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| 1 | Coaxial multi-interface hollow Ni-AI203-ZnO nanowires tailored by atomic layer deposition for selective- frequency absorptions显示文摘 | Lili Yan Jia Liu Shichao Zhao Bin Zhang Zhe Gao Huibin Ge Yao Chen Maosheng Cao Yong Qin | 2017 | Nano Research2017，10，5： | 13 |
| 2 | Microbial aerosol characteristics in highly polluted and nearpristine environments featuring different climatic conditions显示文摘There is an increasing interest in understanding ambient bioaerosols due to their roles both in health and in climate. Here, we deployed an Ultraviolet Aerodynamic Particle Sizer to monitor viable(fluorescent) bioaerosol concentration levels at city centers(highly polluted) and their corresponding suburbs(near pristine)(total 40 locations) in 11 provinces featuring different climate zones in China between July 16 and 28, 2013. The concentration levels of viable bioaerosol particles(Bio PM) of [0.5 lm were measured, and corresponding percentages of Bio PM%(biological fraction of total PM) and Bio PM2.5%(biological fraction of PM2.5) in particulate matter(PM)and Bio PM, respectively, were determined. For some key cities, indoor viable bioaerosol levels were also obtained.In addition, bacterial structures of the air samples collected across these monitoring locations were studied using pyrosequencing. Bio PM concentration levels ranged from2.1 9 104 to 2.4 9 105/m3 for city centers [Bio PM% =6.4 %(±6.3 %)] and 0.5 9 104 to 4.7 9 105/m3 for suburbs [Bio PM% = 10 %(±8.7 %)]. Distinctive bioaerosol size distribution patterns were observed for different climate zones, e.g., some had fluorescence peaks at 3 lm, while the majority had peaks at 1 lm. Ambient bacterial aerosol community structures were also found different for different geophysical locations. Results suggest that there was a poor overall relationship between PM and Bio PM across 40 monitoring locations(R2= 0.081, two-tailed P value =0.07435). Generally, city centers had higher PM concentrations than suburbs, but not Bio PM and Bio PM%. Indoor bioaerosol levels were found at least tenfold higher than those corresponding outdoors. Bacillus was observed to dominate the bacterial aerosol community in the air sample. | Kai Wei Yunhao Zheng Jing Li Fangxia Shen Zhuanglei Zou Hanqing Fan Xinyue Li Chang-yu Wu Maosheng Yao | 2015 | Science Bulletin2015，60，16： | 10 |
| 3 | Microbial aerosol chemistry characteristics in highly polluted air显示文摘Aerosol chemistry is often studied without considering microbial involvements. Here, we investigated time-and size-resolved bacterial aerosol dynamics in air. Under high particulate matter(PM) polluted episodes, bacterial aerosols exhibited a viability of up to 50%–70% in the 0.56–1 μm size range, at which elevated levels of SO42-, NO3- and NH4+ were concurrently observed.Engineered or acclimated for both industrial use, bacteria such as Psychrobacter spp., Massilia spp., Acinetobacter lwoffii,Exiguobacteriumaurantiacum and Bacillusmegaterium were shown to have experienced massive abundance shifts in polluted air on early mornings and late afternoons, on which rapid new particle formation events were widely reported. Here, Psychrobacter spp. were shown to account for >96% abundance at a corresponding PM2.5 level of 208 μg/m3. These observed bacterial aerosol changes corresponded to the PM2.5 mass peak shift from 3.2–5.6 μm to the high viability size range of 0.56–1 μm. Additionally,elevated levels of soluble Na, Ca, Mg, K, Al, Fe and P elements, required for bacterial growth, were observed to co-occur with those significant bacterial aerosol structure shifts in the air. For particular time-resolved PM2.5 pollution episodes, Acinetobacter,Psychrobacter and Massilia were shown to alternate in dominating the time-resolved aerosol community structures. The results from a HYSPLIT trajectory model simulation suggested that air mass transport played a minor role in affecting the observed bacterial aerosol structure dynamics. All the data here suggested that airborne bacteria in the size range of 0.56–1 μm could be extensively involved in aerosol chemistry in highly polluted humid air. | Ting Zhang Xinyue Li Minfei Wang Haoxuan Chen Maosheng Yao | 2019 | Science China Chemistry2019，62，8： | 8 |
| 4 | In situ airborne virus inactivation by microwave irradiation显示文摘Infectious diseases cause tremendous costs of both human and economy annually.Previously,we have studied the bacterial,fungal,and allergen aerosol inactivation by direct microwave irradiation.Here,we further investigated its effects on airborne viruses.MS2 coliphage used as a human model virus was aerosolized and exposed to the direct microwave irradiation for*2 min at three different power levels(700,385,and 119 W).In addition to the survival rate,the viral genes before and after the microwave treatments were also examined using PCR and gel electrophoresis.Direct exposure of airborne MS2viruses to the microwave irradiation at 700 W for less than2 min was shown to result in more than 90%inactivation efficiency,about 65%at medium power level(385 W),and 50%at the lowest level(119 W).The aerosol inactivation rate followed a linear relationship with the microwave exposure time(R2=0.9889).Scanning electron images revealed visible damages to the viral surface after the exposure.Damages were also observed to the viral RNA genes coding for coat proteins,among which the A protein gene was completely destroyed.This study demonstrated that even without the filtration the direct microwave irradiation could also achieve rapid inactivation of viral aerosols.The information obtained can provide useful guidance on the development of microwave-based viral threat mitigation solutions in a closed or semi-closed space. | Yan Wu Maosheng Yao | 2014 | Chinese Science Bulletin2014，59，13： | 3 |
| 5 | Circular dichroism-like response of terahertz wave caused by phase manipulation via all-silicon metasurface显示文摘Chiral metasurfaces based on asymmetric meta-atoms have achieved artificial circular dichroism(CD),spin-dependent wavefront control,near-field imaging,and other spin-related electromagnetic control.In this paper,we propose and experimentally verify a scheme for achieving high-efficiency chiral response similar to CD of terahertz(THz)wave via phase manipulation.By introducing the geometric phase and dynamic phase in an all-silicon metasurface,the spin-decoupled terahertz transmission is obtained.The giant circular dichroism-like effect in the transmission spectrum is observed by using a random phase distribution for one of the circular polarization components.More importantly,the effect can be adjusted when we change the area of the metasurface illuminated by an incident terahertz beam.In addition,we also demonstrate the spin-dependent arbitrary wavefront control of the transmitted terahertz wave,in which one of the circularly polarized components is scattered,while the other forms a focused vortex beam.Simulated and experimental results show that this method provides a new idea for spin selective control of THz waves. | Jie Li Chenglong Zheng Guocui Wang Jitao Li Hongliang Zhao Yue Yang Zhang Zhang Maosheng Yang Liang Wu Jining Li Yating Zhang Yan Zhang Jianquan Yao | 2021 | Photonics Research2021，9，4： | 3 |
| 6 | Three Gorges Dam: friend or foe of riverine greenhouse gases?显示文摘Dams are often regarded as greenhouse gas(GHG) emitters. However, our study indicated that the world’s largest dam, the Three Gorges Dam(TGD), has caused significant drops in annual average emissions of CO, CHand NO over 4300 km along the Yangtze River, accompanied by remarkable reductions in the annual export of CO(79%), CH(50%) and NO(9%) to the sea. Since the commencement of its operation in 2003, the TGD has altered the carbonate equilibrium in the reservoir area, enhanced methanogenesis in the upstream, and restrained methanogenesis and denitrification via modifying anoxic habitats through long-distance scouring in the downstream. These findings suggest that ‘large-dam effects’ are far beyond our previous understanding spatiotemporally, which highlights the fundamental importance of whole-system budgeting of GHGs under the profound impacts of huge dams. | Jinren Ni Haizhen Wang Tao Ma Rong Huang Philippe Ciais Zhe Li Yao Yue Jinfeng Chen Bin Li Yuchun Wang Maosheng Zheng Ting Wang Alistair G.L.Borthwick | 2022 | National Science Review2022，9，6： | 3 |
| 7 | Synthesis of selective PAK4 inhibitors for lung metastasis of lung cancer and melanoma cells显示文摘The p21 activated kinase 4(PAK4) is serine/threonine protein kinase that is critical for cancer progression.Guided by X-ray crystallography and structure-based optimization,we report a novel subseries of C-3-substituted 6-ethynyl-1 H-indole derivatives that display high potential and specificity towards group Ⅱ PAKs.Among these inhibitors,compound 55 exhibited excellent inhibitory activity and kinase selectivity,displayed superior anti-migratory and anti-invasive properties against the lung cancer cell line A549 and the melanoma cell line B16.Compound 55 exhibited potent in vivo antitumor metastatic efficacy,with over 80% and 90% inhibition of lung metastasis in A549 or B16-BL6 lung metastasis models,respectively.Further mechanistic studies demonstrated that compound 55 mitigated TGF-β1-induced epithelial-mesenchymal transition(EMT). | Peilu Song Fan Zhao Dahong Li Jiqiang Qu Miao Yao Yuan Su Hanxun Wang Miaomiao Zhou Yujie Wang Yinli Gao Feng Li Dongmei Zhao Fengjiao Zhang Yu Rao Mingyu Xia Haitao Li Jian Wang Maosheng Cheng | 2022 | Acta Pharmaceutica Sinica B2022，12，6： | 2 |
| 8 | Plant flowers transmit various bio-agents through air显示文摘Growing air pollution,known as'April snow',by fluffy catkins from plant flowering was frequently observed during the Spring time in China.Current efforts mainly focus on controlling catkin release,while their public health and environmental impacts are unknown.Here,using culturing,microscopic and sequence methods we found that the flying catkins carry a significant amount of bio-agents(bacteria,fungal,viruses,and pollens),e.g.,up to 6.33×10^4 bacterial and 7.46×10^5 fungal cells per catkin.Abundant pollens from plants were also found riding on the flying catkins.For collected fluffy catkins,bacterial Paracoccus,Massilia,fungal Ophiocordyceps,Arthrocladiella,pollen Robina,Pickeringia,Pinus,and viral family Genomoviridae,to name a few,were found to be dominant.With infection and allergic potentials,the detected microbial structures on the fluffy catkins were different from those of local air,varying from one location to another.Being not just white pollution,flying plant fluffy catkins were discovered here also acting as a cloud of biological agents,and further actions need to be taken urgently to understand and limit their environmental and ecological consequences. | Siyu XU Maosheng YAO | 2020 | Science China Earth Sciences2020，63，10： | 2 |
| 9 | Regulating bifunctional flower-like NiFe_(2)O_(4)/graphene for green EMI shielding and lithium ion storage显示文摘Environment and energy are the eternal hot topics in the world,multiloculated microscale materials have attracted great attention in the field of electromagnetic interference(EMI)shielding and lithium ions storage.Herein,a novel flower-like NiFe_(2)O_(4)/graphene composite with adjustable structure was fabricated as EMI shielding material and anode material of lithium-ion batteries.NiFe_(2)O_(4)/graphene composite is a potential green EMI shielding material.The EMI shielding effectiveness(SE)increases with the increase of graphene content in NiFe_(2)O_(4)/graphene composite,and the total EMI SE of NiFe_(2)O_(4)/graphene with 73.6 wt.%graphene increases from 26.5 to 40.6 d B with the increase of frequency in 2–18 GHz.Furthermore,it exhibits long-life and large capacity lithium storage performance at high current density.The capacity reaches 732.79 m Ah g^(-1)after 100 cycles at 0.1 A g^(-1),recovering to more than 139%from the minimum capacity value.After 300 cycles at 0.5 A g^(-1),the capacity increases to 688.5 mAh g^(-1).The initial capacities at 2 and 5 A g^(-1)are 704.9 and 717.8 mAh g^(-1),and remain 297.9 and 203.2 m Ah g^(-1)after 1000 cycles.The distinguished EMI shielding performance and electrochemical performance are mainly ascribed to the structure regulation of NiFe_(2)O_(4)/graphene composite,as well as the synergistic effect of graphene and NiFe_(2)O_(4).This research opens up infinite opportunities for the application of multifunctional and interdisciplinary materials. | Lihua Yao Wenqiang Cao Jianguo Zhao Qi Zheng Yuchang Wang Shang Jiang Qiliang Pan Jie Song Youqi Zhu Maosheng Cao | 2022 | Journal of Materials Science & Technology2022，，32： | 2 |
| 10 | Negatively and positively charged bacterial aerosol concentration and diversity in natural environments显示文摘Bioaerosol charge information is of vital importance for their electrostatic collection. Here, electrostatic means and molecular tools were applied to studying bioaerosol charge dynamics. Positively or negatively charged bioaerosols were collected using an electrostatic sampler operated with a field strength of 1.1 kV cm 1 at a flow rate of 3 L min 1 for 40 min. Those with fewer or no charges bypassing the sampler were also collected using a filter at the downstream of the electrostatic sampler in one environment. The experiments were independently conducted three times in three different environments. The collected bacterial aerosols were cultured directly on agar plates at 26°C, and the colony forming units (CFU) were manually counted. In addition, the CFUs were washed off from the agar plates, and further subjected to polymerase chain reaction (PCR) and denaturing gradient gel electrophoresis (DGGE) for culturable diversity analysis. The results revealed remarkable differences in positively and negatively charged culturable bacterial aerosol concentration and diversity among the studied environments. In the office environment, negatively charged culturable bacterial aerosols appeared to dominate (P = 0.0489), while in outdoor and hotel environments both polarities had similar concentration levels (P = 0.078, P = 0.88, respectively). DGGE patterns for positively charged culturable bacterial aerosols were shown strikingly different from those of negatively charged regardless of the sampling environments. In addition, for each of the environments positively charged culturable bacterial aerosols collected were found to have more band pattern similarity with those positively charged for respective regions of agar plates than those negatively charged, and vice versa. The information developed here is useful for developing efficient electrostatic sampling protocols for bioaerosols. | SHEN FangXia KAI Wei YAO MaoSheng | 2013 | Chinese Science Bulletin2013，58，26： | 1 |
| 11 | Inactivation of bacteria and fungus aerosolsusing microwave irradiation显示文摘 | WU Yan YAO Maosheng | 2010 | Journal of Aerosol Science2010，41，7： | 1 |
| 12 | Investigation of transition metal ion doping behaviors on TiO2 nanoparticles显示文摘 | Jianhua Chen Maosheng Yao Xiaolin Wang | 2008 | Journal of Nanoparticle Research2008，10，1： | 1 |
| 13 | Airborne endotoxin in fine particulate matter in Beijing显示文摘 | Guan Tianjia Yao Maosheng Wang Junxia | 2014 | Atmospheric Environment2014，97，： | 1 |
| 14 | Rapid magnetic removal of aqueous heavy metals and their relevant mechanisms using nanoscale zero valent iron (nZVI) particles显示文摘 | Pengpeng Huang Zhengfang Ye Wuming Xie Qi Chen Jing Li Zhencheng Xu Maosheng Yao | 2013 | Water Research2013，，12： | 1 |
| 15 | Monitoring of bioaerosol inhalation risks in different environments using a six-stage Andersen sampler and the PCR-DGGE method显示文摘 | Zhenqiang Xu Maosheng Yao | 2013 | Environmental Monitoring and Assessment2013，，5： | 1 |
| 16 | Development of a novel conductance-based technology for environmental bacterial sensing显示文摘In this study, a simple impedance based technology for measuring bacterial concentrations was developed. The measurement system includes the signal amplification, copper probes and a sample loader. During the experiments, the conductance of Bacillus subtilis var niger, Pseudomonas fluorescens, and Escherichia coli were measured using the combination of a pre-amplifier and a lock-in amplifier. The conductance data were modeled verses the bacterial concentrations. Results indicated that the relationship between the conductance of bacterial suspensions and their concentrations follows a generic model: Y=C1+C2×e ( X/C3 ) , where Y is the conductance (S), X is the bacterial concentration (Number/mL: abbreviated to N/mL) for all species tested, and C1 3 are constants. Gram negative P. fluorescens and E. coli assumed similar conductance curves, which were flatter than that of gram positive B. subtilis var niger. For P. fluorescens and E. coli the culturing technique resulted in higher concentration levels (statistically significant) from 2 to 4 times that measured by the impedance based technology. For B. subtilis var niger, both methods resulted in similar concentration levels. These differences might be due to membrane types, initial culturability and the obtained conductance curves. The impedance based technology here was shown to obtain the bacterial concentration instantly, holding broad promise in realtime monitoring biological agents. | SHEN FangXia TAN MiaoMiao XU Hong XU ZhenCheng YAO MaoSheng | 2013 | Chinese Science Bulletin2013，58，4： | 1 |
| 17 | Airflow resistance and bio-fihering performanee of carbon nanotube filters and current facepieee respirators显示文摘 | ZOU Zhuanglci YAO Maosheng | 2015 | Journal of Aerosol Science2015，79，： | 1 |
| 18 | High-sensitivity modulation of electromagnetically induced transparency analog in a THz asymmetric metasurface integrating perovskite and graphene显示文摘Active control of the electromagnetically induced transparency(EIT)analog is desirable in photonics development.Here,we theoretically and experimentally proposed a novel terahertz(THz)asymmetric metasurface structure that can possess high-sensitivity modulation under extremely low power density by integrating perovskite or graphene.Using the novel metasurface structure with the perovskite coating,the maximum amplitude modulation depth(AMD)of this perovskite-based device reached 490.53%at a low power density of 12.8037 mW/cm^(2).In addition,after the novel THz metasurface structure was combined with graphene,this graphene-based device also achieved high AMD with the maximum AMD being 180.56%at 16.312 mW/cm^(2),and its transmission amplitude could be electrically driven at a low bias voltage.The physical origin of this modulation was explained using a two-oscillator EIT model.This work provides a promising platform for developing high-sensitivity THz sensors,light modulators,and switches. | TONGLING WANG TENGTENG LI HAIYUN YAO YUYING LU XIN YAN MAOYONG CAO LANJU LIANG MAOSHENG YANG JIANQUAN YAO | 2022 | Photonics Research2022，10，10： | 0 |
| 19 | Hybrid metasurface using graphene/graphitic carbon nitride heterojunctions for ultrasensitive terahertz biosensors with tunable energy band structure显示文摘Integrating novel materials is critical for the ultrasensitive,multi-dimensional detection of biomolecules in the terahertz(THz)range.Few studies on THz biosensors have used semiconductive active layers with tunable energy band structures.In this study,we demonstrate three THz biosensors for detecting casein molecules based on the hybridization of the metasurface with graphitic carbon nitride,graphene,and heterojunction.We achieved lowconcentration detection of casein molecules with a 3.54 ng/m L limit and multi-dimensional sensing by observing three degrees of variations(frequency shift,transmission difference,and phase difference).The favorable effect of casein on the conductivity of the semiconductive active layer can be used to explain the internal sensing mechanism.The incorporation of protein molecules changes the carrier concentration on the surface of the semiconductor active layer via the electrostatic doping effect as the concentration of positively charged casein grows,which alters the energy band structure and the conductivity of the active layer.The measured results indicate that any casein concentration can be distinguished directly by observing variations in resonance frequency,transmission value,and phase difference.With the heterojunction,the biosensor showed the highest response to the protein among the three biosensors.The Silvaco Atlas package was used to simulate the three samples'energy band structure and carrier transport to demonstrate the benefits of the heterojunction for the sensor.The simulation results validated our proposed theoretical mechanism model.Our proposed biosensors could provide a novel approach for THz metasurface-based ultrasensitive biosensing technologies. | HAIYUN YAO ZHAOQING SUN LANJU LIANG XIN YAN YARUWANG MAOSHENG YANG XIAOFEI HU ZIQUN WANG ZHENHUA LI MENG WANG CHUANXIN HUANG QILI YANG ZHONGJUN TIAN JIANQUAN YAO | 2023 | Photonics Research2023，11，5： | 0 |
| 20 | Assessment of heavy metal pollution in Laizhou Bay(China)using the ecological risk index and the integrated biomarker response of the goby Acanthogobius ommaturus显示文摘We used the Integrated Biological Responses version 2(IBRv2)method to evaluate the biological eff ects of heavy metals in the sediments in Laizhou Bay,China on the benthic goby Acanthogobius ommaturus.In December 2018,gobies and sediments were collected from 15 stations.We measured the activities of defense enzymes and the contents of malondialdehyde(MDA)and metallothionein(MT)in the goby liver as well as the levels of heavy metals in the sediments and goby muscle tissue.Most of the heavy metal concentrations in sediment at each station were below the Class I criteria set by Chinese Standards for Marine Sediment Quality,and the Håkanson ecological risk index suggested low risk for the heavy metals.We found that A.ommaturus could eff ectively accumulate mercury,cadmium,arsenic,and zinc and that the contents of MT and MDA and the activities of glutathione peroxidase and glutathione reductase were suitable biomarkers of heavy metal pollution in this species.The IBRv2 method integrated these four biomarkers and discriminated stations according to heavy metal pollution.Higher IBRv2 values suggested more adverse eff ects in gobies,corroborating more serious heavy metal contamination.The stations with high IBRv2 values and high contents of heavy metals were mainly distributed in the west and northeast parts of the bay.These results show that the IBRv2 approach is a feasible strategy for assessing heavy metal pollution through biological response and biological status and that it can be implemented for environmental monitoring in Laizhou Bay. | Maosheng LIU Hua XU Qiang ZOU Fei FANG Shan SUN Yuting ZHAO Xin HE Yonghui BO Lei YAO Yan FANG | 2023 | Journal of Oceanology and Limnology2023，41，4： | 0 |
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