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| 1 | Underground ground control monitoring and interpretation,and numerical modeling, and shield capacity design显示文摘Mine or longwall panel layout is a 3D structure with highly non-uniform stress distribution. Recognition of such fact will facilitate underground problem identification/investigation and solving by numerical modeling through proper model construction. Due to its versatility, numerical modeling is the most popular method for ground control design and problem solving. However numerical modeling results require highly experienced professionals to interpret its validity/applicability to actual mining operations due to complicated mining and geological conditions. Underground ground control monitoring is routinely performed to predict roof behavior such as weighting and weighting interval without matching observation of face mining condition while the mining pressures are being monitored, resulting in unrealistic interpretation of the obtained data on mining pressure. The importance of ground control pressure monitoring and simultaneous observation of mining and geological conditions is illustrated by an example of shield leg pressure monitoring and interpretation in an U.S. longwall coal mine: it was found that the roof strata act like a plate, not an individual block of the size of a shield dimension, as commonly assumed by all researchers and shield capacity is not a fixed property for a longwall panel or a mine or a coal seam. A new mechanism on the interaction between shield's hydraulic leg pressure and roof strata for shield loading is proposed. | Syd S.Peng Jingyi Cheng Feng Du Yuting Xue | 2019 | International Journal of Mining Science and Technology2019，29，1： | 7 |
| 2 | Guiding T lymphopoiesis from pluripotent stem cells by defined transcription factors显示文摘Achievement of immunocompetent and therapeutic T lymphopoiesis from pluripotent stem cells(PSCs)is a central aim in T cell regenerative medicine.To date,preferentially reconstituting T lymphopoiesis in vivo from PSCs remains a practical challenge.Here we documented that synergistic and transient expression of Runx1 and Hoxa9 restricted in the time window of endothelial-to-hematopoietic transition and hematopoietic maturation stages in a PSC differentiation scheme(iR9-PSC)in vitro induced preferential generation of engraftable hematopoietic progenitors capable of homing to thymus and developing into mature T cells in primary and secondary immunodeficient recipients.Single-cell transcriptome and functional analyses illustrated the cellular trajectory of T lineage induction from PSCs,unveiling the T-lineage specification determined at as early as hemogenic endothelial cell stage and identifying the bona fide pre-thymic progenitors.The induced T cells distributed normally in central and peripheral lymphoid organs and exhibited abundant TCRαβrepertoire.The regenerative T lymphopoiesis restored immune surveillance in immunodeficient mice.Furthermore,gene-edited iR9-PSCs produced tumor-specific T cells in vivo that effectively eradicated tumor cells.This study provides insight into universal generation of functional and therapeutic T cells from the unlimited and editable PSC source. | Rongqun Guo Fangxiao Hu Qitong Weng Cui Lv Hongling Wu Lijuan Liu Zongcheng Li Yang Zeng Zhijie Bai Mengyun Zhang Yuting Liu Xiaofei Liu Chengxiang Xia Tongjie Wang Peiqing Zhou Kaitao Wang Yong Dong Yuxuan Luo Xiangzhong Zhang Yuxian Guan Yang Geng Juan Du Yangqiu Li Yu Lan Jiekai Chen Bing Liu Jinyong Wang | 2020 | Cell Research2020，30，1： | 7 |
| 3 | Structural Surface Crack Monitoring Method Based on Electrical Potential Technique and Modern Surface Technology显示文摘Crack monitoring plays a great role in modern structural health monitoring, however, most of the conventional crack inspections have disadvantages in terms of the accuracy, expense, reliability, durability and level of instrumentation required. Thus, development of a simple and reliable crack inspection technique that allows continuous monitoring has been desired. In this paper, electrical potential technique and modern surface technology are employed together to develop a new structural surface crack monitoring method. A special crack monitoring coating sensor based on electrical potential technique was deposited on the hot spot of the structure by modern surface technology. The sensor consists of three layers: the isolated layer, the sensing layer and the protective layer. The isolated layer is prepared by anodic oxidation technology, the sensing layer is made of ion plated copper, and the protective layer is made of silicone. The thickness of each layer is at micrometer magnitude. The electrical conductivity of the sensor is very stable, and the fatigue performance of the specimen with or without coating sensor is nearly unchanged. The crack monitoring experiment result shows that there are two sudden rises of the coating sensor electrical potential values, corresponding to different stages of the crack initiation and propagation. Since the width of the surface coating sensor is only 0.5 mm, this crack monitoring sensor can detect the propagation of cracks less than 0.5 mm long. The method proposed takes the simplicity of electrical potential technique and can monitor surface crack of nearly all kinds of structures precisely. The results of this paper may form the basis of a new crack monitoring system. | CUI Ronghong HE Yuting YU Zhiming LI Hongpeng SHU Wenjun DU Jinqiang | 2011 | Chinese Journal of Mechanical Engineering2011，24，4： | 7 |
| 4 | Natural convection heat transfer of molten salt in a single energy storage tank显示文摘在在一辆柱体坦克的熔融的盐的热转移经由模拟和实验被学习在一辆单个精力存储坦克获得它的自然传送对流热转移。模拟和在一辆柱体坦克的水的自然传送对流热转移与 Garons 关联适合很好的试验性的结果表演。然而,当因为它的高粘性和低热电导率, Garons 关联被用来预言熔融的盐的自然传送对流热转移时,重要偏差发生。然而,熔融的盐的自然传送对流热转移的模仿的数据试验性的结果与那些适合很好。因此,考虑可变物理性质的效果的关联在这研究被建议预言熔融的盐的自然传送对流热转移。从建议关联的现在的数据的偏差是不到 d 控制模拟。在 summe 枼 ? 枼期间?? | LU YuanWei YU Qiang DU WenBin WU YuTing MA ChongFang | 2016 | Science China(Technological Sciences)2016，59，8： | 7 |
| 5 | No expenditure difference among patients with liver cancer at stageⅠ-ⅣV:Findings from a multicenter cross-sectional study in China显示文摘Objective:The number of liver cancer patients in China accounts for more than half of the world.However,China currently lacks national,multicenter economic burden data,and meanwhile,measuring the differences among different subgroups will be informative to formulate corresponding policies in liver cancer control.Thus,the aim of the study was to measure the economic burden of liver cancer by various subgroups.Methods:A hospital-based,multicenter and cross-sectional survey was conducted during 2012・2014,covering 39 hospitals and 21 project sites in 13 provinces across China.The questionnaire covers clinical information,sociology,expenditure,and related variables.All expenditure data were reported in Chinese Yuan(CNY)using 2014 values.Results:A total of 2,223 liver cancer patients were enrolled,of whom 59.61%were late-stage cases(III-IV),and 53.8%were hepatocellular carcinoma.The average total expenditure per liver cancer patient was estimated as 53,220 CNY,including 48,612 CNY of medical expenditures(91.3%)and 4,608 CNY of non-medical expenditures(8.7%).The average total expenditures in stage I,H,m and stage IV were 52,817 CNY,50,877 CNY,50,678 CNY and 54,089 CNY(P>0.05),respectively.Non-medical expenditures including additional meals,additional nutrition care,transportation,accommodation and hired informal nursing were 1,453 CNY,839 CNY,946 CNY,679 CNY and 200 CNY,respectively.The one-year out-of-pocket expenditure of a newly diagnosed patient was 24,953 CNY,and 77.2%of the patients suffered an unmanageable financial burden.Multivariate analysis showed that overall expenditure differed in almost all subgroups(P<0.05),except for sex,clinical stage,and pathologic type.Conclusions:There was no difference in treatment expenditure for liver cancer patients at different clinical stages,which suggests that maintaining efforts on treatment efficacy improvement is important but not enough.To fiirtherly reduce the overall economic burden from liver cancer,more effort should be given to primary and secondary prevention strategies. | Haike Lei Lin Lei Jufang Shi Yongzhong Wu Ling Liang Huiyao Huang Mei He Fangzhou Bai Maomao Cao Hui Qiu Yuting Wang Chengcheng Liu Jia Du Hong Wang Yan Zhang Mengdi Cao Ji Peng Ni Li Chunfeng Qu Min Dai Wanqing Chen Jie He | 2020 | Chinese Journal of Cancer Research2020，32，4： | 7 |
| 6 | Integrated genomic analysis identifies deregulated JAK/STAT-MYC-biosynthesis axis in aggressive NK-cell leukemia显示文摘好攻击的 NK 房间白血病(ANKL ) 是在从亚洲的人之中是更流行的 NK 房间瘤的一种稀罕形式并且中央并且南美洲。病人们通常在天以内死到月,甚至在收到迅速的治疗学的管理以后。这里,我们由集成整个染色体执行了 ANKL 的第一全面研究, transcriptome 并且定序指向,象功能的试金一样的 cytokine 数组。在 JAK-STAT 小径的变化在 48% 被识别(14/29 ) ANKL 病人,当细胞外的 STAT3 激发器 IL10 被 56 褶层的一般水准提高时(P < 0.0001 ) 在检查的所有病人的血浆。另外的经常变异的基因包括的 TP53 (34%) , TET2 (28%) , CREBBP (21%) 和 MLL2 (21%) 。耐心的 NK 白血病房间在多重新陈代谢的小径显示出 STAT3 phosphorylation, MYC 表示和 transcriptional 活动的突出的激活。机能上地, STAT3 激活和 MYC 表示为 ANKL 房间的增长和幸存是批评的。发信号的 STAT 调整了发信号的 MYC 抄写节目,和两 STAT, MYC 抄写被要求维持核苷酸合成和 glycolysis 的激活。一起, JAK-STAT 小径在 ANKL 为 genomic 改变和 IL10 刺激代表一个主要目标。这最新发现的 JAK/STAT-MYC-biosynthesis 轴可以在对待白血病的这种子类型为新奇治疗学的策略的发展提供机会。 | Liang Huang Dan Liu Na Wang Shaoping Ling Yuting Tang Jun Wu Lingtong Hao Hui Luo Xuelian Hu Lingshuang Sheng Lijun Zhu Di Wang Yi Luo Zhen Shang Min Xiao Xia Mao Kuangguo Zhou Lihua Cao Lili Dong Xinchang Zheng Pinpin Sui Jianlin He Shanlan Mo Jin Yan Qilin Ao Lugui Qiu Hongsheng Zhou Qifa Liu Hongyu Zhang Jianyong Li Jie Jin Li Fu Weili Zhao Jieping Chen Xin Du Guoliang Qing Hudan Liu Xin Liu Gang Huang Ding Ma Jianfeng Zhou Qian-fei Wang | 2018 | Cell Research2018，28，2： | 5 |
| 7 | COPII mitigates ER stress by promoting formation of ER whorls显示文摘Cells mitigate ER stress through the unfolded protein response(UPR).Here,we report formation of ER whorls as an effector mechanism of the ER stress response.We found that strong ER stress induces formation of ER whorls,which contain ER-resident proteins such as the Sec61 complex and PKR-like ER kinase(PERK).ER whorl formation is dependent on PERK kinase activity and is mediated by COPII machinery,which facilitates ER membrane budding to form tubular-vesicular ER whorl precursors.ER whorl precursors then go through Sec22b-mediated fusion to form ER whorls.We further show that ER whorls contribute to ER stressinduced translational inhibition by possibly modulating PERK activity and by sequestering translocons in a ribosome-free environment.We propose that formation of ER whorls reflects a new type of ER stress response that controls inhibition of protein translation. | Fang Xu Wanqing Du Qin Zou Yuting Wang Xin Zhang Xudong Xing Ying Li Dachuan Zhang Huimin Wang Wenhao Zhang Xinyao Hu Xin Liu Xiaoling Liu Shaojin Zhang Jinqiang Yu Jianhuo Fang Fajin Li Ying Zhou Tieqiang Yue Na Mi Haiteng Deng Peng Zou Xiaowei Chen Xuerui Yang Li Yu | 2021 | Cell Research2021，31，2： | 4 |
| 8 | INTERFERENCE BY NON-HOST PLANT ROOTS AND ROOT EXUDATES IN THE INFECTION PROCESSES OF PHYTOPHTHORA NICOTIANAE显示文摘Crop rotations are widely used because they can significantly reduce the incidence of pests and diseases.The interactions between non-host roots and pathogens may be key in the inhibition of soilborne pathogens in crop rotations.Interactions between fennel(Foeniculum vulgare)roots/root exudates and Phytophthora nicotianae were investigated because of the known allelopathy between fennel and tobacco(Nicotiana tabacum).The effects of the key compounds in the fennel rhizosphere on the mycelial growth and zoospore behavior of P.nicotianae were assessed.The roots of fennel attracted P.nicotianae zoospores and inhibited their motility and the germination of cystospores,with some cystospores rupturing.4-ethylacetophenone,vanillin and N-formylpiperidine were consistently identified in the fennel rhizosphere and were found to interfere with the infection of P.nicotianae,especially vanillin.Hyphae treated with these compounds produced more abnormal branches and accumulated reactive oxygen species.These interspecific interactions between non-host roots and pathogens were found to be an important factor in the inhibition by fennel of infection by P.nicotianae. | Yuxin YANG He ZHANG Yuting FANG Ying LI Xinyue MEI Huichuan HUANG Fei DU Shusheng ZHU Min YANG Yixiang LIU | 2021 | Frontiers of Agricultural Science and Engineering2021，8，3： | 3 |
| 9 | Heavy ion and X-ray irradiation alter the cytoskeleton and cytomechanics of cortical neurons显示文摘Heavy ion beams with high linear energy transfer exhibit more beneficial physical and biological performance than conventional X-rays, thus improving the potential of this type of radiotherapy in the treatment of cancer. However, these two radiotherapy modalities both cause inevitable brain injury. The objective of this study was to evaluate the effects of heavy ion and X-ray irradiation on the cytoskeleton and cytomechanical properties of rat cortical neurons, as well as to determine the potential mechanism of neuronal injury after irradiation. Cortical neurons from 30 new-born mice were irradiated with heavy ion beams at a single dose of 2 Gy and X-rays at a single dose of 4 Gy; subsequent evaluation of their effects were carried out at 24 hours after irradiation. An immunofluorescence assay showed that after irradiation with both the heavy ion beam and X-rays, the number of primary neurons was significantly decreased, and there was evidence of apoptosis. Radiation-induced neuronal injury was more apparent after X-irradiation. Under atomic force microscopy, the neuronal membrane appeared rough and neuronal rigidity had increased. These cell changes were more apparent following exposure to X-rays. Our findings indicated that damage caused by heavy ion and X-ray irradiation resulted in the structural distortion and rearrangement of the cytoskeleton, and affected the cytomechanical properties of the cortical neurons. Moreover, this radiation injury to normal neurons was much severer after irradiation with X-rays than after heavy ion beam irradiation. | Yuting Du Jie Zhang Qian Zheng Mingxin Li Yang Liu Baoping Zhang Bin Liu Hong Zhang Guoying Miao | 2014 | Neural Regeneration Research2014，9，11： | 3 |
| 10 | Effects of Angelica sinensis extracts on lipid oxidation in fish feeds and growth performance of juvenile Jian carp(Cyprinus carpio var. Jian)显示文摘The study was to explore the effect of the extracts of Angelica sinensis(EAs) on lipid oxidation in fish feeds compared with ethoxyquin(EQ) and the effect of dietary EAs on growth performance of carp(Cyprinus carpio var. Jian). Firstly, fish feeds were respectively added with EQ, and ethyl ether extract ethyl acetate extract(EAE), acetone extract, ethanol extract(EE) and aqueous extract(AQE) of Angelica sinensis, except for the control. The results showed that EAs and EQ inhibited lipid oxidation in fish feed(P < 0.05). Of all of the examined EAs, EAE showed the strongest protective effects against lipid oxidation(P < 0.05). Moreover, EAE at high concentrations showed a stronger effect on lipid oxidation compared with EQ(P < 0.05). Then, 7 experimental diets respectively supplemented with 0.0, 1.0, 2.0, 3.0, 4.0, 5.0 and 6.0 g/kg of EAE were fed to the respective treatment groups for 30 d. Four replicates were performed for each treatment group; 20 carp(mean weight: 12.10 ± 0.13 g) were in each replicate. The result indicated that dietary EAE improved the growth performance in carp(P < 0.05). The appropriate con centration of EAE for carp growth was estimated to be 3.643 g/kg diet. Thus, EAE could be used as a natural antioxidant in feeds for Jian carp. | Huatao Li Dandan Yang Zhihao Li Mingquan He Fengyi Li Jun Jiang Siyi Tang Peiyuan Peng Wenhao Du Yuting Ma Ying Liu | 2019 | Animal Nutrition2019，，1： | 2 |
| 11 | Damage-Monitoring Forward Equivalent-model Construction of Rosette Eddy Current Sensors显示文摘结构损伤监测对于保证结构安全是极其重要的。针对金属螺栓连接结构中螺栓孔位置处的裂纹损伤定量监测需求,在Goldfine等人的基础之上,该文提出一种花萼状涡流传感器,构建了传感器损伤监测正向等效模型并通过搭建实验装置验证损伤监测正向等效模型准确性并进行误差分析。相对于传统的多层导电结构谐波涡流场的积分/级数解析模型,构建的损伤监测正向等效模型考虑了在高频激励下导线电流密度分布的集肤效应,并可用于互感式涡流传感器建模。实验结果表明:对测量结果经空气标定后,传感器贴于2A12-T4标准试件表面时的模型计算结果和实验结果较为吻合,第1、2和3感应通道的幅值比量模型计算结果误差随频率变化均在10%以内,第4感应通道的幅值比量模型计算结果误差随频率变化在15%以内。 | DING Hua HE Yuting JIAO Shenbo DU Jingqiang | 2013 | 中国电机工程学报2013，33，9： | 2 |
| 12 | Effect of conformable substrate thickness on an eddy current sensor array′s output characteristics显示文摘 | Du Jinqiang He Yuting Ding Hua | 2011 | Applied Mechanics and Materials2011，，： | 1 |
| 13 | Prepara- tion of ZnO: Eu3+ nanospheres via a micro - emulsion method and analysis of the photoluminescence properties 显示文摘 | Zhao Shihua Du Xuelian Cui Yuting | 2014 | Journal of Nanoscience and Nanotechnology2014，14，5： | 1 |
| 14 | Simulation analysis of an eddy current sensor array based on finite element method 显示文摘 | Du Jinqiang He Yuting Ding Hua | 2011 | Materials and Manufacturing2011，，： | 1 |
| 15 | Progress of polymer reaction engineering:From process engineering to product engineering显示文摘Polymer reaction engineering studies the design,operation,and optimization of reactors for industrial scale polymerization,based on the theory of polymerization kinetics and transfer processes(e.g.,flow,heat and mass transfer).Although the foundation and development of this discipline are less than80 years,the global production of polymers has exceeded 400 million tons per annum.It demonstrates that polymer reaction engineering is of vital importance to the polymer industry.Along with the matu rity of production processes and market saturation for bulk polymers,emerging industries such as information technology,modern transportation,biomedicine,and new energy have continued to develop.As a result,the research objective for polymer reaction engineering has gradually shifted from maximizing the efficiency of the polymerization process to the precise regulation of high-end product-oriented macro molecules and their aggregation structures,i.e.,from polymer process engineering to polymer product engineering.In this review,the frontiers of polymer reaction engineering are introduced,including the precise regulation of polymer chain structure,the control of primary aggregation structure,and the rational design of polymer products.We narrow down the topic to the polymerization reaction engineering of vinyl monomers.Moreover,the future prospects are provided for the field of polymer reaction engineering. | Pingwei Liu Jigang Du Yuting Ma Qingyue Wang Khak Ho Lim Bo-Geng Li | 2022 | Chinese Journal of Chemical Engineering2022，，10： | 1 |
| 16 | Experimental investigation of the isothermal section at 400℃of the Mgsingle bondCesingle bondSr ternary system显示文摘The objective of this study is to determine the isothermal section at 400℃ of the Mgsingle bondCesingle bondSr system.In this study,the constitution of the Cesingle bondSr system and the Mgsingle bondCesingle bondSr system have been investigated over the entire composition range using X-ray diffraction(XRD),field emission scanning electron microscope(SEM)and energy dispersive spectroscopy(EDS).No any new binary compound has been found in the Cesingle bondSr system and no ternary compound has been found in the Mgsingle bondCesingle bondSr system also.Nine three-phase regions have been experimentally observed.Six binary phases Mg_(2)Sr,Mg_(23)Sr_(6),Mg_(38)Sr_(9),Mg_(17)Sr_(2),Mg_(12)Ce,Mg_(41)Ce_(5) are detected dissolving about 3-7 at.%the third element.This study first detected the experimental data of the Cesingle bondSr binary system and determined the isothermal section at 400℃ of the Mgsingle bondCesingle bondSr ternary system. | Songxiang Sun Yuting Qin Hua Zhou Yong Du Cuiyun He | 2016 | Journal of Magnesium and Alloys2016，4，1： | 1 |
| 17 | Development of corrector magnet power supply for high energy photon source显示文摘Purpose High Energy Photon Source(HEPS)requires high quality,high energy beam and ultra-low emittance of 0.1 nm·rad,which puts forward high demand for power supply.In this paper,a high-performance corrector magnet power supply is developed to calibrate and adjust beam track within a certain bandwidth range to ensure the stability of beam track.Methods The prototype of power supply adopts the new'One control Two'control mode,which adjusts the performance of two power supplies simultaneously based on digital control.Results The experimental results show that the stability of the power supply is lower than 20 ppm,which is far better than the design index.Voltage ripple is less than 10 mV,and other performance indexes meet the physical design requirements,which can well meet the requirements of HEPS construction.Conclusions After a lot of experiments and tests,all the parameters passed the design indicators.The successful development of this power supply has laid a foundation for the successful application of HEPS. | Han Chao Long Fengli Gao Yao Wei Pengfei Liu Yuting Guo Xiaoling Chen Suying Du Yunze | 2022 | Radiation Detection Technology and Methods2022，6，4： | 1 |
| 18 | Functional nucleic acid-based cell imaging and manipulation显示文摘Cells are the basic structural and functional units of organisms.Dynamic analysis and manipulation of specific components in living cells would provide valuable information for the study of related biological processes.Advances in fluorescence microscopy have allowed real-time monitoring of biological events at the molecular level.Meanwhile,the development of highperformance fluorescence probes has become a critical issue.Functional nucleic acids(FNAs)are oligonucleotides with special chemical and biological functions,and aptamers with excellent molecular recognition capability are one of the most important representatives.They have attracted extensive attention in the field of live-cell study,owing to intrinsic advantages of simple synthesis,convenient modification,low immunogenicity and high programmability.This review focuses on recent research progress in fluorescence imaging and manipulation of cells using FNAs,particularly aptamers,as the molecular tools.Finally,a summary is provided and the related challenges are discussed. | Yan Zhou Yuting Zhuo Ruizi Peng Yutong Zhang Yulin Du Qiang Zhang Yue Sun Liping Qiu | 2021 | Science China Chemistry2021，64，11： | 1 |
| 19 | Tuning Surface Spin Polarization of CoFeB by Boron Diffusion Detected by Spin Resolved Photoemission显示文摘Research of spin polarization of magnetic CoFeB thin films is of practical importance in spintronic applications.Here,using a direct characterization technique of spin-resolved photoemission spectroscopy,we obtain the surface spin polarization of amorphous Co_(40)Fe_(40)B_(20)thin films with different annealing temperatures from 100℃to 500℃prepared by magnetron sputtering.After high annealing temperature,a quasi-semiconductor state is gradually formed at the CoFeB surface due to the boron diffusion.While the global magnetization remains almost constant,the secondary electrons’spin polarization,average valence band spin polarization and the spin polarization at Fermi level from spin-resolved photoemission spectroscopy show a general trend of decreasing with the increasing annealing temperature above 100℃.These distinct surface properties are attributed to the enhanced Fe-B bonding due to the boron segregation upon surface after annealing as confirmed by x-ray photoelectron spectroscopy and scanning transmission electron microscopy with energy dispersive spectroscopy.Our findings provide insight into the surface spin-resolved electronic structure of the CoFeB thin films,which should be important for development of high-performance magnetic random-access memories. | Qi Liu Xianyang Lu Chengrui Fu Jiarui Chen Zhe Zhang Yuting Gong Xinyue Wang Yu Yan Qinwu Gao Hui Li Xuezhong Ruan Yao Li Jun Du Jing Wu Liang He Bo Liu Rong Zhang Yongbing Xu | 2023 | Chinese Physics Letters2023，40，8： | 0 |
| 20 | Developing high-Q × f value MgNb_(2–x)Ta_(x)O_(6)(0≤x≤0.8) columbite ceramics and clarifying the impact mechanism of dielectric loss: Crystal structure, Raman vibrations, microstructure, lattice defects, chemical bond characteristics, structural parameters, and microwave dielectric properties in-depth studies显示文摘With the increasing frequency of wireless mobile communication,dielectric materials with higher Q×f are required to enhance the signal strength of microwave passive devices and thus compensate for the rapid attenuation of high-frequency signals during propagation.In order to improve the Q×f of the MgNb2O6 system and study the internal mechanism between the structure and microwave dielectric properties,Ta5+ion is introduced to design and fabricate MgNb_(2-x)Ta_(x)O_(6)(0≤x≤0.8)ceramics by the solid-state reaction method.The single columbite phase and dense structure are observed throughout the entire composition range.All elements(Mg,Nb,Ta,and O)can be detected by X-ray photoelectron spectroscopy.Insights from the Raman spectroscopy and group theoretical analysis reveal that the Ag(2)and Ag(3)modes located at∼905 cm−1 dominate the Raman vibration.In addition,theɛr depends on the polarizability reflected by the C–M equation and Raman shift.Theτf closely relates to the bond energy of the Nb/Ta–O bond and restoring force characterized by average octahedral distortion of[Nb/TaO6].Notably,the crucial factors for the huge improvement of Q×f are clarified deeply,in terms of the lower internal strain,the reduced ordering-induced domain size,and the chemical bond valence closer to the ionic valence state,which promotes the stability of crystal structure.Moreover,the introduction of lower electronegative ions enhances the ability of electrons to compensate for oxygen vacancies,thereby reducing the dielectric loss caused by the conductance.Excellent microwave properties(ɛr=19.2,Q×f=170,000 GHz,andτf=−55.6 ppm℃–1)are achieved in MgNb1.4Ta0.6O6 ceramic,specifically a nearly 40%increase in the Q×f.This work has enriched the theory associated with low dielectric loss and provided the MgNb_(1.4)Ta_(0.6)O_(6) ceramic with a pretty high-Q×f for the application in the design of the 5G/6G wireless communication devices. | Lingxia Li Yuting Li Jianli Qiao Mingkun Du | 2023 | Journal of Materials Science & Technology2023，，15： | 0 |
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