topographical factors)was 71.4%,which is larger than biotic factors(28.6%).Overall,these findings sug-gest that abiotic factors play a more important role than plants in driving the spatial variation of aboveground litter stock in the subtropical forest.Given that the global carbon-cycle models have been aiming to refine from the hundred kilometers to sub-kilometer scale,this study highlights the urgency of a better understanding of the spatial variation of litter stock on the fine scale. | Jing Wang Qingsong Yang Yang Qiao Deli Zhai Lifen Jiang Guopeng Liang Xiaoying Sun Ning Wei Xihua Wang Jianyang Xia | 2019 | Journal of Plant Ecology2019，12，4： | 1 |
| 10 | Carbon nanodots as reductant and stabi- lizer for one-pot sonochemical synthesis of amorphous carbon-supported silver nanopar- ticles for electrochemical nonenzymatic H202 sensing显示文摘 | Deli Jiang Yuan Zhang Minhu Huang et al | 2014 | Journal of Electroanalyti- cal Chemistry2014，728，： | 1 |
| 11 | A new visible light active muhifunctional ternary composite based on TiO2-ln203 nanocrystals heterojunction decorated porous graphiticcarbon nitride for photocatalytic treatment of hazardous pollutant and t/2 evolution显示文摘 | Jiang Zhifeng Jiang Deli Yan Zaoxue Liu Dong Qian Kun Xie Jimin | 2015 | Applied Catalysis B: Environmental2015，170，： | 1 |
| 12 | SYNTHESIS OF FUNCTIONAL MACROMOLECULE INTERMEDIATE THROUGH ACYLATION CATALYZED BY [Emim]Cl-AlCl_3 IONIC LIQUID显示文摘Acylation reaction of anthracene with oxalyl chloride in the presence of [Emim]C1-A1C13 ionic liquid has been investigated. Pure 1,2-aceanthryenedione, which is used as intermediate of functional aromatic polymer material, was obtained by recrystalling the reaction mixture with aether and was determined by GC/MS, 1HNMR and FTIR analysis. The influences of various parameters, such as the contents of AlCl3 in [Emim]C1-A1C13, the amount of acylation agent, amount of [Emim]C1-A1C13, reaction temperature and reaction time were investigated. The optimum conditions were as follows: the molar fraction of A1C13 in ionic liquid [x(AlCl3)] being 0.67 , molar ratio of ionic liquid to anthracene being 2:1 , molar ratio of oxalyl chloride to anthracene being 2:1, reaction temperature being 40℃ and reaction time being 6h. Under above conditions, the yield and selectivity of 1,2-aceanthrylenedione can reach 91.5% and 98.3% respectively. Further more, [Emim]C1-A1C13 ionic liquid, compared with metal halides such as AlCl3, was found to catalyze the reaction as a novel environmental friendly catalyst and solvent and can be reused. | CHEN Min JIANG Deli ZHANG Chunyan YU Long YAN Yongsheng | 2007 | Chinese Journal of Reactive Polymers2007，16，1： | 1 |
| 13 | Design and experiment of nail tooth picking up device for strip type residual film recycling and baling machine显示文摘In order to solve the problem of residual film pollution caused by large area of cotton mulched planting in Xinjiang,a strip type residual film recycling and baling machine was designed,which can complete mulching film picking up,impurities separation,baling and other operations.The picking up device,as the key part of residual film recycling machine,was designed and analyzed.The kinematics of the pick-up nail tooth was analyzed,and its motion equation,motion trajectory and the conditions for completing the film pick-up were determined.And the key parameters were determined by analyzing the conditions of no missing picking and the stress of the residual film.According to the Box-Benhnken test design principle,field experiments were carried out with the forward speed of machine,the pickup speed ratio and the number of auxiliary film removing mechanisms as the key experimental factors,and the residual film pickup rate,the cotton stalk content and the residual film winding rate as the operation performance indexes of the picking up device.The mathematical models between the experimental factors and indexes were established,and the effect of each factor was analyzed.Through multi-objective parameter optimization and field experiment,the optimal combination of operation parameters was obtained as follows:the forward speed of machine of 1.67 m/s,the pickup speed ratio of 1.13,and the number of auxiliary film removing mechanisms of 6.Under this parameter combination,the pickup rate of residual film was 88.9%,the cotton stalk content in recycled residual film of 3.9%,and the residual film winding rate of 1.5%.The absolute error with the theoretical value was less than 0.6%.The research results show that the picking up device has stable operation performance and good residual film recycling effect,which meets the design and practical operation requirements. | Deli Jiang Limin Yan Xuegeng Chen Yisong Mo Jiacheng Yang | 2023 | International Journal of Agricultural and Biological Engineering2023，16，6： | 0 |
| 14 | SYNTHESIS OF 1,2-ACEANTHRYLENEDIONE THROUGH ACYLATION OF ANTHRACENE WITH OXALYL CHLORIDE显示文摘Acylation of anthracene and oxalyl chloride in the presence of anhydrous AlCl3 was investigated. Pure 1,2-aceanthrylenedione, which is used as new functional macromolecule, was prepared by extraction and recrystallation. The structure of 1,2-aceanthrylenedione was identified by measure of melting point, GC/MS, FTIR and 1HNMR analyses. The influences of various parameters, such as solvent, dosage of catalyst, molar ratio of anthracene to oxalyl chloride, reaction temperature, and reaction time were studied. The anhydrous AlCl3 was found to catalyze the reaction with high yeild and good selectivity. When the reaction temperature is 303K, reaction time is 5h and molar ratio of anthracene to oxalyl chloride is 1:2, the yield and selectivity of 1,2-aceanthrylenedione is 83.8 % and 92.3% respectively. | ZHANG Chunyan CHEN Min YU Long JIANG Deli YAN Yongsheng | 2007 | Chinese Journal of Reactive Polymers2007，16，1： | 0 |
| 15 | Sedimentary Features of Shallow Ancient River Channels on the Northern Shelf of the South China Sea显示文摘Quaternary buried ancient river channels are widespread in the shallow-level sediments of the northern shelf of the South China Sea. The sedimentary sequence mainly of fluvial deposits comprise an important component part of the low-stand system tract and transgressive system tract in the study region. The plannar variation and spatial association of the sedimentary features such as incised valley fillings, deltaic foreset wedges and block slides of shelf-marginal fans reflect the palaeogeographic environment during the fall of the regional sea level in the northern part of the South China Sea. Based on the high-resolution seismic reflection data and gelogical data from boreholes, the present paper makes an integrated interpretation of the Quaternary ancient river channels in the shallow sediments of the study area, studies the sedimentary features of the ancient channels such as their spatial distribution, seismic facies reflection indicators, sedimentary facies and sand -body types, and discusses | Kou Yangqi and Du Deli 2nd Marine Geological Investigation Party, MGMR, Guangzhou, Guangdong Jiang M inxi | 1995 | Acta Geologica Sinica(English Edition)1995，69，1： | 0 |
| 16 | Anthelmintics nitazoxanide protects against experimental hyperlipidemia and hepatic steatosis in hamsters and mice显示文摘Lipid metabolism disorders contribute to hyperlipidemia and hepatic steatosis.It is ideal to develop drugs simultaneous improving both hyperlipidemia and hepatic steatosis.Nitazoxanide is an FDA-approved oral antiprotozoal drug with excellent pharmacokinetic and safety profile.We found that nitazoxanide and its metabolite tizoxanide induced mild mitochondrial uncoupling and subsequently activated AMPK in Hep G2 cells.Gavage administration of nitazoxanide inhibited high-fat diet(HFD)-induced increases of liver weight,blood and liver lipids,and ameliorated HFD-induced renal lipid accumulation in hamsters.Nitazoxanide significantly improved HFD-induced histopathologic changes of hamster livers.In the hamsters with pre-existing hyperlipidemia and hepatic steatosis,nitazoxanide also showed therapeutic effect.Gavage administration of nitazoxanide improved HFD-induced hepatic steatosis in C57BL/6J mice and western diet(WD)-induced hepatic steatosis in Apoe-/-mice.The present study suggests that repurposing nitazoxanide as a drug for hyperlipidemia and hepatic steatosis treatment is promising. | Fengfeng Li Man Jiang Minghui Ma Xuyang Chen Yidan Zhang Yixin Zhang Yuanyuan Yu Yunfeng Cui Jiahui Chen Hui Zhao Zhijie Sun Deli Dong | 2022 | Acta Pharmaceutica Sinica B2022，12，3： | 0 |
| 17 | Determination and Analysis of Amino Acid Content in Maca from Different Habitats and Varieties显示文摘[Objectives]To determine and analyze amino acid content in Maca from different habitats and varieties.[Methods]Maca from two habitats and three colors were selected and a kind of turnip commonly used was to fake Maca.After optimizing the hydrolysis conditions,100 mg Maca samples were hydrolyzed in the concentration of 6 mol/L hydrochloric acid at 110℃for 24 h.The content range of amino acids in each sample was detected by HPLC.[Results]The average total content of amino acids in Maca was 9.52 g/100 g.Yunnan yellow Maca contained 16 kinds of amino acids,including 7 kinds of human essential amino acids,accounting for 17.2%of the total amino acids while Yunnan purple Maca held 16 kinds of amino acids,counting 7 kinds of human essential amino acids,accounting for 16.5%of the total amino acids.The amino acid ratio coefficient method also showed that the two kinds of Maca had higher nutritional value than the others.15 kinds of amino acids were detected in Yunnan black Maca,including 6 kinds of essential amino acids,accounting for 9.60%of the total amino acids.Among amino acids in Yunnan Maca,the highest content was Arg.A total of 12 kinds of amino acids,together with 6 essential human amino acids,were determined in Peru black Maca,accounting for 11.6%of the total amino acids.In Peru black Maca the highest concentration of amino acid was Pro.It was noteworthy that the amino acid species were comprehensive in Maca,and high level of amino acids resulted in high nutritional value.Its specific amino acid composition ratio was obviously different from Turnip,the counterfeit goods to deceive customers.[Conclusions]The method of automatic amino acid analyzer is simple and accurate,and can be used for the identification and content determination of amino acids in Maca as amino acid is an essential nutrient in Maca. | Yuting LI Ziyi LI Lin JIANG Deli XIAO | 2022 | Medicinal Plant2022，13，3： | 0 |
| 18 | 100 km wear-free sliding achieved by microscale superlubric graphite/DLC heterojunctions under ambient conditions显示文摘Wear-free sliding between two contacted solid surfaces is the ultimate goal in the effort to extend the lifetime of mechanical devices,especially when it comes to inventing new types of micro-ele ctromechanical systems where wear is often a major obstacle.Here we report experimental observations of wear-free sliding for a micrometer-sized graphite flake on a diamond-like-carbon(DLC) surface under ambient conditions with speeds up to 2.5 m/s,and over a distance of 100 km.The coefficient of friction(COF) between the microscale graphite flake,a van der Waals(vdW) layered material and DLC,a non-vdW-layered material,is measured to be of the order of 10^(-3),which belongs to the superlubric regime.Such ultra-low COFs are also demonstrated for a microscale graphite flake sliding on six other kinds of non-vdW-layered materials with sub-nanometer roughness.With a synergistic analysis approach,we reve al the underlying mechanism to be the combination of interfacial vdW interaction,atomic-smooth interfaces and the low normal stiffness of the graphite flake.These features guarantee a persistent full contact of the interface with weak interaction,which contributes to the ultra-low COFs.Together with the extremely high in-plane strength of graphene,wear-free sliding is achieve d.Our results broaden the scope of superlubricity and promote its wider application in the future. | Deli Peng Jin Wang Haiyang Jiang Shuji Zhao Zhanghui Wu Kaiwen Tian Ming Ma Quanshui Zheng | 2022 | National Science Review2022，9，1： | 0 |
| 19 | Peculiar dynamical properties of plutonium hydrides显示文摘在 PuH 的结构和系列是的现在的工作, PuH 2 被 PuH 2 的分析势能功能从被导出的 B3LYP/SDD 方法定义。伪古典的分子的反应动力学的分析被执行学习 Pu 的州状态的过程(7 f g )+H2(x(g+) 。这被发现反应 Pu (7 F8 )+ H2 (x (g+) PuH2 (x7 (B1 ) 没有阀值。有 PuH 2 的主要产品的钚的同时的加氢过程理论上第一次被证明。 | MENG Daqiao ZHU Zhenghe LUO Deli JIANG Gang | 2006 | Progress in Natural Science:Materials International2006，16，3： | 0 |
| 20 | On scientif ic expedition tourism of desert region:a case of eastern Ulan Buh Inner Mongolia显示文摘Desert-based adventure tourism is a rapidly expanding tourism market segment after the late 20th century around the world.Perhaps the most signif icant factor in the development of desert adventure tourism is the extent to which common tourists are really engaged in scientif ic expedition.Inner Mongolia has long been considered as the resources accumulation area of desert tourism.The investigation on the Ulan Buh Desert has discovered that the desert animals,the vegetation,the insects,the fungus,the landform and the climate are impressive for both the researchers and the mass tourists.After the resources investigation a survey was carried out in 2007 to get the detailed information of the tourists' attitude toward the planning desert scientif ic product in the Ulan Buh Desert.Based on the resources and market analysis,this paper tries to make a planning of the desert scientif ic expedition tour of the Ulan Buh Desert.The planning includes the functional division,expedition route design,tour-explaining system,facility of safety guaranty and service planning,and the professional training base. | Liu Jun Chen Yuansheng Cheng Shengkui Jiang Yiyi Qi Deli | 2008 | Ecological Economy2008，4，4： | 0 |
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