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| 1 | 120 mm Single-crystalline perovskite and wafers: towards viable applications显示文摘As the large single-crystalline silicon wafers have revolutionized many industries including electronics and solar cells, it is envisioned that the availability of large single-crystalline perovskite crystals and wafers will revolutionize its broad applications in photovoltaics, optoelectronics, lasers, photodetectors, light emitting diodes(LEDs), etc. Here we report a method to grow large single-crystalline perovskites including single-halide crystals: CH3NH3PbX3(X=I, Br, Cl), and dual-halide ones:CH3NH3Pb(ClxBr1.x)3 and CH3NH3Pb(BrxI1.x)3, with the largest crystal being 120 mm in length. Meanwhile, we have advanced a process to slice the large perovskite crystals into thin wafers. It is found that the wafers exhibit remarkable features:(1)its trap-state density is a million times smaller than that in the microcrystalline perovskite thin films(MPTF);(2) its carrier mobility is 410 times higher than its most popular organic counterpart P3HT;(3) its optical absorption is expanded to as high as910 nm comparing to 797 nm for the MPTF;(4) while MPTF decomposes at 150 °C, the wafer is stable at high temperature up to270 °C;(5) when exposed to high humidity(75% RH), MPTF decomposes in 5 h while the wafer shows no change for overnight;(6) its photocurrent response is 250 times higher than its MPTF counterpart. A few electronic devices have been fabricated using the crystalline wafers. Among them, the Hall test gives low carrier concentration with high mobility. The trap-state density is measured much lower than common semiconductors. Moreover, the large SC-wafer is found particularly useful for mass production of integrated circuits. By adjusting the halide composition, both the optical absorption and the light emission can be fine-tuned across the entire visible spectrum from 400 nm to 800 nm. It is envisioned that a range of visible lasers and LEDs may be developed using the dual-halide perovskites. With fewer trap states, high mobility, broader absorption, and humidity resistance, it is expected that solar cells with high stable efficiency maybe attainable using the crystalline wafers. | Yucheng Liu Xiaodong Ren Jing Zhang Zhou Yang Dong Yang Fengyang Yu Jiankun Sun Changming Zhao Zhun Yao Bo Wang Qingbo Wei Fengwei Xiao Haibo Fan Hao Deng Liangping Deng Shengzhong (Frank) Liu | 2017 | Science China Chemistry2017，60，10： | 5 |
| 2 | Effects of dietary ratio of n-6 to n-3 polyunsaturated fatty acids on immunoglobulins, cytokines, fatty acid composition, and performance of lactating sows and suckling piglets显示文摘This experiment was conducted to investigate the effects of dietary ratios of n-6:n-3 polyunsaturated fatty acids (PUFA) on the performance of lactating sows and their piglets. Thirty pregnant Landrace sows were assigned to one of three treatments from d 108 of gestation until weaning (26-29 d) and were fed diets containing different ratios of n-6:n-3 PUFA including 3:1, 9:1 and 13:1. The effects on sow and litter production traits were examined together with an assessment of sow body condition. No differences were detected among the treatments for the daily feed intake of sows or changes in sow weight and back-fat levels during lactation (P > 0.05). Litter size at d 14 and d 21 were tended to increase in 3:1 treatment compared with 9:1 and 13:1 treatments (P < 0.10). Litter weight gain (1.77 kg/d) from d 0 to d 14 was tended to increase in 9:1 groups compared with the other two treatments (P < 0.10). A significant difference was observed for the content of α -linolenic acid, total n-3 PUFA, and the ratio of n-6:n-3 PUFA in the colostrum, milk, and piglets plasma (P < 0.01). The effects of different ratios of n-6:n-3 PUFA in sow diets on colostrum, milk, and piglet plasma immunoglobulin concentrations are studied. No difference was observed among treatments in the concentrations of IgM, and IgA in colostrum (P > 0.05). A great significant difference for IgG concentration was observed among 3 group in colostrum. A great significant difference for IgA, and IgM (P < 0.01) concentrations in piglet plasma at d14 and a significant difference for IgG(P < 0.05) was observed at d14. Furthermore, at d 21 of lactation, piglet plasma IgG and IgA concentration were greater in 3:1 compared with 13:1 group (P < 0.01). In summary, the current study demonstrated that altering the ratio of n-6:n-3 PUFA in lactating sow diet had an effect on the immune component including immunoglobulin and cytokines, and it tended to increase the litter average daily gain and improve the immune status of piglets when dietary ratio of n-6:n-3 PUFA was 9:1. | Wei Yao Jie Li Jun jun Wang Weiliang Zhou Qingbo Wang Rongchang Zhu Fenglai Wang Phil Thacker | 2013 | Journal of Animal Science and Biotechnology2013，4，2： | 4 |
| 3 | Improved perovskite solar cell efficiency by tuning the colloidal size and free ion concentration in precursor solution using formic acid additive显示文摘Improving the quality of the perovskite active layer is crucial to obtaining high performance perovskite solar cells(PSCs). In this work, by introducing formic acid into the formamidinium lead iodide(FAPbI3)precursor solution, we managed to achieve reduced colloidal size in the solution, leading to more uniform deposition of FAPbI3 film with lower trap state density and higher carrier mobility. The solar cells based on the FAPbI3 absorber layer modified with formic acid show significantly better photovoltaic performance than that on the reference FAPbI3 film without formic acid. The device performance shows a close correlation with the colloidal size. Within the range studied from 6.7 to 1.0 nm, the smaller the colloidal size is, the higher the solar cell efficiency. More specifically, the cell efficiency is improved from17.82% for the control cell without formic acid to 19.81% when 0.764 M formic acid was used. Formic acid has also been added into a CH3NH3PbI3(MAPbI3) precursor solution, which exhibits a similar effect on the resulting MAPb I3 films and solar cells, with efficiency improved from 16.07% to 17.00%. | Lina Meng Qingbo Wei Zhou Yang Dong Yang Jiangshan Feng Xiaodong Ren Yucheng Liu Shengzhong(Frank)Liu | 2020 | Journal of Energy Chemistry2020，29，2： | 2 |
| 4 | ADAMTS-7 Mediates Vascular Smooth Muscle Cell Migration and Neointima Formation in Balloon-Injured Rat Arteries显示文摘 | Li Wang Jingang Zheng Xue Bai Bo Liu Chuan-ju Liu Qingbo Xu Yi Zhu Nanping Wang Wei Kong Xian Wang | 2009 | Circulation Research2009，，5： | 2 |
| 5 | Single-cell RNA sequencing reveals B cell-T cell interactions in vascular adventitia of hyperhomocysteinemia-accelerated atherosclerosis显示文摘Dear Editor Cardiovascular disease(CVD)is the leading cause of death around the world(Truelsen,et al.,2015).Atherosclerosis,the dominant underlying cause of CVD,is a chronic inflam-matory disease characterized by lipid accumulation and immune cell infiltration in plaques and vessels(Weber,et al.,1950).The immune microenvironment is critical for the development of atherosclerosis.Homocysteine(Hcy)is an intermediate product of methionine metabolism,and its ele-vation in plasma(>15μmol/L),known as hyperhomocys-teinemia(HHcy),is an independent risk factor for atherosclerosis.HHcy is more common in Asia because of genetic factors and dietary habits(Huo,et al.,2015).folic acid supplement is one of the most important way to treat HHcy in clinic.Although HHcy potentiates atherosclerosis mainly through endothelial injury and inflammatory activa-tion(Luo,et al.,2016),a comprehensive understanding of the immune microenvironment and potential mechanisms in HHcy-accelerated atherosclerotic aortas(HHcy-AA)is still lacking. | Xiaolong Ma Jiacheng Deng Lulu Han Yuwei Song Yutong Miao Xing Du Guohui Dang Dongmin Yang Bitao Zhong Changtao Jiang Wei Kong Qingbo Xu Juan Feng Xian Wang | 2022 | Protein & Cell2022，13，7： | 2 |
| 6 | Effective shape-controlled synthesis of gallium selenide nanosheets by vapor phase deposition显示文摘The controlled synthesis of large and uniform gallium selenide(GaSe)crystals is crucial for its various applications based on the attractive properties of this emerging material.In this work,vapor phase growth of high-quality monolayer GaSe nanosheets with multiple shape and size is achieved by tuning the Ga/GaSe ratio in the precursor.A theoretical model based on density functional theory calculations and kinetic Wulff construction theory describe the observed shape evolution of the GaSe nanosheets.Results show that the Ga/Se ratio plays a critical role in the evolution of the domain shape and size.Moreover,the as-grown GaSe nanosheets show improved performance with photoresponse time less than 0.7 ms and responsibility up to 3,000 AW.This study presents a previously unexplored strategy for the controlled growth of two-dimensional(2D)GaSe nanosheets for promising applications in next-generation optoelectronics. | Lilan Tan Qingbo Liu Yufeng Ding Xiaogang Lin Wei Hu Meng-Qiu Cai Hong Zhou | 2020 | Nano Research2020，13，2： | 2 |
| 7 | Cartilage oligomeric matrix protein is an endogenous β-arrestin-2-selective allosteric modulator of AT1 receptor counteracting vascular injury显示文摘Compelling evidence has revealed that biased activation of G protein-coupled receptor(GPCR)signaling,including angiotensin II(AngII)receptor type 1(AT1)signaling,plays pivotal roles in vascular homeostasis and injury,but whether a clinically relevant endogenous biased antagonism of AT1 signaling exists under physiological and pathophysiological conditions has not been clearly elucidated.Here,we show that an extracellular matrix protein,cartilage oligomeric matrix protein(COMP),acts as an endogenous allosteric biased modulator of the AT1 receptor and its deficiency is clinically associated with abdominal aortic aneurysm(AAA)development.COMP directly interacts with the extracellular N-terminus of the AT1 via its EGF domain and inhibits AT1-β-arrestin-2 signaling,but not Gq or Gi signaling,in a selective manner through allosteric regulation of AT1 intracellular conformational states.COMP deficiency results in activation of AT1a-β-arrestin-2 signaling and subsequent exclusive AAA formation in response to AngII infusion.AAAs in COMP–/–or ApoE–/–mice are rescued by AT1a orβ-arrestin-2 deficiency,or the application of a peptidomimetic mimicking the AT1-binding motif of COMP.Explorations of the endogenous biased antagonism of AT1 receptor or other GPCRs may reveal novel therapeutic strategies for cardiovascular diseases. | Yi Fu Yaqian Huang Zhao Yang Yufei Chen Jingang Zheng Chenfeng Mao Zhiqing Li Zhixin Liu Bing Yu Tuoyi Li Meili Wang Chanjuan Xu Yiwei Zhou Guizhen Zhao Yiting Jia Wei Guo Xin Jia Tao Zhang Li Li Ziyi Liu Shengchao Guo Mingliang Ma Heng Zhang Bo Liu Junbao Du Wengong Wang Chaoshu Tang Pei Gao Qingbo Xu Xian Wang Jianfeng Liu Jinpeng Sun Wei Kong | 2021 | Cell Research2021，31，7： | 2 |
| 8 | Synthesis, characterization, and swelling kinetics of pH-responsive and temperature-responsive carboxymethyl chitosan/ polyacrylamide hydrogels 显示文摘 | Wei Qingbo Luo Yanling Fu Feng | 2012 | Journal of Applied Polymer Science2012，129，2： | 1 |
| 9 | Study on activated carbon derived from sewage sludge for adsorption of gaseous formaldehyde显示文摘 | Qingbo Wen Caiting Li Zhihong Cai Wei Zhang Hongliang Gao Lijun Chen Guangming Zeng Xin Shu Yapei Zhao | 2010 | Bioresource Technology2010，，2： | 1 |
| 10 | Rare-earth La2 03 modification of laser-clad coatings 显示文摘 | Wang Kunlin Zhang Qingbo Wei Xingguo | 1998 | Journal of Materi- als Science1998，33，14： | 1 |
| 11 | Rare-earth La2O3 modification of laser - clad coatings 显示文摘 | Wang Kunlin Zhang Qingbo Wei Xingguo | 1998 | Journal of Materials Science1998，33，14： | 1 |
| 12 | Genome-wide analysis of GH3 gene family in soybean( Glycine max)显示文摘 | Wei ZHAO Xinjie SHEN Wei GUO Qingbo YOU Yanjie YAO Jianhua LU Juncheng ZHANG Lei HUANG Bingbing DUAN Huarong LV Aili BAO Yongqing JIAO | 2016 | Oil Crop Science2016，1，2： | 1 |
| 13 | Study on activated carbon derived from sewage sludge for adsorption of gaseous formaldehyde显示文摘 | Qingbo Wen Caiting Li Zhihong Cai Wei Zhang Hongliang Gao Lijun Chen Guangming Zeng Xin Shu Yapei Zhao | 2010 | Bioresource Technology2010，，2： | 1 |
| 14 | Study on activated carbon derived from sewage sludge for adsorption of gaseous formaldehyde 显示文摘 | Qingbo Wen Caiting Li Zhihong Cai Wei Zhang Hongliang Gao Lijun Chen Guangming Zeng Xin Shu Yapei Zhao | 2011 | Bioresource Technology2011，102，2： | 1 |
| 15 | Highly stable and efficient perovskite solar cells produced via high-boiling point solvents and additive engineering synergistically显示文摘The active absorber layer plays a crucial role in a perovskite solar cell.Herein,we used high boiling pointγ-butyrolactone(GBL)as the main solvent,Pb(SCN)2 and dimethyl sulfoxide(DMSO)as an effective additive in the FA0.83MA0.17Cs0.05PbI(3-x)Brx solution to improve the quality of perovskite films.The GBL will delay the crystallization speed of the perovskite,and lead to the grain growth assisted by thiocyanate.The synergistic effect of the solvent engineering and additive engineering is beneficial to the slow growth of the grain size.It is found that the addition of Pb(SCN)2 increases Gibbs free energy barrier for the nucleation,leading to the formation of fewer nuclei,which results in a high quality of perovskite absorbers with larger grains and smoother surfaces.The synergistic effect of solvents and Pb(SCN)2 on the morphology and photovoltaic performances is investigated.Compared to devices without the additive,the efficiency of devices with 5%Pb(SCN)2-doped FA0.83MA0.17Cs0.05PbI(3-x)Brx is raised to 19.01%from 15.21%.We believe this breakthrough regarding high efficiency perovskite solar cells will help for their transitions. | Qingbo Wei Zhangwen Ye Xiaodong Ren Feng Fu Zhou Yang Shengzhong(Frank)Liu Dong Yang | 2020 | Science China Chemistry2020，63，6： | 1 |
| 16 | Hard and tough novel high-pressure γ-Si_(3)N_(4)/Hf_(3)N_(4) ceramic nanocomposites显示文摘Cubic silicon nitride(-Si_(3)N_(4))is superhard and one of the hardest materials after diamond and cubic boron nitride(cBN),but has higher thermal stability in an oxidizing environment than diamond,making it a competitive candidate for technological applications in harsh conditions(e.g.,drill head and abrasives).Here,we report the high-pressure synthesis and characterization of the structural and mechanical properties of a γ-Si_(3)N_(4)/Hf_(3)N_(4) ceramic nanocomposite derived from single-phase amorphous silicon(Si)-hafnium(Hf)-nitrogen(N)precursor.The synthesis of the-Si_(3)N_(4)/Hf_(3)N_(4) nanocomposite is performed at~20 GPa and ca.1500 ℃ in a large volume multi anvil press.The structural evolution of the amorphous precursor and its crystallization to-Si_(3)N_(4)/Hf_(3)N_(4) nanocomposites under high pressures is assessed by the in situ synchrotron energy-dispersive X-ray diffraction(ED-XRD)measurements at~19.5 GPa in the temperature range of ca.1000-1900℃.The fracture toughness(K_(IC))of the two-phase nanocomposite amounts~6/6.9 MPa·m^(1/2) and is about 2 times that of single-phaseγ-Si_(3)N_(4),while its hardness of ca.30 GPa remains high.This work provides a reliable and feasible route for the synthesis of advanced hard and tough-Si_(3)N_(4)-based nanocomposites with excellent thermal stabililty. | Wei Li Zhaoju Yu Leonore Wiehl Tianshu Jiang Ying Zhan Emmanuel III Ricohermoso Martin Etter Emanuel Ionescu Qingbo Wen Christian Lathe Robert Farla Dharma Teppala Teja Sebastian Bruns Marc Widenmeyer Anke Weidenkaff Leopoldo Molina-Luna Ralf Riedel Shrikant Bhat | 2023 | Journal of Advanced Ceramics2023，12，7： | 0 |
| 17 | Talachalasins A-C,Undescribed Cytochalasans with a 16β-Methyl or 2-Oxabicyclo[3.3.1]nonan-3-one unit from the Deep-Sea-Derived Fungus Talaromyces muroii sp.SCSIO 40439显示文摘Comprehensive Summary Talachalasins A-C(1-3),three new cytochalasans(CYTs),were isolated from deep-sea-derived fungus Talaromyces muroii sp.SCSIO 40439.The structures of 1-3,including absolute configurations,were determined based on HRESIMS,NMR spectroscopic data,ECD comparison,and single crystal X-ray diffraction analysis.Talachalasins A-C(1-3)represented the first examples of cytochalasans possessing a unique 16β-methyl group,distinct from>500 reported CYTs.Talachalasin C(3)was an unprecedented 20,21-seco-cytochalasans characterized by a 2-oxabicyclo[3.3.1]nonan-3-one unit.Talachalasin A(1)displayed moderate cytotoxic activity against four tumor cell lines(IC_(50)3.40-10.02μM).Talachalasin B(2)showed comparable anti-RSV and HSV-1 activities(IC5012.5μM or IC5020.0μM). | Xuemin Ding Weixia Ye Bin Tan Qiaoyun Song Yuchan Chen Wei Liu Lili Sun Wei Tang Yulei Qiao Qingbo Zhang Haibo Zhang Ying Wang Weimin Zhang Changsheng Zhang Wenjun Zhang | 2023 | Chinese Journal of Chemistry2023，41，8： | 0 |
| 18 | Antioxidant induced bulk passivation for efficient and stable hole transport layer-free carbon electrode perovskite solar cells显示文摘Defect passivation is one of the important strategies to improve the efficiency and stability of perovskite solar cells.In this work,2,6-di-tert-butyl-4-methylphenol(BHT)as antioxidant was introduced into the perovskite precursor solution to improve the quality of the prepared perovskite films,so that these films performed a larger and uniform grain size.Moreover,the-OH functional group in BHT interacts with I-,thus reducing the density of defect states and inhibiting the non-radiative recombination.The presence of hydrophobic groups in BHT protects the film from moisture erosion and improves the long-term stability of PSCs devices.The maximum photoelectric conversion efficiency of the constructed ITO/SnO_(2)/BHTMAPbI_(3)/Carbon device is 16.88%,and the unpackaged cell maintains the initial efficiency of 99.3%after698 h of storage under the environmental condition of 30%humidity.This work provides an efficient approach to improve the performance of printable hole transport layer-free carbon electrode perovskite solar cells. | Yetai Cheng Qingbo Wei Nannan Wang Zhangwen Ye Yanbin Zhao Qiongyao Wang Depeng Chu Lingxing Zan Feng Fu Yucheng Liu | 2023 | Chinese Chemical Letters2023，34，6： | 0 |
| 19 | Effects of Loading-Dose Statins Combined with PCSK9 Inhibitor Pre-Treatment before Primary Percutaneous Coronary Intervention on the Short-Term Prognosis in Patients with ST-Segment Elevation Myocardial Infarction显示文摘Objective:This study was aimed at investigating the effects of preoperative treatment with a loading dose of statins combined with a PCSK9 inhibitor on coronary blood perfusion and short-term cardiovascular adverse events in patients with ST-segment elevation myocardial infarction(STEMI).Method:Sixty-five patients with STEMI who had visited the Shanxi Cardiovascular Disease Hospital between May 2018 and May 2021 were enrolled in the study.The enrolled patients had no history of oral statins or antiplatelet therapy.The patients were divided into a combined treatment group(loading dose of statins combined with PCSK9 inhibitors,35 patients)and a routine treatment group(loading dose of statins only,30 patients).The primary endpoints were thrombolysis in myocardial infarction(TIMI)blood flow grading,corrected TIMI frame count(CTFC),and TIMI myocardial perfusion grading(TMPG),immediately after and 30 days after the operation.The secondary endpoint was a composite endpoint of cardiovascular death,nonfatal myocardial infarction,and target vessel revascularization 30 days after the operation.Results:The combined treatment group had significantly lower CTFC(14.09±8.42 vs 26±12.42,P=0.04)and better TMPG(2.74±0.61 vs 2.5±0.73,P=0.04)than the routine treatment group immediately after the operation.Similarly,the combined treatment group had a significantly lower CTFC(16.29±7.39 vs 26.23±11.53,P=0.04)and significantly better TMPG(2.94±0.24 vs 2.76±0.43,P=0.01)than the routine treatment group 1 month after the operation.Conclusion:Preoperative treatment with a loading dose of high-intensity statins combined with PCSK9 inhibitors increased coronary blood flow and myocardial perfusion after emergency thrombus aspiration in patients with STEMI.However,the treatment did not significantly decrease the incidence of cardiovascular death,nonfatal myocardial infarction,or target vessel revascularization. | Zhe Wang Qingbo Bao Xiaojian Song Hengjie Song Shoudong Wei Junwei Lv Fei Wang Jian An | 2022 | Cardiovascular Innovations and Applications2022，7，3： | 0 |
| 20 | Building damage mapping based on Touzi decomposition using quad-polarimetric ALOS PALSAR data显示文摘Building damage assessment is of great significance to disaster monitoring.Polarimetric Synthetic Aperture Radar(SAR)can record the polarization scattering measurement matrix of ground objects and obtain more abundant ground object information,meaning that they can be used for assessing damage to buildings.In this paper,a new approach is proposed to assess building damage using the Touzi incoherent decomposition and SAR-based characteristics of buildings before and after damage.The March 11th,2011 earthquake that struck the coast of northeast Japan serves as the demonstration of the technique using quad-polarimetric ALOS PALSAR data acquired before and after the disaster.The analysis shows that after the buildings are damaged,there is a clear decrease in theαs1(the dominant scattering-type magnitude)components and the degree of this reduction corresponds to the degree of building damage.This means that theαs1 components obtained by Touzi decomposition can effectively reflect the degree of building damage.On this basis,a model based on Touzi decomposition was established to evaluate the degree of damage to buildings,and the accuracy of the model was validated using high-resolution optical data acquired before and after the earthquake.The experimental results show that Touzi decomposition can be effectively used for damage assessment mapping in built-up areas. | Shan LIU Fengli ZHANG Shiying WEI Qingbo LIU Na LIU Yun SHAO Steven JBURIAN | 2020 | Frontiers of Earth Science2020，14，2： | 0 |
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