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| 1 | Adsorption of VOCs on reduced graphene oxide显示文摘A modified Hummer's method was adopted for the synthesis of graphene oxide(GO) and reduced graphene oxide(rGO). It was revealed that the modified method is effective for the production of GO and rGO from graphite. Transmission electron microscopy(TEM) images of GO and rGO showed a sheet-like morphology. Because of the presence of oxygenated functional groups on the carbon surface, the interlayer spacing of the prepared GO was higher than that of rGO. The presence of \OH and C_O groups in the Fourier transform infrared spectra(FTIR) spectrum and G-mode and 2D-mode in Raman spectra confirmed the synthesis of GO and rGO. rGO(292.6 m^2/g) showed higher surface area than that of GO(236.4 m^2/g). The prepared rGO was used as an adsorbent for benzene and toluene(model pollutants of volatile organic compounds(VOCs)) under dynamic adsorption/desorption conditions. rGO showed higher adsorption capacity and breakthrough times than GO. The adsorption capacity of rGO for benzene and toluene was 276.4 and 304.4 mg/g, respectively.Desorption experiments showed that the spent rGO can be successfully regenerated by heating at 150.0°C. Its excellent adsorption/desorption performance for benzene and toluene makes rGO a potential adsorbent for VOC adsorption. | Lian Yu Long Wang Weicheng Xu Limin Chen Mingli Fu Junliang Wu Daiqi Ye | 2018 | Journal of Environmental Sciences2018，30，5： | 10 |
| 2 | Highly efficient Cu/anatase TiO2 {001}-nanosheets catalysts for methanol synthesis from CO2显示文摘Anatase TiO_2 nanosheets(-ns-) with dominant exposed {001} facets were used as support to load copper,and the synthesized Cu/TiO_2-ns catalysts were evaluated for CO_2 hydrogenation to methanol. Under the reaction conditions, P = 3.0 MPa, T = 260 ℃, V(N_2):V(H_2):V(CO_2) = 8:69:23 and gas hourly space velocity(GHSV) = 3600 mL g^(-1)h^(-1), the methanol yield reached an appealing high value, 5.6%. Copper-loading amount, calcination temperature and reduction atmosphere have been investigated in this work, which significantly influence the particle sizes of copper and/or the defect concentration in TiO_2, then leading to different catalytic performance. Characterizations of XRD, EPR, CO_2-TPD and FTIR demonstrate that higher specific surface area of Cu is good for the hydrogenation of CO_2 and adequate amount of Ti^(3+) plays important roles in CO_2 activation. Both of them facilitate high turnover frequency(TOF) of methanol formation. | Yunfeng Bao Chunlei Huang Limin Chen Yu dong Zhang Long Liang Jinjun Wen Mingli Fu Junliang Wu Daiqi Ye | 2018 | Journal of Energy Chemistry2018，27，2： | 7 |
| 3 | Macroporous Ni foam-supported Co_3O_4 nanobrush and nanomace hybrid arrays for high-efficiency CO oxidation显示文摘Herein, we reported the synthesis of well-defined Co_3O_4 nanoarrays(NAs) supported on a monolithic three-dimensional macroporous nickel(Ni) foam substrate for use in highefficiency CO oxidation. The monolithic Co_3O_4 NAs catalysts were obtained through a generic hydrothermal synthesis route with subsequent calcination. By controlling the reaction time,solvent polarity and deposition agent, these Co_3O_4 NAs catalysts exhibited various novel morphologies(single or hybrid arrays), whose physicochemical properties were further characterized by using several analytical techniques. Based on the catalytic and characterization analyses, it was found that the Co_3O_4 NAs-6 catalyst with nanobrush and nanomace arrays displayed enhanced catalytic activity for CO oxidation, achieving an efficient 100% CO oxidation conversion at a gas hourly space velocity(GHSV) 10,000 hr^(-1) and 150°C with longterm stability. Compared with the other Co_3O_4 NAs catalysts, it had the highest abundance of surface-adsorbed oxygen species, excellent low-temperature reducibility and was rich in surface-active sites(Co^(3+)/Co^(2+)= 1.26). | Shengpeng Mo Hui He Quanming Ren Shuangde Li Weixia Zhang Mingli Fu Limin Chen Junliang Wu Yunfa Chen Daiqi Ye | 2019 | Journal of Environmental Sciences2019，31，1： | 4 |
| 4 | Carbazole-endcapped Spiro[fluorene-9,9'-xanthene] with Large Steric Hindrance as Hole-transporting Host for Heavily-doped and High Performance OLEDs显示文摘 | Xianghua Zhao Yukun Wu Nannan Shi Xiaoyu Li Yi Zhao Mingli Sun Dongxue Ding Hui Xu Linghai Xie | 2015 | Chinese Journal of Chemistry2015，33，8： | 3 |
| 5 | Rett syndrome-causing mutations compromise MeCP2- mediated liquid—liquid phase separation of chromatin显示文摘Rett syndrome(RTT),a severe postnatal neurodevelopmental disorder,is caused by mutations in the X-linked gene encoding methyl-CpG-binding protein 2(MeCP2).MeCP2 is a chromatin organizer regulating gene expression.RTT-causing mutations have been shown to affect this function.However,the mechanism by which MeCP2 organizes chromatin is unclear.In this study,we found that MeCP2 can induce compaction and liquid-liquid phase separation of nudeosomal arrays in vitro,and DNA methylation further enhances formation of chromatin condensates by MeCP2.Interestingly,RTT-causing mutations compromise MeCP2-mediated chromatin phase separation,while benign variants have little effect on this process.Moreover,MeCP2 competes with linker histone H1 to form mutually exclusive chromatin condensates in vitro and distinct heterochromatin foci in vivo.RTT-causing mutations reduce or even abolish the ability of MeCP2 to compete with histone H1 and to form chromatin condensates.Together,our results identify a novel mechanism by which phase separation underlies MeCP2-mediated heterochromatin formation and reveal the potential link between this process and the pathology of RTT. | Liang Wang Mingli Hu Mei-Qing Zuo Jicheng Zhao Di Wu Li Huang Yongxin Wen Yunfan Li Ping Chen Xinhua Bao Meng-Qiu Dong Guohong Li Pilong Li | 2020 | Cell Research2020，30，5： | 3 |
| 6 | Unraveling specific role of carbon matrix over Pd/quasi-Ce-MOF facilitating toluene enhanced degradation显示文摘Metal organic frameworks(MOFs)derivatives represented by quasi-MOFs have excellent physical and chemical properties and can be applied for the catalytic combustion of volatile organic compounds(VOCs).In this work,Pd/quasi-Ce-BTC synthesized by simple one-step Npyrolysis was applied to the oxidation of toluene,showing excellent toluene catalytic activity(T_(90)=175℃,30000 mL/(g·h)).Microscopic analyses indicate the formation and interaction of a carbon matrix composite quasi-MOF structure interface.The results show that the amorphous carbon matrix formed during the partial pyrolysis of Ce-BTC significantly improves the adsorption and activation capacity of toluene in the reaction,and constructs a reductive system to maintain high concentrations of Ce^(3+)and Pd^(0),which can facilitate the activation and utilization of oxygen in reaction.Quasi in-situ XPS proves that carbon matrix is indirectly involved in the activation and storage of oxygen,and Pd^(0)is the crucial active site for the activation of oxygen.Stability and water resistance tests display good stability of Pd/quasi-Ce-BTC.This work provides a potential method for designing quasi-MOF catalysts towards VOCs effective abatement. | Chunjing Su Zhi Li Mengqi Mao Wenhua Ye Jinping Zhong Quanming Ren Hairong Cheng Haomin Huang Mingli Fu Junliang Wu Yun Hu Daiqi Ye Haihong Xu | 2022 | Journal of Rare Earths2022，40，11： | 2 |
| 7 | Nikethamide affects inspiratory neuron discharge in the nucleus retrofacialis medial region in brain slices from neonatal rats显示文摘BACKGROUND:Nikethamide,a respiratory center stimulant,is widely used in China.However,its effects on the central nervous system and medullary respiratory center remain poorly understood.OBJECTIVE:To investigate the influence of nikethamide on inspiratory neuron discharge in the medial region of the nucleus retrofacialis in neonatal rats,based on the observations addressing rhythmic respiratory discharge generated by the basic medullary respiratory center and various respiration neuron discharges in brain slices.DESIGN,TIME AND SETTING:A controlled,observational study utilizing in vitro neuroelectrophysiology was performed at the Department of Physiology in Southern Medical University between September and December in 2007.MATERIALS:Nikethamide was purchased from Sigma,USA;BL-420E biological signal collection and management system was provided by Chengdu TME Technology,China.METHODS:Isolated medulla-spinal cord preparations were collected from neonatal Sprague Dawley rats,aged 1-3 days.Tissues were divided to include the medial region of the nucleus retrofacialis,ventral respiratory,and dorsal respiratory groups.Subsequently,modified Kreb's solution and 5 μg/mL nikethamide-containing modified Kreb's solution were consecutively perfused into the medial region of the nucleus retrofacialis in neonatal rat brain slices.MAIN OUTCOME MEASURES:Hypoglossal nerve root respiratory-related rhythmic discharge activities and inspiratory neuron discharges were recorded with an adsorption electrode and microelectrode.RESULTS:Nikethamide resulted in prolonged inspiratory neuron discharge time,shortened respiratory cycle and expiratory time.Nikethamide intervention resulted in enhanced integral amplitude of some inspiratory neurons with no changes in discharge frequency or increased discharge frequency in remaining inspiratory neurons with no changes in integral amplitude.CONCLUSION:Nikethamide excites inspiratory neurons in the basic rhythmic respiration and medullary respiratory center,in addition to increased inspiratory neuron and neural network excitability. | Zhibin Qian Mingli Ji Zhonghai Wu | 2010 | Neural Regeneration Research2010，5，4： | 2 |
| 8 | Internal Loads and Bioavailability of Phosphorus and Nitrogen in Dianchi Lake,China显示文摘Sediments have a significant influence on the cycling of nutrient elements in lake environments. In order to assess the distribution characteristics and estimate the bioavailability of phosphorus and nitrogen in Dianchi Lake, organic and inorganic phosphorus and nitrogen forms were analysed. The 210 Pb radiometric dating method was employed to study temporal changes in the phosphorus and nitrogen pools in Dianchi Lake. The result show that the total phosphorus(TP) and total nitrogen(TN) were both at high concentrations, ranging from 697.5–3210.0 mg/kg and 1263.7–7155.2 mg/kg, respectively. Inorganic phosphorus(IP) and total organic nitrogen(TON) were the main constituents, at percentages of 59%–78% and 74%–95%, respectively, in the sediments. Spatially, there was a decreasing trend in phosphorus and nitrogen contents from the south and north to the lake centre, which is related to the distribution pattern of local economic production. The burial rates of the various phosphorus and nitrogen forms increased in same spatially and over time. Particularly in the past two decades, the burial rates doubled, with that TN reached to 1.287 mg/(cm^2·yr) in 2014. As the most reactive forms, nitrate nitrogen(NO_3-N) and ammonia nitrogen(NH_4-N) were buried more rapidly in the south region, implying that the potential for releasing sedimentary nitrogen increased from north to south. Based on their concentrations and burial rates, the internal loads of phosphorus and nitrogen were analysed for the last century. A TP pool of 71597.6 t and a TN pool of 81191.7 t were estimated for Dianchi Lake. Bioavailable phosphorus and nitrogen pools were also estimated at 44468.0 t and 5429.7 t, respectively, for the last century. | WU Yalin HUANG Tao HUANG Changchun SHEN Yinyin LUO Yang YANG Hao YU Yanhong LI Ruixiao GAO Yan ZHANG Mingli | 2018 | Chinese Geographical Science2018，28，5： | 2 |
| 9 | A novel non-precious metal catalyst synthesized via pyrolysis of polyaniline-coated tungsten carbide particles for oxygen reduction reaction显示文摘 | Kezhu Jiang Qingmin Jia Mingli Xu Daping Wu Lunquan Yang Guotao Yang Linyan Chen Guanghua Wang Xikun Yang | 2012 | Journal of Power Sources2012，，： | 1 |
| 10 | Load modeling and identification based on ant colony al- gorithms for EV charging stations显示文摘 | Shaobing Yang Mingli Wu Xiu Yao | 2015 | IEEE trans- actions on Power System2015，30，4： | 1 |
| 11 | Analysis of low- frequency oscillation in electric railways based on small- signal modeling of vehicle-grid system in dq frame 显示文摘 | Wang Hui Wu Mingli Sun Juanjuan | 2015 | IEEE Transactions on Power Electronics2015，30，9： | 1 |
| 12 | The predictive value of TNF-c and IL-6 and the incidence of macrovascular complications in patients with type 2 diabetes显示文摘 | Weihua Wu Mingli Wang Zhenjie Sun | 2012 | Acta Diabetol2012，49，1： | 1 |
| 13 | The anomeric mixture of some O-glycolipid derivatives is more toxic against cancer cells than either anomer alone显示文摘 | Song Shaoxing Wu Mingli He Xiaopeng | 2012 | Bioorg Med Chem Lett2012，22，5： | 1 |
| 14 | A novel non-precious metal catalyst synthesized via pyrolysis of polyaniline-coated tungsten carbide particles for oxygen reduction reaction显示文摘 | Kezhu Jiang Qingmin Jia Mingli Xu Daping Wu Lunquan Yang Guotao Yang Linyan Chen Guanghua Wang Xikun Yang | 2012 | Journal of Power Sources2012，，： | 1 |
| 15 | High speed EMU modeling based on the measured data显示文摘 | YANG Shaobing HUANG Mei WU Mingli | 2009 | Sustainable Power Ge- neration and Supply2009，12，4： | 1 |
| 16 | Controlling Ebola: what we can learn from China’s 1911 battle against the pneumonic plague in Manchuria显示文摘 | He Liu Mingli Jiao Siqi Zhao Kai Xing Ye Li Ning Ning Libo Liang Qunhong Wu Yanhua Hao | 2015 | International Journal of Infectious Diseases2015，，： | 1 |
| 17 | A Simple Way of Calculating the Change in the Gibbs' Free Energy of Ion Adsorption Reactions显示文摘 | Wu Xiaofu Zhao Fang Chen Mingli | 2009 | Adsorption Science & Technology2009，27，1： | 1 |
| 18 | Factors Affecting the Adsorption of Zn2 and Cd2+ Ions from Aqueous Solution onto Vermiculite显示文摘 | Wu Xiaofu Zhao Fang Chen Mingli | 2008 | Adsorpiton Science & Technology2008，26，3： | 1 |
| 19 | Decontamination efficiency and root structure change in the plant-intercropping model in vertical-flow constructed wetlands显示文摘副热带的气候的条件能在冬季贡献构造沼泽地工厂的天线部分的死亡。这介绍一个障碍给构造沼泽地的普遍申请并且是着急地需要被解决的一个问题。三形成对照实验,杂种植物的模型(A) ,温暖季节的工厂模型(B) ,和非植物为(C) 建模,在在垂直流动的构造沼泽地以内在杂种植物的模型在工厂的根结构移开污染物质,和变化以他们的效率被学习。结果显示模型 A 能解决上述的问题。总的来说,平均三种污染物质的移动率(货到付款 < 潜水艇 class= “ a-plus-plus ” > Cr , 总数氮(TN ) 和总数磷(TP )) 用模型, A 比用模型 B 和 C 获得的那些显著地高(P < 0.01 ) 。而且,处于三种污染物质的移动率的重要差别都没在一年的更高的温度部分期间在 A 和 B 之间被检测(P > 0.05 ) 。相反地,三种污染物质的移动率被发现比在一年的更低的温度部分期间用模型 B 观察的那些用模型 A 显著地更高(P < 0.01 ) 。而且,形态学和工厂根的内部结构进一步表明那众多的白根,其在土壤的分发通常是浅的,在模型 A 下面进一步延长。这些水的工厂的根有 aerenchyma 结构因此,实质房间创作了有主要生长优点的寒冷季节的工厂的根在 A 使用了能够创造更有利的垂直流动的构造沼泽地 mediamicroenvironment。在结论,杂种植物的模型(A) 对在构造沼泽地在冬季期间经验丰富的冷环境的使用更合适。 | Yonghua CHEN Xiaofu WU Mingli CHEN Kelin LI Jing PENG Peng ZHAN | 2013 | Frontiers of Environmental Science & Engineering2013，7，6： | 1 |
| 20 | Plasma-Catalytic Oxidation of Toluene on Mn x O y at Atmospheric Pressure and Room Temperature显示文摘 | Meijuan Lu Rong Huang Peitao Wang Limin Chen Junliang Wu Mingli Fu William Wen Bichun Huang Daiqi Ye | 2014 | Plasma Chemistry and Plasma Processing2014，，5： | 1 |
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