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1A micro-adjusting attitude mechanism for autonomous drilling robot end-effector显示文摘Drilling end-effector is a key unit in autonomous drilling robot.The perpendicularity of the hole has an important influence on the quality of airplane assembly.Aiming at the robot drilling perpendicularity,a micro-adjusting attitude mechanism and a surface normal measurement algorithm are proposed in this paper.In the mechanism,two rounded eccentric discs are used and the small one is embedded in the big one,which makes the drill’s point static when adjusting the drill’s attitude.Thus,removal of drill’s point position after adjusting the drill attitude can be avoided.Before the micro-adjusting progress,four non-coplanar points in space are used to determine a unique sphere.The normal at the drilling point is measured by four laser ranging sensors.The adjusting angles at which the motors should be rotated to adjust attitude can be calculated by using the deviation between the normal and the drill axis.Finally,the motors will drive the two eccentric discs to achieve micro-adjusting progress.Experiments on drilling robot system and the results demonstrate that the adjusting mechanism and the algorithm for surface normal measurement are effective with high accuracy and efficiency.YUAN PeiJiang WANG QiShen SHI ZhenYun WANG TianMiao WANG ChengKun CHEN DongDong SHEN LiHeng 2014Science China(Information Sciences)2014,57,12:8
2Two-dimensional material separation membranes for renewable energy purification, storage, and conversion显示文摘The current energy crisis has prompted the development of new energy sources and energy storage/conversion devices. Membranes, as the key component, not only provide enormous separation potential for energy purification but also guarantee stable and high-efficiency operation for rechargeable batteries and fuel cells. Remarkably, two-dimensional(2D) material separation membranes have attracted intense attention on their excellent performance in energy field applications, owing to high mechanical/chemical stability, low mass transport resistance, strict sizeexclusion, and abundant modifiable functional groups. In this review, we concentrate on the recent progress of 2D membrane and introduce 2D membranes based on graphene oxide(GO), MXenes, 2D MOFs, 2D COFs, and 2D zeolite nanosheets, which are applied in membrane separation(H2 collection and biofuel purification) and battery separators(vanadium flow battery, Li–S battery, and fuel cell). The mass transport mechanism, selectivity mechanism, and modification methods of these 2D membranes are stated in brief, mainly focusing on interlayer dominant membranes(GO and MXenes) and pore dominant membranes(MOFs, COFs, and zeolite nanosheets). In conclusion, we highlight the challenges and outlooks of applying 2D membranes in energy fields.Liheng Dai Kang Huang Yongsheng Xia Zhi Xu 2021Green Energy & Environment2021,6,2:6
3Prediction of cutting forces in flank milling of parts with non-developable ruled surfaces显示文摘Predicting the cutting forces required for five-axis flank milling is a challenging task due to the difficulties involved in determining the Undeformed Chip Thickness(UCT) and CutterWorkpiece Engagement(CWE). To solve these problems, this paper presents a new mechanistic cutting force model based on the geometrical analysis of a flank milling process. In the model,the part feature and corresponding cutting location data are taken as input information. The UCT considering cutter runout is calculated according to the instantaneous feed rate of the element cutting edges. A solid-discrete-based method is used to precisely and efficiently identify the CWE between the end mill and the surface being machined. Then, after calibrating the specific force coef-ficients, the mechanistic milling force can be obtained. During the validation process, two practical operations, three-axis flank milling of a vertical surface and five-axis flank milling of a nondevelopable ruled surface, are conducted. Comparisons between predicted and measured cutting forces demonstrate the reliability of the proposed cutting force model.Liping WANG Hao SI Liheng GU 2019Chinese Journal of Aeronautics2019,32,7:6
4Broadband perovskite quantum dot spectrometer beyond human visual resolution显示文摘The quantum dot spectrometer,fabricated by integrating different quantum dots with an image sensor to reconstruct the target spectrum from spectral-coupled measurements,is an emerging and promising hyperspectrometry technology with high resolution and a compact size.The spectral resolution and spectral range of quantum dot spectrometers have been limited by the spectral variety of the available quantum dots and the robustness of algorithmic reconstruction.Moreover,the spectrometer integration of quantum dots also suffers from inherent photoluminescence emission and poor batch-to-batch repeatability.In this work,we developed nonemissive in situ fabricated MA_(3)Bi_(2)X_(9) and Cs_(2)SnX_(6)(MA=CH_(3)NH_(3);X=Cl,Br,I)perovskite-quantum-dot-embedded films(PQDFs)with precisely tunable transmittance spectra for quantum dot spectrometer applications.The resulting PQDFs contain in situ fabricated perovskite nanocrystals with homogenous dispersion in a polymeric matrix,giving them advantageous features such as high transmittance efficiency and good batch-to-batch repeatability.By integrating a filter array of 361 kinds of PQDFs with a silicon-based photodetector array,we successfully demonstrated the construction of a perovskite quantum dot spectrometer combined with a compressive-sensing-based total-variation optimization algorithm.A spectral resolution of ~1.6 nm was achieved in the broadband of 250-1000 nm.The performance of the perovskite quantum dot spectrometer is well beyond that of human eyes in terms of both the spectral range and spectral resolution.This advancement will not only pave the way for using quantum dot spectrometers for practical applications but also significantly impact the development of artificial intelligence products,clinical treatment equipment,scientific instruments,etc.Xiaoxiu Zhu Liheng Bian Hao Fu Lingxue Wang Bingsuo Zou Qionghai Dai Jun Zhang Haizheng Zhong 2020Light(Science & Applications)2020,9,1:5
5Establishment and Characterization of a Cell Based Artificial Antigen-Presenting Cell for Expansion and Activation of CD8^+ T Cells Ex Vivo显示文摘Artificial antigen-presenting cells are expected to stimulate the expansion and acquisition of optimal therapeutic features of T cells before infusion. Here CD32 that binds to a crystallizable fragment of IgG monoclonal antibody was genetically expressed on human K562 leukemia cells to provide a ligand for T-cell receptor. CD86 and 4-1BBL,which are ligands of co-stimulating receptors of CD28 and 4-1BB,respectively,were also expressed on K562 cells. Then we accomplished the artificial antigen-presenting cells by coupling K32/CD86/4-1BBL cell with OKT3 monoclonal antibody against CD3,named K32/CD86/4-1BBL/OKT3 cells. These artificial modified cells had the abilities of inducing CD8+ T cell activation,promoting CD8+ T cell proliferation,division,and long-term growth,inhibiting CD8+ T cell apoptosis,and enhancing CD8+ T cell secretion of IFN-γ and perforin. Furthermore,antigen-specific cytotoxic T lymphocytes could be retained in the culture stimulated with K32/CD86/4-1BBL/OKT3 cells at least within 28 days. This approach was robust,simple,reproducible and economical for expansion and activation of CD8+ T cells and may have important therapeutic implications for adoptive immunotherapy.Weijuan Gong Mingchun Ji Zhengfeng Cao Liheng Wang Yayun Qian Maozhi Hu Li Qian Xingyuan Pan 2008Cellular & Molecular Immunology2008,5,1:5
6The Future is in the Past: Projecting and Plotting the Potential Rate of Growth and Trajectory of the Structural Change of the Chinese Economy for the Next 20 Years显示文摘基于集中假设并且从 1950 ~ 2010 指东方亚洲高执行的经济的经验,这份报纸在下一 20 年投射并且阴谋中国经济的潜在的生长率。当 2015 的潜在的 GDP 生长率将仍然超过 8% 时,它预言购买调整的人均的 GDP 的潜在的生长率从 2015 ~ 2035 在 6.02% 点驱动同等值一般水准,它暗示自从 2012,认识到的增长率没到达它的潜力。基于投射的人均的 GDP 并且在横越田野的比较上,而且,纸从 2015 ~ 2035 阴谋中国经济的结构的变化的轨道。结果显示出那:主要工业的增值份额将比雇用份额更快掉的(i) ;(ii ) 第二等的工业愿望衰落的增值份额和雇用份额将介绍点其拐弯处将可能在 2020 和 2025 之间来的转换 U 形状;(iii ) 增值和第三级的工业的雇用份额将连续地增加。Jun Zhang Liheng Xu Fang Liu 2015China & World Economy2015,23,1:4
7Sodium Tanshinone Ⅱ A sulfonate for acute myocardial infarction:a systematic review and Meta-analysis显示文摘OBJECTIVE: To investigate the efficacy and safety of Sodium tanshinone ⅡA sulfonate(STS) plus the conventional treatment on acute myocardial infarction(AMI) patients.METHODS: We searched several electrical databases and hand searched several Chinese medical journals up to January 2019. Randomized controlled trials(RCTs) comparing STS plus conventional treatment with conventional treatment were retrieved.Study screening, data extraction, quality assessment, and data analysis were conducted in accordance with the Cochrane standards.RESULTS: Sixteen trials involving 1383 people were included. The Meta-analysis showed STS combined with conventional treatment was a better treatment option than conventional treatment alone in reducing the risk of mortality, heart failure, arrhythmia and shock. In addition, STS was associated with improvement in left ventricular ejection fraction(LVEF) and left ventricular end diastolic dimension(LVEDD). No significant difference of STS was found on recurrent angina and recurrent AMI. However,the safety of STS remained uncertain for limited data.CONCLUSION: Compared with conventional treatment alone, STS combined with conventional treatment may provide more benefits for patients with AMI. Due to the fact that the overall quality of all included trials is generally low, further large-scale high quality trials are warranted.LIAN Baotao ZENG Ruixiang LIAO Pengda GUO Liheng ZHANG Minzhou CHEN Yuanfang 2021Journal of Traditional Chinese Medicine2021,41,1:4
8Toward Sustainable,Economic,and Tailored Production of Cellulose Nanomaterials显示文摘This paper introduces a concentrated di-carboxylic acid(DCA) hydrolysis process for the integrated production of thermally stable and carboxylated cellulose nanocrystals(CNCs) and cellulose nanofibrils(CNFs). The DCA hydrolysis process addressed several issues associated with mineral acid hydrolysis for CNC production, such as cellulose loss and acid recovery. The surface and morphological properties of the cellulose nanomaterials resulting from the DCA hydrolysis process can be tailored simply by controlling the severity of DCA hydrolysis. To further reduce cost, a lowtemperature(≤80℃) hydrotropic chemical process using p-toluenesulfonic acid(p-Ts OH) was also introduced to rapidly fractionate raw lignocelluloses for the production of lignin containing cellulose nanofibrils(LCNFs) and lignin nanoparticles(LNPs). The LCNF surface hydrophobicity and morphology can be tailored by controlling the fractionation severity, i.e., the extent of delignification. The lignin also improved the thermal stability of LCNFs. LNPs can be easily separated by diluting the spent acid liquor to below the p-Ts OH minimal hydrotropic concentration of approximately 10%. p-Ts OH can also be easily recovered by re-concentrating the diluted spent liquor after lignin precipitation. We believe that these two novel processes presented here have the potential to achieve true sustainable, economic, and tailored production of cellulose nanomaterials, suitable for a variety of applications.HuiYang Bian JunYong Zhu LiHeng Chen Roland Gleisner 2017Paper And Biomaterials2017,2,4:4
9A panel of monoclonal antibodies against the prion protein proves that there is no prion protein in human pancreatic ductal epithelial cells显示文摘Prion diseases are a group of neurodegenerative diseases that are fatal. The study of these unique diseases in China is hampered by a lack of resources. Amongst the most important resources for biological study are monoclonal antibodies. Here, we characterize a panel of monoclonal antibodies specific for cellular prion protein by enzyme-linked immunosorbent assay(ELISA), immunofluorescent staining, flow cytometry, and western blotting. We identify several antibodies that can be used for specific applications and we demonstrate that there is no prion protein expression in human pancreatic ductal epithelial cells(HPDC).Liheng Yang Yan Zhang Lipeng Hu Ying Zhu Man-Sun Sy Chaoyang Li 2014Virologica Sinica2014,29,4:3
10Phonon scattering and exciton localization: molding exciton flux in two dimensional disorder energy landscape显示文摘Two dimensional excitonic devices are of great potential to overcome the dilemma of response time and integration in current generation of electron or/and photon based systems.The ultrashort diffusion length of exciton arising from ultrafast relaxation and low carrier mobility greatly discounts the performance of excitonic devices.Phonon scattering and exciton localization are crucial to understand the modulation of exciton flux in two dimensional disorder energy landscape,which still remain elusive.Here,we report an optimized scheme for exciton diffusion and relaxation dominated by phonon scattering and disorder potentials in WSe2 monolayers.The effective diffusion coefficient is enhanced by>200%at 280 K.The excitons tend to be localized by disorder potentials accompanied by the steadily weakening of phonon scattering when temperature drops to 260 K,and the onset of exciton localization brings forward as decreasing temperature.These findings identify that phonon scattering and disorder potentials are of great importance for long-range exciton diffusion and thermal management in exciton based systems,and lay a firm foundation for the development of functional excitonic devices.Pengfei Qi Yang Luo Beibei Shi Wei Li Donglin Liu Liheng Zheng Zhixin Liu Yanglong Hou Zheyu Fang 2021eLight2021,1,1:3
11FROM-GC: 30 m global cropland extent derived through multisource data integration显示文摘We report on a global cropland extent product at 30-m spatial resolution developed with two 30-m global land cover maps(i.e.FROM-GLC,Finer Resolution Observation and Monitoring,Global Land Cover;FROM-GLC=agg)and a 250-m cropland probability map.A common land cover validation sample database was used to determine optimal thresholds of cropland probability in different parts of the world to generate a cropland/noncropland mask according to the classification accuracies for cropland samples.A decision tree was then applied to combine two 250-m cropland masks:one existing mask from the literature and the other produced in this study,with the 30-m global land cover map FROM-GLC-agg.For the smallest difference with country-level cropland area in Food and Agriculture Organization Corporate Statistical(FAOSTAT)database,a final global cropland extent map was composited from the FROM-GLC,FROM-GLC-agg,and two masked crop=land layers.From this map FROM-GC(Global Cropland),we estimated the global cropland areas to be 1533.83 million hectares(Mha)in 2010,which is 6.95 Mha(0.45%)less than the area reported by the Food and Agriculture Organization(FAO)of the United Nations for the year 2010.A country-by=country comparison between the map and the FAOSTAT data showed a linear relationship(FROM-GC=1.05*FAOSTAT-1.2(Mha)with R^(2)=0.97).Africa,South America,Southeastern Asia,and Oceania are the regions with large discrepancies with the FAO survey.Le Yu Jie Wang Nicholas Clinton Qinchuan Xin Liheng Zhong Yanlei Chen Peng Gong 2013International Journal of Digital Earth2013,6,6:3
12Up-conversion fluorescence biosensor for sensitive detection of CA-125 tumor markers显示文摘Sensitive and specific bioassays of tumor markers are critical for early cancer detection and treatment.In recent years,lanthanide(Ln3+)doped upconversion nanoparticles(UCNPs)have attracted wide attentions in tumor markers detectio n.Herein,we co mbined NaYF4:Yb,Tm and silver nanoparticles,serving as energy donor and receptor,respectively,to form an up-conversion fluorescence based inhibitory tumor marker biosensor system.The tumor marker CA-125 molecules are labeled with silver NPs,and the energy transfer fluorescent signal can be detected between the UCNPs and the silver NP receptors.The biosensor shows good stability,high sensitivity and selectivity in the tumor marker concentration range from 5 to 100 ng/mL,as well as a detection limit of 120 pg/mL.Due to the advantage of ease of fabrication and operation,low cost and high information capacity,this technology holds great potential for the clinical applications.Jingshi Liu Sai Xu Liheng Sun Songtao Hu Jiao Sun Min Liu Cui Ma Haipeng Liu Ziqing Wang Ying Yang Biao Dong Decheng Hong 2019Journal of Rare Earths2019,37,9:3
13Recent advances in integrated optical directed logic operations for high performance optical computing: a review显示文摘Optical directed logic(DL)is a novel logic operation scheme that employs electrical signals as operands to control the working states of optical switches to perform the logic functions.This review first provides an overview of the concept and working principle of DL.The developing trends of DL computing are then discussed in detail,including the fundamental optical DL gates,combinational optical DL operations,reconfigurable logic computing,low power optical logic computing,and programmable photonic network.The concluding remarks provide an outlook on the DL future development and its impacts in optical computing.Ciyuan Qiu Huifu Xiao Liheng Wang Yonghui Tian 2022Frontiers of Optoelectronics2022,15,1:2
14Ultrathin,elastic,and self-adhesive nanofiber bio-tape:An intraoperative drug-loading module for ureteral stents with localized and controlled drug delivery properties for customized therapy显示文摘During the postoperative management of urinary diseases,oral or intravenous administration of drugs and implanting ureteral stents are usually required,making localized drug delivery by ureteral stent a precise and effective medication strategy.In the traditional drug loading method,the drug was premixed in the implants in production lines and the versatility of drugs was restricted.However,the complex situation in the urinary system fails the possibility of finding a“one fits all”medication plan,and the intraoperative drug-loading of implants is highly desired to support customized therapy.Here,we designed an ultrathin(8μm),elastic,and self-adhesive nanofiber bio-tape(NFBT)that can easily encapsulate drugs on the stent surface for controllable localized drug delivery.The NFBT exhibited high binding strength to a ureteral stent,a sustained release over 7 d in PBS for hydrophilic drug,and a zero-order release curve over 28 days for the hydrophobic drug nitrofurantoin(NFT).Further in vivo experiments using a porcine ureteral tract infection model demonstrated that NFBT loaded with NFT could significantly reduce the bacterial concentration in urine.The total amount of NFT delivered by the NFBT was about 2.68 wt%of the recommended dose for the systemic administration.Liheng Gao Mingxi Xu Wenshuo Zhao Ting Zou Fujun Wang Jun Da Yiwei Wang Lu Wang 2022Bioactive Materials2022,7,12:2
15Large-scale phase retrieval显示文摘High-throughput computational imaging requires efficient processing algorithms to retrieve multi-dimensional and multi-scale information.In computational phase imaging,phase retrieval(PR)is required to reconstruct both amplitude and phase in complex space from intensity-only measurements.The existing PR algorithms suffer from the tradeoff among low computational complexity,robustness to measurement noise and strong generalization on different modalities.In this work,we report an efficient large-scale phase retrieval technique termed as LPR.It extends the plug-and-play generalized-alternating-projection framework from real space to nonlinear complex space.The alternating projection solver and enhancing neural network are respectively derived to tackle the measurement formation and statistical prior regularization.This framework compensates the shortcomings of each operator,so as to realize high-fidelity phase retrieval with low computational complexity and strong generalization.We applied the technique for a series of computational phase imaging modalities including coherent diffraction imaging,coded diffraction pattern imaging,and Fourier ptychographic microscopy.Extensive simulations and experiments validate that the technique outperforms the existing PR algorithms with as much as 17dB enhancement on signal-to-noise ratio,and more than one order-of-magnitude increased running efficiency.Besides,we for the first time demonstrate ultralarge-scale phase retrieval at the 8K level(7680×4320 pixels)in minute-level time.Xuyang Chang Liheng Bian Jun Zhang 2021eLight2021,1,1:2
16MOF-Like 3D Graphene-Based Catalytic Membrane Fabricated by One-Step Laser Scribing for Robust Water Purification and Green Energy Production显示文摘Increasing both clean water and green energy demands for survival and development are the grand challenges of our age.Here,we successfully fabricate a novel multifunctional 3D graphene-based catalytic membrane(3D-GCM)with active metal nanoparticles(AMNs)loading for simultaneously obtaining the water purification and clean energy generation,via a“green”one-step laser scribing technology.The as-prepared 3D-GCM shows high porosity and uniform distribution with AMNs,which exhibits high permeated fluxes(over 100 L m^(−2) h^(−1))and versatile super-adsorption capacities for the removal of tricky organic pollutants from wastewater under ultra-low pressure-driving(0.1 bar).After adsorption saturating,the AMNs in 3D-GCM actuates the advanced oxidization process to self-clean the fouled membrane via the catalysis,and restores the adsorption capacity well for the next time membrane separation.Most importantly,the 3D-GCM with the welding of laser scribing overcomes the lateral shear force damaging during the long-term separation.Moreover,the 3D-GCM could emit plentiful of hot electrons from AMNs under light irradiation,realizing the membrane catalytic hydrolysis reactions for hydrogen energy generation.This“green”precision manufacturing with laser scribing technology provides a feasible technology to fabricate high-efficient and robust 3D-GCM microreactor in the tricky wastewater purification and sustainable clean energy production as well.Xinyu Huang Liheng Li Shuaifei Zhao Lei Tong Zheng Li Zhuiri Peng Runfeng Lin Li Zhou Chang Peng Kan-Hao Xue Lijuan Chen Gary J.Cheng Zhu Xiong Lei Ye 2022Nano-Micro Letters2022,14,11:2
17Morphology-dependent electrocatalytic performance of Fe_(2)(MoO_(4))_(3) for electro-oxidation of methanol in alkaline medium显示文摘Electrochemically synthesized nanosphere,nanorod and nanotube Fe_(2)(MoO_(4))_(3) at optimized temperature and current density are characterized with XRD,SEM,TEM,XPS.Crystal lattices of the three types Fe_(2)(MoO_(4))_(3) detected by HRTEM are well matched with the simulation analysis results from Materials Studio 6.0 based on the inorganic crystal structure database(ICSD)data and the modified XRD lattice parameters.The ratios of Fe/Mo on the surface resulted from XPS analysis are 1.47,1.63 and 2.22 respectively for nanosphere,nanorod and nanotube.The mixture of Fe_(2)(MoO_(4))_(3) with polytetrafluoroethylene dispersion are coated on glass carbon substrate as electrode for electrocatalytic performance test by cyclic voltammetries in 0.1 mol/L KOH and 1 mol/L methanol electrolyte.Methanol oxidation peak current density of the Nanotube-Fe_(2)(MoO_(4))_(3)/GCEs electrode is 3.27 mA/cm^(2) higher than 2.8 mA/cm^(2) of platinum foil electrode,which shows enhanced catalytic activity of Nanotube-Fe_(2)(MoO_(4))_(3)/GCEs.The cyclic stability in terms of peak current retention are 91%,92%and 88%respectively for Nanosphere-Fe_(2)(MoO_(4))_(3)/GCE,Nanorod-Fe_(2)(MoO_(4))_(3)/GCE and Nanotube-Fe_(2)(MoO_(4))_(3)/GCE electrode after 220 cycles.It is concluded that nanosized Fe_(2)(MoO_(4))_(3) could be promising alternative non-noble electro-catalysts for electro-oxidation of methanol in alkaline medium.Daoming Zhang Liheng Zhang Wei Zhang Mengfei Huo Jiajia Yin Guoju Dang Zhen Ren Quansheng Zhang Jingying Xie Samuel S.Mao 2017Journal of Materiomics2017,3,2:2
18Novel method of gait switching in six-legged robot walking on continuous-nondifferentiable terrain by utilizing stability and interference criteria显示文摘Continuous-nondifferentiable terrains are extremely challenging for the environment adaption of six-legged robots. Previous researches have focused on gait planning methods to improve inherent ability of legged robots to walk over moderate terrains.However,most six-legged robots utilize relatively monotonic gait so that they still cannot well adapt tough terrains. As a result,the current legged robots easily get stuck and fall when encountering continuous-nondifferentiable terrains,such as stairs.Therefore,a method of gait switching is proposed so that six-legged robots can flexibly generate multiple gaits to adapt complex terrains. This study investigated the relationship between six-legged robot gait topologies and physical constraints,such as robot stability and robot-terrain interference. The proposed gait switcher can generate 0-6,1-5,2-4 and 3-3 gaits,which is instructed by the stability and interference criteria. Simulations and experiments were performed on a novel six-legged robot Hexa-XIII that succeeded climbing stairs over 45°. The effectiveness of the gait switching method is validated by the experiment results.MAO LiHeng TIAN Yuan GAO Feng ZHAO Yue 2020Science China(Technological Sciences)2020,63,12:2
19Helically Grooved Gold Nanoarrows: Controlled Fabrication, Superhelix, and Transcribed Chiroptical Switching显示文摘Plasmonic chiroptical materials,coupled by chirality and surface plasmons,have been attracting great interest due to their potential applications,such as photonics,chiral recognition,asymmetric catalysis and biosensing.Herein,we constructed a new chiral plasmonic nanostructure—helically grooved gold nanoarrows(HeliGNAs)by introducing L-/Dcysteine(L-/D-Cys)during the growth of the gold nanoarrows(GNAs).The variation of the concentration of L-/D-Cys leads to the HeliGNAs with a tunable plasmonic circular dichroism(PCD).Song Wang Liheng Zheng Wenjie Chen Lukang Ji Li Zhang Wensheng Lu Zheyu Fang Fucheng Guo Limin Qi Minghua Liu 2021CCS Chemistry2021,3,9:2
20Tailoring Bi_(2)Te_(3) edge with semiconductor and metal properties under electron beam irradiation显示文摘In pursuit of miniaturization in the semiconductor industry,two-dimensional(2D)materials are used to fabricate new electronic devices.The topological insulator(TI)material bismuth telluride(Bi_(2)Te_(3)),as an emerging 2D material,has potential applications in electronic and spintronic devices due to its unique electrical properties.It is well known that the surface-to-volume ratio increases as the thickness of the material decreases,resulting in a more prominent edge effect.Therefore,for a single-layer Bi_(2)Te_(3),the atomic structure of the edge plays a crucial role in its electrical properties.Here,combining first-principles calculations and in situ transmission electron microscopy(TEM)experimental studies,we report that there are two types of edge structures in single-layer Bi2Te3:semiconducting flat edges and metallic zigzag edges.The dynamic evolution process of the edge structure with atomic resolution shows that the proportions of these two edges change with continuous electron beam irradiation.Our findings demonstrate the viability to use electron beam as an effective tool to precisely tailor the edge of Bi_(2)Te_(3) with desired properties,which paves the way for implementation of single-layer Bi2Te3 in electronics and spintronics.Ning Cao Peng Liu Jialiang Pan Liheng Liang Kunpeng Cai Qingguo Shao Hongwei Zhu Xiaobei Zang 2022Nano Research2022,15,5:2
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